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Register a new userSuperconducting properties of Fe-based layered superconductor LaO$_{0.9}$F$_{0.1-delta}$FeAs
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We have employed a new route to synthesize single phase F-doped LaOFeAs compound and confirmed the superconductivity above 20 K in this Fe-based system. We show that the new superconductor has a rather high upper critical field of about 54 T. A clear signature of superconducting gap opening below T$_c$ was observed in the far-infrared reflectance spectra, with 2$Delta/textit{k}T_capprox$3.5-4.2. Furthermore, we show that the new superconductor has electron-type conducting carrier with a rather low carrier density.
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We present point-contact spectroscopy data for junctions between a normal metal and the newly discovered F-doped superconductor LaO$_{0.9}$F$_{0.1-delta}$FeAs (F-LaOFeAs). A zero-bias conductance peak was observed and its shape and magnitude suggests the presence of Andreev bound states at the surface of F-LaOFeAs, which provides a possible evidence of an unconventional pairing symmetry with a nodal gap function. The maximum gap value $Delta_0approx3.9pm0.7$meV was determined from the measured spectra, in good agreement with the recent experiments on specific heat and lower critical field.
We have performed 75As Nuclear Magnetic Resonance (NMR) measurements on aligned powders of the new LaO0.9F0.1FeAs superconductor. In the normal state, we find a strong temperature dependence of the spin shift and Korringa behavior of the spin lattice relaxation rate. In the superconducting state, we find evidence for line nodes in the superconducting gap and spin-singlet pairing. Our measurements reveal a strong anisotropy of the spin lattice relaxation rate, which suggest that superconducting vortices contribute to the relaxation rate when the field is parallel to the c-axis but not for the perpendicular direction.
We report the specific heat measurements on the newly discovered Fe-based layered superconductor LaO_0.9F_{0.1-delta}FeAs with the onset transition temperature T_c approx 28 K. A nonlinear magnetic field dependence of the electronic specific heat coefficient gamma(H) has been found in the low temperature limit, which is consistent with the prediction for a nodal superconductor. The maximum gap value Delta_0 approx 3.4$pm$0.5 meV was derived by analyzing gamma(H) based on the d-wave model. We also detected the electronic specific heat difference between 9 T and 0 T in wide temperature region, a specific heat anomaly can be clearly observed near T_c. The Debye temperature of our sample was determined to be about 315.7 K. Our results suggest an unconventional mechanism for this new superconductor.
Using angle-integrated photoemission spectroscopy we have probed the novel LaO$_{0.9}$F$_{0.1}$FeAs superconductor over a wide range of photon energies and temperatures. We have provided the first full characterization of the orbital character of the VB DOS and of the magnitude of the d-p hybridization energy. Finally, we have identified two characteristic temperatures: 90K where a pseudogap-like feature appears to close and 120K where a sudden change in the DOS near E$_F$ occurs. We associate these phenomena with the SDW magnetic ordering and the structural transition seen in the parent compound, respectively. These results suggest the important role of electron correlation, spin physics and structural distortion in the physics of Fe-based superconductors.
We have studied the newly found superconductor compound LaO$_{1-x}$F$_x$FeAs through the first-principles density functional theory calculations. We find that the parent compound LaOFeAs is a quasi-2-dimensional antiferromgnetic semimetal with most carriers being electrons and with a magnetic moment of $2.3mu_B$ located around each Fe atom on the Fe-Fe square lattice. Furthermore this is a commensurate antiferromagnetic spin density wave due to the Fermi surface nesting, which is robust against the F-doping. The observed superconduction happens on the Fe-Fe antiferromagnetic layer, suggesting a new superconductivity mechanism, mediated by the spin fluctuations. An abrupt change on the Hall measurement is further predicted for the parent compound LaOFeAs.
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