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Register a new userOn the Microscopic Foundations of Elasticity
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The modeling of the elastic properties of disordered or nanoscale solids requires the foundations of the theory of elasticity to be revisited, as one explores scales at which this theory may no longer hold. The only cases for which microscopically based derivations of elasticity are documented are (nearly) uniformly strained lattices. A microscopic approach to elasticity is proposed. As a first step, microscopically exact expressions for the displacement, strain and stress fields are derived. Conditions under which linear elastic constitutive relations hold are studied theoretically and numerically. It turns out that standard continuum elasticity is not self-evident, and applies only above certain spatial scales, which depend on details of the considered system and boundary conditions. Possible relevance to granular materials is briefly discussed.
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Due to their unique structural and mechanical properties, randomly-crosslinked polymer networks play an important role in many different fields, ranging from cellular biology to industrial processes. In order to elucidate how these properties are controlled by the physical details of the network (textit{e.g.} chain-length and end-to-end distributions), we generate disordered phantom networks with different crosslinker concentrations $C$ and initial density $rho_{rm init}$ and evaluate their elastic properties. We find that the shear modulus computed at the same strand concentration for networks with the same $C$, which determines the number of chains and the chain-length distribution, depends strongly on the preparation protocol of the network, here controlled by $rho_{rm init}$. We rationalise this dependence by employing a generic stress-strain relation for polymer networks that does not rely on the specific form of the polymer end-to-end distance distribution. We find that the shear modulus of the networks is a non-monotonic function of the density of elastically-active strands, and that this behaviour has a purely entropic origin. Our results show that if short chains are abundant, as it is always the case for randomly-crosslinked polymer networks, the knowledge of the exact chain conformation distribution is essential for predicting correctly the elastic properties. Finally, we apply our theoretical approach to published experimental data, qualitatively confirming our interpretations.
In a recent series of papers [1--3], a statistical model that accounts for correlations between topological and geometrical properties of a two-dimensional shuffled foam has been proposed and compared with experimental and numerical data. Here, the various assumptions on which the model is based are exposed and justified: the equiprobability hypothesis of the foam configurations is argued. The range of correlations between bubbles is discussed, and the mean field approximation that is used in the model is detailed. The two self-consistency equations associated with this mean field description can be interpreted as the conservation laws of number of sides and bubble curvature, respectively. Finally, the use of a Grand-Canonical description, in which the foam constitutes a reservoir of sides and curvature, is justified.
Disordered biopolymer gels have striking mechanical properties including strong nonlinearities. In the case of athermal gels (such as collagen-I) the nonlinearity has long been associated with a crossover from a bending dominated to a stretching dominated regime of elasticity. The physics of this crossover is related to the existence of a central-force isostatic point and to the fact that for most gels the bending modulus is small. This crossover induces scaling behavior for the elastic moduli. In particular, for linear elasticity such a scaling law has been demonstrated [Broedersz et al. Nature Physics, 2011 7, 983]. In this work we generalize the scaling to the nonlinear regime with a two-parameter scaling law involving three critical exponents. We test the scaling law numerically for two disordered lattice models, and find a good scaling collapse for the shear modulus in both the linear and nonlinear regimes. We compute all the critical exponents for the two lattice models and discuss the applicability of our results to real systems.
We study the shape, elasticity and fluctuations of the recently predicted (cond-mat/9510172) and subsequently observed (in numerical simulations) (cond-mat/9705059) tubule phase of anisotropic membranes, as well as the phase transitions into and out of it. This novel phase lies between the previously predicted flat and crumpled phases, both in temperature and in its physical properties: it is crumpled in one direction, and extended in the other. Its shape and elastic properties are characterized by a radius of gyration exponent $ u$ and an anisotropy exponent $z$. We derive scaling laws for the radius of gyration $R_G(L_perp,L_y)$ (i.e. the average thickness) of the tubule about a spontaneously selected straight axis and for the tubule undulations $h_{rms}(L_perp,L_y)$ transverse to its average extension. For phantom (i.e. non-self-avoiding) membranes, we predict $ u=1/4$, $z=1/2$ and $eta_kappa=0$, exactly, in excellent agreement with simulations. For membranes embedded in the space of dimension $d<11$, self-avoidance greatly swells the tubule and suppresses its wild transverse undulations, changing its shape exponents $ u$ and $z$. We give detailed scaling results for the shape of the tubule of an arbitrary aspect ratio and compute a variety of correlation functions, as well as the anomalous elasticity of the tubules. Finally we present a scaling theory for the shape of the membrane and its specific heat near the continuous transitions into and out of the tubule phase and perform detailed renormalization group calculations for the crumpled-to-tubule transition for phantom membranes.
The holographic principle has proven successful in linking seemingly unrelated problems in physics; a famous example is the gauge-gravity duality. Recently, intriguing correspondences between the physics of soft matter and gravity are emerging, including strong similarities between the rheology of amorphous solids, effective field theories for elasticity and the physics of black holes. However, direct comparisons between theoretical predictions and experimental/simulation observations remain limited. Here, we study the effects of non-linear elasticity on the mechanical and thermodynamic properties of amorphous materials responding to shear, using effective field and gravitational theories. The predicted correlations among the non-linear elastic exponent, the yielding strain/stress and the entropy change due to shear are supported qualitatively by simulations of granular matter models. Our approach opens a path towards understanding complex mechanical responses of amorphous solids, such as mixed effects of shear softening and shear hardening, and offers the possibility to study the rheology of solid states and black holes in a unified framework.
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