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Kinks in the dispersion of strongly correlated electrons

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 Added by Marcus Kollar
 Publication date 2006
  fields Physics
and research's language is English




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The properties of condensed matter are determined by single-particle and collective excitations and their interactions. These quantum-mechanical excitations are characterized by an energy E and a momentum hbar k which are related through their dispersion E_k. The coupling of two excitations may lead to abrupt changes (kinks) in the slope of the dispersion. Such kinks thus carry important information about interactions in a many-body system. For example, kinks detected at 40-70 meV below the Fermi level in the electronic dispersion of high-temperature superconductors are taken as evidence for phonon or spin-fluctuation based pairing mechanisms. Kinks in the electronic dispersion at binding energies ranging from 30 to 800 meV are also found in various other metals posing questions about their origins. Here we report a novel, purely electronic mechanism yielding kinks in the electron dispersions. It applies to strongly correlated metals whose spectral function shows well separated Hubbard subbands and central peak as, for example, in transition metal-oxides. The position of the kinks and the energy range of validity of Fermi-liquid (FL) theory is determined solely by the FL renormalization factor and the bare, uncorrelated band structure. Angle-resolved photoemission spectroscopy (ARPES) experiments at binding energies outside the FL regime can thus provide new, previously unexpected information about strongly correlated electronic systems.



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We investigate the origin of ubiquitous low energy kinks found in Angle Resolved Photoemission (ARPES) experiments in a variety of correlated matter. Such kinks are unexpected from weakly interacting electrons and hence identifying their origin should lead to fundamental insights in strongly correlated matter. We devise a protocol for extracting the kink momentum and energy from the experimental data which relies solely on the two asymptotic tangents of each dispersion curve, away from the feature itself. It is thereby insensitive to the different shapes of the kinks as seen in experiments. The body of available data is then analyzed using this method. We proceed to discuss two alternate theoretical explanations of the origin of the kinks. Some theoretical proposals invoke local Bosonic excitations (Einstein phonons or other modes with spin or charge character), located exactly at the energy of observed kinks, leading to a momentum independent self energy of the electrons. A recent alternate is the theory of extremely correlated Fermi liquids (ECFL). This theory predicts kinks in the dispersion arising from a momentum dependent self energy of correlated electrons. We present the essential results from both classes of theories, and identify experimental features that can help distinguish between the two mechanisms. The ECFL theory is found to be consistent with currently available data on kinks in the nodal direction of cuprate superconductors, but conclusive tests require higher resolution energy distribution curve data.
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