Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userElasticity, Shape Fluctuations and Phase Transitions in the New Tubule Phase of Anisotropic Tethered Membranes
72
0
0.0
(
0
)
Authors
Leo Radzihovsky
Ask ChatGPT about the research
No Arabic abstract
We study the shape, elasticity and fluctuations of the recently predicted (cond-mat/9510172) and subsequently observed (in numerical simulations) (cond-mat/9705059) tubule phase of anisotropic membranes, as well as the phase transitions into and out of it. This novel phase lies between the previously predicted flat and crumpled phases, both in temperature and in its physical properties: it is crumpled in one direction, and extended in the other. Its shape and elastic properties are characterized by a radius of gyration exponent $ u$ and an anisotropy exponent $z$. We derive scaling laws for the radius of gyration $R_G(L_perp,L_y)$ (i.e. the average thickness) of the tubule about a spontaneously selected straight axis and for the tubule undulations $h_{rms}(L_perp,L_y)$ transverse to its average extension. For phantom (i.e. non-self-avoiding) membranes, we predict $ u=1/4$, $z=1/2$ and $eta_kappa=0$, exactly, in excellent agreement with simulations. For membranes embedded in the space of dimension $d<11$, self-avoidance greatly swells the tubule and suppresses its wild transverse undulations, changing its shape exponents $ u$ and $z$. We give detailed scaling results for the shape of the tubule of an arbitrary aspect ratio and compute a variety of correlation functions, as well as the anomalous elasticity of the tubules. Finally we present a scaling theory for the shape of the membrane and its specific heat near the continuous transitions into and out of the tubule phase and perform detailed renormalization group calculations for the crumpled-to-tubule transition for phantom membranes.
rate research
Read More
Motivated by a freely suspended graphene and polymerized membranes in soft and biological matter we present a detailed study of a tensionless elastic sheet in the presence of thermal fluctuations and quenched disorder. The manuscript is based on an extensive draft dating back to 1993, that was circulated privately. It presents the general theoretical framework and calculational details of numerous results, partial forms of which have been published in brief Letters (Le Doussal and Radzihovsky 1992). The experimental realization of atom-thin graphene sheets has driven a resurgence in this fascinating subject, making our dated predictions and their detailed derivations timely. To this end we analyze the statistical mechanics of a generalized D-dimensional elastic membrane embedded in d dimensions using a self-consistent screening approximation (SCSA), that has proved to be unprecedentedly accurate in this system, exact in three complementary limits: d --> infinity, D --> 4, and D=d. Focusing on the critical flat phase, for a homogeneous two-dimensional membrane embedded in three dimensions, we predict its universal length-scale dependent roughness, elastic moduli exponents, and a universal negative Poisson ratio of -1/3. We also extend these results to short- and long-range correlated random heterogeneity, predicting a variety of glassy wrinkled membrane states. Finally, we also predict and analyze a continuous crumpling transition in a phantom elastic sheet. We hope that this detailed presentation of the SCSA theory will be useful for further theoretical developments and corresponding experimental investigations on freely suspended graphene.
The holographic principle has proven successful in linking seemingly unrelated problems in physics; a famous example is the gauge-gravity duality. Recently, intriguing correspondences between the physics of soft matter and gravity are emerging, including strong similarities between the rheology of amorphous solids, effective field theories for elasticity and the physics of black holes. However, direct comparisons between theoretical predictions and experimental/simulation observations remain limited. Here, we study the effects of non-linear elasticity on the mechanical and thermodynamic properties of amorphous materials responding to shear, using effective field and gravitational theories. The predicted correlations among the non-linear elastic exponent, the yielding strain/stress and the entropy change due to shear are supported qualitatively by simulations of granular matter models. Our approach opens a path towards understanding complex mechanical responses of amorphous solids, such as mixed effects of shear softening and shear hardening, and offers the possibility to study the rheology of solid states and black holes in a unified framework.
We show that smectic liquid crystals confined in_anisotropic_ porous structures such as e.g.,_strained_ aerogel or aerosil exhibit two new glassy phases. The strain both ensures the stability of these phases and determines their nature. One type of strain induces an ``XY Bragg glass, while the other creates a novel, triaxially anisotropic ``m=1 Bragg glass. The latter exhibits anomalous elasticity, characterized by exponents that we calculate to high precision. We predict the phase diagram for the system, and numerous other experimental observables.
Disordered biopolymer gels have striking mechanical properties including strong nonlinearities. In the case of athermal gels (such as collagen-I) the nonlinearity has long been associated with a crossover from a bending dominated to a stretching dominated regime of elasticity. The physics of this crossover is related to the existence of a central-force isostatic point and to the fact that for most gels the bending modulus is small. This crossover induces scaling behavior for the elastic moduli. In particular, for linear elasticity such a scaling law has been demonstrated [Broedersz et al. Nature Physics, 2011 7, 983]. In this work we generalize the scaling to the nonlinear regime with a two-parameter scaling law involving three critical exponents. We test the scaling law numerically for two disordered lattice models, and find a good scaling collapse for the shear modulus in both the linear and nonlinear regimes. We compute all the critical exponents for the two lattice models and discuss the applicability of our results to real systems.
Due to their unique structural and mechanical properties, randomly-crosslinked polymer networks play an important role in many different fields, ranging from cellular biology to industrial processes. In order to elucidate how these properties are controlled by the physical details of the network (textit{e.g.} chain-length and end-to-end distributions), we generate disordered phantom networks with different crosslinker concentrations $C$ and initial density $rho_{rm init}$ and evaluate their elastic properties. We find that the shear modulus computed at the same strand concentration for networks with the same $C$, which determines the number of chains and the chain-length distribution, depends strongly on the preparation protocol of the network, here controlled by $rho_{rm init}$. We rationalise this dependence by employing a generic stress-strain relation for polymer networks that does not rely on the specific form of the polymer end-to-end distance distribution. We find that the shear modulus of the networks is a non-monotonic function of the density of elastically-active strands, and that this behaviour has a purely entropic origin. Our results show that if short chains are abundant, as it is always the case for randomly-crosslinked polymer networks, the knowledge of the exact chain conformation distribution is essential for predicting correctly the elastic properties. Finally, we apply our theoretical approach to published experimental data, qualitatively confirming our interpretations.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
