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Register a new userInterfacial anisotropic exciton-polariton manifolds in ReS$_2$
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Added by
Devarshi Chakrabarty
Publication date
2021
fields
Physics
and research's language is
English
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Light-matter coupling in van der Waals materials holds significant promise in realizing Bosonic condensation and superfluidity. The underlying semiconductors crystal asymmetry, if any, can be utilized to form anisotropic half-light half-matter quasiparticles. We demonstrate generation of such highly anisotropic exciton-polaritons at the interface of a biaxial layered semiconductor, stacked on top of a distributed Bragg reflector. The spatially confined photonic mode in this geometry couples with polarized excitons and their Rydberg states, creating a system of highly anisotropic polariton manifolds, displaying vacuum Rabi splitting of upto 68 meV. Rotation of the incident beam polarization is used to tune coupling strength and smoothly switch regimes from weak to strong coupling, while also enabling transition from one three-body coupled oscillator system to another. Light-matter coupling is further tunable by varying the number of weakly coupled optically active layers. Our work provides a versatile method of engineering devices for applications in polarization-controlled polaritonics and optoelectronics.
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Compression dramatically changes the transport and localization properties of graphene. This is intimately related to the change of symmetry of the Dirac cone when the particle hopping is different along different directions of the lattice. In particular, for a critical compression, a semi-Dirac cone is formed with massless and massive dispersions along perpendicular directions. Here we show direct evidence of the highly anisotropic transport of polaritons in a honeycomb lattice of coupled micropillars implementing a semi-Dirac cone. If we optically induce a vacancy-like defect in the lattice, we observe an anisotropically localized polariton distribution in a single sublattice, a consequence of the semi-Dirac dispersion. Our work opens up new horizons for the study of transport and localization in lattices with chiral symmetry and exotic Dirac dispersions.
We have used angle resolved photoemission spectroscopy to investigate the band structure of ReS$_2$, a transition-metal dichalcogenide semiconductor with a distorted 1T crystal structure. We find a large number of narrow valence bands, which we attribute to the combined influence of the structural distortion and spin-orbit coupling. We further image how this leads to a strong in-plane anisotropy of the electronic structure, with quasi-one-dimensional bands reflecting predominant hopping along zig-zag Re chains. We find that this does not persist up to the top of the valence band, where a more three-dimensional character is recovered with the fundamental band gap located away from the Brillouin zone centre along $k_z$. These experiments are in good agreement with our density-functional theory calculations, shedding new light on the bulk electronic structure of ReS$_2$, and how it can be expected to evolve when thinned to a single layer.
Topological insulators (TIs) are a striking example of materials in which topological invariants are manifested in robustness against perturbations. Their most prominent feature is the emergence of topological edge states with reduced dimension at the boundary between areas with distinct topological invariants. The observable physical effect is unidirectional robust transport, unaffected by defects or disorder. TIs were originally observed in the integer quantum Hall effect for fermionic systems of correlated electrons. However, during the past decade the concepts of topological physics have been introduced into numerous fields beyond condensed matter, ranging from microwaves and photonic systems to cold atoms, acoustics and even mechanics. Recently, TIs were proposed in exciton-polariton systems organized as honeycomb lattices, under the influence of a magnetic field. Topological phenomena in polaritons are fundamentally different from all topological effects demonstrated experimentally thus far: exciton-polaritons are part-light part-matter quasiparticles emerging from the strong coupling of quantum well excitons and cavity photons. Here, we demonstrate experimentally the first exciton-polariton TI. This constitutes the first symbiotic light-matter TIs. Our polariton lattice is excited non-resonantly, and the chiral topological polariton edge mode is populated by a polariton condensation mechanism. We image real- and Fourier-space to measure photoluminescence, and demonstrate that the topological edge mode avoids defects, and that the propagation direction of the mode can be reversed by inverting the applied magnetic field. Our exciton-polariton TI paves the way for a variety of new topological phenomena, as they involve light-matter interaction, gain, and perhaps most importantly - exciton-polaritons interact with one another as a nonlinear many-body system.
Interactions of few-cycle terahertz pulses with the induced optical polarization in a quantum-well microcavity reveal that the lower and higher exciton-polariton modes together with the optically forbidden 2p-exciton state form a unique {Lambda}-type three-level system. Pronounced nonlinearities are observed via time-resolved strong-terahertz and weak-optical excitation spectroscopy and explained with a fully microscopic theory. The results show that the terahertz pulses strongly couple the exciton-polariton states to the 2p-exciton state while no resonant transition between the two polariton levels is observed.
We show theoretically that a lattice of exciton-polaritons can behave as a life-like cellular automaton when simultaneously excited by a continuous wave coherent field and a time-periodic sequence of non-resonant pulses. This provides a mechanism of realizing a range of highly sought spatiotemporal structures under the same conditions, including: discrete solitons, oscillating solitons, rotating solitons, breathers, soliton trains, guns, and choatic behaviour. These structures can survive in the system indefinitely, despite the presence of dissipation, and allow universal computation.
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