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Unconventional spin density wave in (TMTSF)2PF6 below T* ~ 4K

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 Added by Mario Basletic
 Publication date 2002
  fields Physics
and research's language is English




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The presence of subphases in spin-density wave (SDW) phase of (TMTSF)2PF6 below T* ~ 4K has been suggested by several experiments but the nature of the new phase is still controversial. We have investigated the temperature dependence of the angular dependence of the magnetoresistance in the SDW phase which shows different features for temperatures above and below T*. For T > 4K the magnetoresistance can be understood in terms of the Landau quantization of the quasiparticle spectrum in a magnetic field, where the imperfect nesting plays the crucial role. We propose that below T* ~ 4K the new unconventional SDW (USDW) appears modifying dramatically the quasiparticle spectrum. Unlike conventional SDW the order parameter of USDW depends on the quasiparticle momentum. The present model describes many features of the angular dependence of magnetoresistance reasonably well. Therefore, we may conclude that the subphase in (TMTSF)2PF6 below T* ~ 4K is described as SDW plus USDW.



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It is well documented that SDW in (TMTSF)2PF6 undergoes another phase transition at T*approx 4K, though the nature of the new low temperature phase is controversial. We have shown recently that the new phase is well described in terms of unconventional SDW (USDW) which modifies the quasiparticle spectrum dramatically. In this paper we show that the same model describes consistently the Hall resistivity observed in (TMTSF)2PF6.
Among many Bechgaard salts, TMTSF2NO3 exhibits very anomalous low temperature properties. Unlike conventional spin density wave (SDW), TMTSF2NO3 undergoes the SDW transition at $T_SDWapprox 9.5$ K and the low temperature quasiparticle excitations are gapless. Also, it is known that TMTSF2NO3 does not exhibit superconductivity even under pressure, while FISDW is found in TMTSF2NO3 only for P=8.5 kbar and B>20 T. Here we shall show that both the angle dependent magnetoresistance data and the nonlinear Hall resistance of TMTSF2NO3 at ambient pressure are interpreted satisfactory in terms of unconventional spin density wave (USDW). Based on these facts, we propose a new phase diagram for Bechgaards salts.
Magnetoresistance in the spin-density wave (SDW) state of (TMTSF)2PF6 is known to exhibit a rich variety of the angular dependencies when a magnetic field B is rotated in the b-c*, a-b and a-c* planes. In the presence of a magnetic field the quasiparticle spectrum in the SDW with imperfect nesting is quantized. In such a case the minimum quasiparticle energy depends both on the magnetic field strength |B| and the angle theta between the field and the crystal direction a, b or c*. This approach describes rather satisfactory the magnetoresistance above T*~4K.
144 - Ning Kang 2010
We report the first comprehensive investigation of the organic superconductor (TMTSF)2PF6 in the vicinity of the endpoint of the spin density wave - metal phase transition where phase coexistence occurs. At low temperature, the transition of metallic domains towards superconductivity is used to reveal the various textures. In particular, we demonstrate experimentally the existence of 1D and 2D metallic domains with a cross-over from a filamentary superconductivity mostly along the c?-axis to a 2D superconductivity in the b?c-plane perpendicular to the most conducting direction. The formation of these domain walls may be related to the proposal of a soliton phase in the vicinity of the critical pressure of the (TMTSF)2PF6 phase diagram.
We report unexpected features of the transport in the dielectric spin density wave (SDW) phase of the quasi one-dimensional compound (TMTSF)_2PF_6: the resistance exhibits a maximum and a subsequent strong drop as temperature decreases below approximately 2K. The maximum in R(T) is not caused by depinning or Joule heating of the SDW. The characteristic temperature of the R(T) maximum and the scaling behavior of the resistance at different magnetic fields B evidence that the non-monotonic R(T) dependence has an origin different from the one known for the quantum Hall effect region of the phase diagram. We also found that the borderline T_0(B,P) which divides the field induced SDW region of the P-B-T phase diagram into the hysteresis and non-hysteresis domains, terminates in the N=1 sub-phase; the borderline has thus no extension to the SDW N=0 phase.
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