Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userComplex electronic states in double layered ruthenates (Sr1-xCax)3Ru2O7
131
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
The magnetic ground state of (Sr$_{1-x}$Ca$_x$)$_3$Ru$_2$O$_7$ (0 $leq x leq$ 1) is complex, ranging from an itinerant metamagnetic state (0 $leq x <$ 0.08), to an unusual heavy-mass, nearly ferromagnetic (FM) state (0.08 $< x <$ 0.4), and finally to an antiferromagnetic (AFM) state (0.4 $leq x leq$ 1). In this report we elucidate the electronic properties for these magnetic states, and show that the electronic and magnetic properties are strongly coupled in this system. The electronic ground state evolves from an AFM quasi-two-dimensional metal for $x =$ 1.0, to an Anderson localized state for $0.4 leq x < 1.0$ (the AFM region). When the magnetic state undergoes a transition from the AFM to the nearly FM state, the electronic ground state switches to a weakly localized state induced by magnetic scattering for $0.25 leq x < 0.4$, and then to a magnetic metallic state with the in-plane resistivity $rho_{ab} propto T^alpha$ ($alpha >$ 2) for $0.08 < x < 0.25$. The system eventually transforms into a Fermi liquid ground state when the magnetic ground state enters the itinerant metamagnetic state for $x < 0.08$. When $x$ approaches the critical composition ($x sim$ 0.08), the Fermi liquid temperature is suppressed to zero Kelvin, and non-Fermi liquid behavior is observed. These results demonstrate the strong interplay between charge and spin degrees of freedom in the double layered ruthenates.
rate research
Read More
We report an unusual nearly ferromagnetic, heavy-mass state with a surprisingly large Wilson ratio $R_{textrm{w}}$ (e.g., $R_{textrm{w}}sim$ 700 for $x =$ 0.2) in double layered ruthenates (Sr$_{1-x}$Ca$_{x}$)$_{3}$Ru$_{2}$O$_{7}$ with 0.08 $< x <$ 0.4. This state does not evolve into a long-range ferromagnetically ordered state despite considerably strong ferromagnetic correlations, but freezes into a cluster-spin-glass at low temperatures. In addition, evidence of non-Fermi liquid behavior is observed as the spin freezing temperature of the cluster-spin-glass approaches zero near $x approx$ 0.1. We discuss the origin of this unique magnetic state from the Fermi surface information probed by Hall effect measurements.
We present a detailed investigation of the specific heat in Ca$_3$(Ru$_{1-x}M_x$)$_2$O$_7$ ($M$ = Ti, Fe, Mn) single crystals. With different dopants and doping levels, three distinct regions are present, including a quasi-2D metallic state with an antiferromagnetic (AFM) order formed by ferromagnetic bilayers (AFM-$b$), a Mott insulating state with G-type AFM order (G-AFM) and a localized state with a mixed AFM-b and G-AFM phase. Our specific heat data provide deep insights into the Mott transitions induced by Ti and Mn dopings. We observed not only an anomalous large mass enhancement but also an additional term in the specific heat i.e. $Cpropto T^2$ in the localized region. The $Cpropto T^2$ term is most likely due to the long-wavelength excitations with both FM and AFM components. A decrease of Debye temperature is observed in the G-type AFM region, indicating a lattice softening associated with the Mott transition.
Mesoscopic irregularly ordered and even amorphous self-assembled electronic structures were recently reported in two-dimensional metallic dichalcogenides (TMDs), created and manipulated with short light pulses or by charge injection. Apart from promising new all-electronic memory devices, such states are of great fundamental importance, since such aperiodic states cannot be described in terms of conventional charge-density-wave (CDW) physics. In this paper we address the problem of metastable mesoscopic configurational charge ordering in TMDs with a sparsely filled charged lattice gas model in which electrons are subject only to screened Coulomb repulsion. The model correctly predicts commensurate CDW states corresponding to different TMDs at magic filling fractions $f_m=1/3,1/4,1/9,1/13,1/16$. Doping away from $f_m$ results either in multiple near-degenerate configurational states, or an amorphous state at the correct density observed by scanning tunnelling microscopy. Quantum fluctuations between degenerate states predict a quantum charge liquid at low temperatures, revealing a new generalized viewpoint on both regular, irregular and amorphous charge ordering in transition metal dichalcogenides.
We have performed non-resonant x-ray diffraction, resonant soft and hard x-ray magnetic diffraction, soft x-ray absorption and x-ray magnetic circular dichroism measurements to clarify the electronic and magnetic states of the Co3+ ions in GdBaCo2O5.5. Our data are consistent with a 3+ Py Co HS state at the pyramidal sites and a 3+ Oc Co LS state at the octahedral sites. The structural distortion, with a doubling of the a axis (2ap x 2ap x 2ap cell), shows alternating elongations and contractions of the pyramids and indicates that the metal-insulator transition is associated with orbital order in the t2g orbitals of the 3+ Py Co HS state. This distortion corresponds to an alternating ordering of xz and yz orbitals along the a and c axes for the 3+ Py Co . The orbital ordering and pyramidal distortion lead to deformation of the octahedra, but the 3+ Oc Co LS state does not allow an orbital order to occur for the 3+ Oc Co ions. The soft x-ray magnetic diffraction results indicate that the magnetic moments are aligned in the ab plane but are not parallel to the crystallographic a or b axes. The orbital order and the doubling of the magnetic unit cell along the c axis support a non-collinear magnetic structure. The x-ray magnetic circular dichroism data indicate that there is a large orbital magnetic contribution to the total ordered Co moment.
The structure of the low-energy electronic states in layered cobaltates is considered starting from the Mott insulating limit. We argue that the coherent part of the wave-functions and the Fermi-surface topology at low doping are strongly influenced by spin-orbit coupling of the correlated electrons on the $t_{2g}$ level. An effective t-J model based on mixed spin-orbital states is radically different from that for the cuprates, and supports unconventional, pseudospin-triplet pairing.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
