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Register a new userStimulated and spontaneous optical generation of electron spin coherence in charged GaAs quantum dots
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We report on the coherent optical excitation of electron spin polarization in the ground state of charged GaAs quantum dots via an intermediate charged exciton (trion) state. Coherent optical fields are used for the creation and detection of the Raman spin coherence between the spin ground states of the charged quantum dot. The measured spin decoherence time, which is likely limited by the nature of the spin ensemble, approaches 10 ns at zero field. We also show that the Raman spin coherence in the quantum beats is caused not only by the usual stimulated Raman interaction but also by simultaneous spontaneous radiative decay of either excited trion state to a coherent combination of the two spin states.
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High-resolution spectral hole burning (SHB) in coherent nondegenerate differential transmission spectroscopy discloses spin-trion dynamics in an ensemble of negatively charged quantum dots. In the Voigt geometry, stimulated Raman spin coherence gives rise to Stokes and anti-Stokes sidebands on top of the trion spectral hole. The prominent feature of an extremely narrow spike at zero detuning arises from spin population pulsation dynamics. These SHB features confirm coherent electron spin dynamics in charged dots, and the linewidths reveal spin spectral diffusion processes.
We study in theory the generation and detection of electron spin coherence in nonlinear optical spectroscopy of semiconductor quantum dots doped with single electrons. In third-order differential transmission spectra, the inverse width of the ultra-narrow peak at degenerate pump and probe frequencies gives the spin relaxation time ($T_1$), and that of the Stoke and anti-Stoke spin resonances gives the effective spin dephasing time due to the inhomogeneous broadening ($T_2^*$). The spin dephasing time excluding the inhomogeneous broadening effect ($T_2$) is measured by the inverse width of ultra-narrow hole-burning resonances in fifth-order differential transmission spectra.
Electron spin coherence has been generated optically in n-type modulation doped (In,Ga)As/GaAs quantum dots (QDs) which contain on average a single electron per dot. The coherence arises from resonant excitation of the QDs by circularly-polarized laser pulses, creating a coherent superposition of an electron and a trion state. Time dependent Faraday rotation is used to probe the spin precession of the optically oriented electrons about a transverse magnetic field. Spin coherence generation can be controlled by pulse intensity, being most efficient for (2n+1)pi-pulses.
Electron spin coherence is induced via light-hole transitions in a quantum well waveguide without either an external or internal DC magnetic field. In the absence of spin precession, the induced spin coherence is detected through effects of quantum interference in the spectral domain coherent nonlinear optical response. We interpret the experimental results qualitatively using a simple few-level model with only the optical transition selection rule as its basic ingredients.
The electron spin coherence in n-doped and undoped, self-assembled CdSe/Zn(S,Se) quantum dots has been studied by time-resolved pump-probe Kerr rotation. Long-lived spin coherence persisting up to 13 ns after spin orientation has been found in the n-doped quantum dots, outlasting significantly the lifetimes of charge neutral and negatively charged excitons of 350 - 530 ps. The electron spin dephasing time as long as 5.6 ns has been measured in a magnetic field of 0.25 T. Hyperfine interaction of resident electrons with a nuclear spin fluctuations is suggested as the main limiting factor for the dephasing time. The efficiency of this mechanism in II-VI and III-V quantum dots is analyzed.
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