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Register a new userProton light yield of fast plastic scintillators for neutron imaging
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J. J. Manfredi
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Plastic organic scintillators have been tailored in composition to achieve ultra-fast temporal response, thereby enabling the design and development of fast neutron detection systems with high timing resolution. Eljen Technologys plastic organic scintillators -- EJ-230, EJ-232, and EJ-232Q -- are prospective candidates for use in emerging neutron imaging systems, where fast timing is paramount. To support the neutron response characterization of these materials, the relative proton light yields of EJ-230, EJ-232, and EJ-232Q were measured at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a broad-spectrum neutron source and a double time-of-flight technique, the proton light yield relations were obtained over a proton recoil energy range of approximately 300 keV to 4 MeV. The EJ-230, EJ-232, and EJ-232Q scintillators exhibited similar proton light yield relations to each other as well as to other plastic scintillators with the same polymer base material. A comparison of the relative proton light yield of different sized cylindrical EJ-232 and EJ-232Q scintillators also revealed consistent results. This work provides key input data for the realistic computational modeling of neutron detection technologies employing these materials, thereby supporting new capabilities in near-field radionuclide detection for national security applications.
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Compact neutron imagers using double-scatter kinematic reconstruction are being designed for localization and characterization of special nuclear material. These neutron imaging systems rely on scintillators with a rapid prompt temporal response as the detection medium. As n-p elastic scattering is the primary mechanism for light generation by fast neutron interactions in organic scintillators, proton light yield data are needed for accurate assessment of scintillator performance. The proton light yield of a series of commercial fast plastic organic scintillators---EJ-200, EJ-204, and EJ-208---was measured via a double time-of-flight technique at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a tunable deuteron breakup neutron source, target scintillators housed in a dual photomultiplier tube configuration, and an array of pulse-shape-discriminating observation scintillators, the fast plastic scintillator light yield was measured over a broad and continuous energy range down to proton recoil energies of approximately 50 keV. This work provides key input to event reconstruction algorithms required for utilization of these materials in emerging neutron imaging modalities.
Recent progress in the development of novel organic scintillators necessitates modern characterization capabilities. As the primary means of energy deposition by neutrons in these materials is n-p elastic scattering, knowledge of the proton light yield is paramount. This work establishes a new model-independent method to continuously measure proton light yield in organic scintillators over a broad energy range. Using a deuteron breakup neutron source at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory and an array of organic scintillators, the proton light yield of EJ-301 and EJ-309, commercially available organic liquid scintillators from Eljen Technology, were measured via a double time-of-flight technique. The light yield was determined using a kinematically over-constrained system in the proton energy range of 1-20 MeV. The effect of pulse integration length on the magnitude and shape of the proton light yield relation was also explored. This work enables accurate simulation of the performance of advanced neutron detectors and supports the development of next-generation neutron imaging systems.
A comparative study of the neutron-$gamma$ Pulse Shape Discrimination (PSD) with seven organic scintillators is performed using an identical setup and digital electronics. The scintillators include plastics (EJ-299-33 and a plastic prototype), single crystals (stilbene and the recent doped $p$-terphenyl) and liquids (BC501A, NE213 and the deuterated liquid BC537). First, the overall PSD performance of the different scintillators is compared and threshold neutron energies for a given discrimination quality are determined. Then, using statistical arguments, two intrinsic contributions to the PSD capability of the scintillating materials are disentangled: the light yield and the specific pulse shapes induced by neutrons and $gamma$-rays. This separation provides additional insight into the behaviour of organic scintillators and allows a detailed comparison of the discrimination performance of the various materials. On the basis of this analysis, limitations of current organic scintillators and of recently proposed alternative scintillators are discussed.
Two generations of a novel detector for high-resolution transmission imaging and spectrometry of fast-neutrons are presented. These devices are based on a hydrogenous fiber scintillator screen and single- or multiple-gated intensified camera systems (ICCD). This detector is designed for energy-selective neutron radiography with nanosecond-pulsed broad-energy (1 - 10 MeV) neutron beams. Utilizing the Time-of-Flight (TOF) method, such a detector is capable of simultaneously capturing several images, each at a different neutron energy (TOF). In addition, a gamma-ray image can also be simultaneously registered, allowing combined neutron/gamma inspection of objects. This permits combining the sensitivity of the fast-neutron resonance method to low-Z elements with that of gamma radiography to high-Z materials.
The fast neutrons produced by a calibrated 241Am-Be source were detected by two different Cs2LiYCl6:Ce (CLYC) scintillator detectors. The two cylindrical crystals (1x1 in size) were enriched with more than 99% of 7Li (C7LYC) and with about 95% of 6Li (C6LYC), respectively. Both crystals can detect fast neutrons whereas only C6LYC can also detect thermal neutrons, due to the presence of 6Li. The measurement was performed at the L.A.S.A. Laboratory of INFN and University of Milano (Italy). To identify the neutron events, the Pulse-Shape-Discrimination technique was used. A value for the detection efficiency of the 241Am-Be emitted neutrons, with energy up to 10 MeV, was deduced.
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