Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userContiguous 3d and 4f magnetism: towards strongly correlated 3d electrons in YbFe2Al10
127
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
We present magnetization, specific heat, and 27Al NMR investigations on YbFe2Al10 over a wide range in temperature and magnetic field. The magnetic susceptibility at low temperatures is strongly enhanced at weak magnetic fields, accompanied by a ln(T0/T) divergence of the low-T specific heat coefficient in zero field, which indicates a ground state of correlated electrons. From our hard X-ray photo emission spectroscopy (HAXPES) study, the Yb valence at 50 K is evaluated to be 2.38. The system displays valence fluctuating behavior in the low to intermediate temperature range, whereas above 400 K, Yb3+ carries a full and stable moment, and Fe carries a moment of about 3.1 mB. The enhanced value of the Sommerfeld Wilson ratio and the dynamic scaling of spin-lattice relaxation rate divided by T [27(1/T1T)] with static susceptibility suggests admixed ferromagnetic correlations. 27(1/T1T) simultaneously tracks the valence fluctuations from the 4f -Yb ions in the high temperature range and field dependent antiferromagnetic correlations among partially Kondo screened Fe 3d moments at low temperature, the latter evolve out of an Yb 4f admixed conduction band.
rate research
Read More
Strong spin-orbit coupling fosters exotic electronic states such as topological insulators and superconductors, but the combination of strong spin-orbit and strong electron-electron interactions is just beginning to be understood. Central to this emerging area are the 5d transition metal iridium oxides. Here, in the pyrochlore iridate Pr2Ir2O7, we identify a nontrivial state with a single point Fermi node protected by cubic and time-reversal symmetries, using a combination of angle-resolved photoemission spectroscopy and first principles calculations. Owing to its quadratic dispersion, the unique coincidence of four degenerate states at the Fermi energy, and strong Coulomb interactions, non-Fermi liquid behavior is predicted, for which we observe some evidence. Our discovery implies that Pr2Ir2O7 is a parent state that can be manipulated to produce other strongly correlated topological phases, such as topological Mott insulator, Weyl semi-metal, and quantum spin and anomalous Hall states.
Soft x-ray resonant scattering has been used to examine the charge and magnetic interactions in the cycloidal antiferromagnetic compound dyfeal. By tuning to the Dy $M_4$ and $M_5$ absorption edges and the Fe L(2) and L(3) absorption edges we can directly observe the behavior of the Dy 4f and Fe 3d electron shells. Magnetic satellites surrounding the (110) Bragg peak were observed below 60 K. The diffraction peaks display a complex spectra at the Dy M(5) edge, indicative of a split 4f electron band. This is in contrast to a simple resonance observed at the Fe L(3) absorption edge, which probes the Fe 3d electron shell. Temperature dependant measurements detail the ordering of the magnetic moments on both the iron and the dysprosium antiferromagnetic cycloids. The ratio between the intensities of the Dy M(4) and M(5) remained constant throughout the temperature range, in contrast to a previous study conducted at the Dy L(2,3) edges. Our results demonstrate the ability of soft x-ray diffraction to separate the individual magnetic components in complicated multi-element magnetic structures.
Ferromagnetism and superconductivity are in most cases adverse. However, recent experiments reveal that they coexist at interfaces of LaAlO3 and SrTiO3. We analyze the magnetic state within density functional theory and provide evidence that magnetism is not an intrinsic property of the two-dimensional electron liquid at the interface. We demonstrate that the robust ferromagnetic state is induced by the oxygen vacancies in SrTiO3- or in the LaAlO3-layer. This allows for the notion that areas with increased density of oxygen vacancies produce ferromagnetic puddles and account for the previous observation of a superparamagnetic behavior in the superconducting state.
The idea of exciton condensation in solids was introduced in 1960s with the analogy to superconductivity in mind. While exciton supercurrents have been realized only in artificial quantum-well structures so far, the application of the concept of excitonic condensation to bulk solids leads to a rich spectrum of thermodynamic phases with diverse physical properties. In this review we discuss recent developments in the theory of exciton condensation in systems described by Hubbard-type models. In particular, we focus on the connections to their various strong-coupling limits that have been studied in other contexts, e.g., cold atoms physics. One of our goals is to provide a dictionary which would allow the reader to efficiently combine results obtained in these different fields.
The properties of condensed matter are determined by single-particle and collective excitations and their interactions. These quantum-mechanical excitations are characterized by an energy E and a momentum hbar k which are related through their dispersion E_k. The coupling of two excitations may lead to abrupt changes (kinks) in the slope of the dispersion. Such kinks thus carry important information about interactions in a many-body system. For example, kinks detected at 40-70 meV below the Fermi level in the electronic dispersion of high-temperature superconductors are taken as evidence for phonon or spin-fluctuation based pairing mechanisms. Kinks in the electronic dispersion at binding energies ranging from 30 to 800 meV are also found in various other metals posing questions about their origins. Here we report a novel, purely electronic mechanism yielding kinks in the electron dispersions. It applies to strongly correlated metals whose spectral function shows well separated Hubbard subbands and central peak as, for example, in transition metal-oxides. The position of the kinks and the energy range of validity of Fermi-liquid (FL) theory is determined solely by the FL renormalization factor and the bare, uncorrelated band structure. Angle-resolved photoemission spectroscopy (ARPES) experiments at binding energies outside the FL regime can thus provide new, previously unexpected information about strongly correlated electronic systems.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
