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Register a new userOpportunities to constrain astrophysical reaction rates for the s-process through determination of the ground state cross sections
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Modern models of s-process nucleosynthesis in stars require stellar reaction rates with high precision. Most of the neutron capture cross sections in the s-process have been measured and for an increasing number of reactions the required precision is achieved. This does not necessarily mean, however, that the stellar rates are constrained equally well because only capture on the ground state of a target is measured in the laboratory. Captures on excited states can considerably contribute to stellar rates already at typical s-process temperatures. We show that the ground state contribution X to a stellar rate is the relevant measure to identify reactions which are or could be well constrained by experiments and apply it to (n,gamma) reactions in the s-process. It is further shown that the maximally possible reduction in uncertainty of a rate through determination of the g.s. cross section is directly given by X. An error analysis of X is presented and it is found that X is a robust measure with overall small uncertainties. Several specific examples (neutron capture on 79Se, 95Zr, 121Sn, 187Os, and 193Pt) are discussed in detail. The ground state contributions for a set of 411 neutron capture reactions around the s-process path are presented in a table. This allows to identify reactions which may be better constrained by experiments and such which cannot be constrained by only measuring ground state cross sections (and thus require supplementary studies). General trends and implications are discussed.
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The total cross sections for the 120Te(p,gamma)121I and 120Te(p,n)120I reactions have been measured by the activation method in the effective center-of-mass energies between 2.47 MeV and 7.93 MeV. The targets were prepared by evaporation of 99.4 % isotopically enriched 120Te on Aluminum and Carbon backing foils, and bombarded with proton beams provided by the FN tandem accelerator at the University of Notre Dame. The cross sections and $S$ factors were deduced from the observed gamma ray activity, which was detected off-line by two Clover HPGe detectors mounted in close geometry. The results are presented and compared with the predictions of statistical model calculations using the codes NON-SMOKER and TALYS.
The composition of the early Solar System can be inferred from meteorites. Many elements heavier than iron were formed by the rapid neutron-capture process (r process), but the astrophysical sources where this occurred remain poorly understood. We demonstrate that the near-identical half-lives ($simeq$ 15.6 Myr) of the radioactive r-process nuclei 129I and 247Cm preserve their ratio, irrespective of the time between production and incorporation into the Solar System. We constrain the last r-process source by comparing the measured meteoritic 129I / 247Cm = 438 $pm$ 184 to nucleosynthesis calculations based on neutron star merger and magneto-rotational supernova simulations. Moderately neutron-rich conditions, often found in merger disk ejecta simulations, are most consistent with the meteoritic value. Uncertain nuclear physics data limit our confidence in this conclusion.
Direct neutron capture on 62Ni is calculated in the DWBA and the cross sections in the energy range relevant for s-process nucleosynthesis are given. It is confirmed that the thermal value of the capture cross section contains a subthreshold resonance contribution. Contrary to previous investigations it is found that the capture at higher energies is dominated by p-waves, thus leading to a considerably increased cross section at s-process energies and a modified energy dependence.
It has been suggested that a $ u$p process can occur when hot, dense, and proton-rich matter is expanding within a strong flux of anti-neutrinos. In such an environment, proton-rich nuclides can be produced in sequences of proton captures and (n,p) reactions, where the free neutrons are created in situ by $overline{ u}_mathrm{e}+mathrm{p} rightarrow mathrm{n}+mathrm{e}^+$ reactions. The detailed hydrodynamic evolution determines where the nucleosynthesis path turns off from N = Z line and how far up the nuclear chart it runs. In this work, the uncertainties on the final isotopic abundances stemming from uncertainties in the nuclear reaction rates were investigated in a large-scale Monte Carlo approach, simultaneously varying ten thousand reactions. A large range of model conditions was investigated because a definitive astrophysical site for the $ u$p process has not yet been identified. The present parameter study provides, for each model, identification of the key nuclear reactions dominating the uncertainty for a given nuclide abundance. As all rates appearing in the $ u$p process involve unstable nuclei, and thus only theoretical rates are available, the final abundance uncertainties are larger than those for nucleosynthesis processes closer to stability. Nevertheless, most uncertainties remain below a factor of three in trajectories with robust nucleosynthesis. More extreme conditions allow production of heavier nuclides but show larger uncertainties because of the accumulation of the uncertainties in many rates and because the termination of nucleosynthesis is not at equilibrium conditions. It is also found that the solar ratio of the abundances of ${}^{92}$Mo and ${}^{94}$Mo could be reproduced within uncertainties.
The stellar (n,gamma) cross section of 40Ca at kT=25 keV has been measured with a combination of the activation technique and accelerator mass spectrometry (AMS). This combination is required when direct off-line counting of the produced activity is compromised by the long half-life and/or missing gamma-ray transitions. The neutron activations were performed at the Karlsruhe Van de Graaff accelerator using the quasistellar neutron spectrum of kT=25 keV produced by the 7Li(p,n)7Be reaction. The subsequent AMS measurements were carried out at the Vienna Environmental Research Accelerator (VERA) with a 3 MV tandem accelerator. The doubly magic 40Ca is a bottle-neck isotope in incomplete silicon burning, and its neutron capture cross section determines the amount of leakage, thus impacting on the eventual production of iron group elements. Because of its high abundance, 40Ca can also play a secondary role as neutron poison for the s-process. Previous determinations of this value at stellar energies were based on time-of-flight measurements. Our method uses an independent approach, and yields for the Maxwellian-averaged cross section at kT=30 keV a value of <sigma>30 keV= 5.73+/-0.34 mb.
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