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Register a new userProton Light Yield in Organic Scintillators using a Double Time-of-Flight Technique
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J. A. Brown
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Recent progress in the development of novel organic scintillators necessitates modern characterization capabilities. As the primary means of energy deposition by neutrons in these materials is n-p elastic scattering, knowledge of the proton light yield is paramount. This work establishes a new model-independent method to continuously measure proton light yield in organic scintillators over a broad energy range. Using a deuteron breakup neutron source at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory and an array of organic scintillators, the proton light yield of EJ-301 and EJ-309, commercially available organic liquid scintillators from Eljen Technology, were measured via a double time-of-flight technique. The light yield was determined using a kinematically over-constrained system in the proton energy range of 1-20 MeV. The effect of pulse integration length on the magnitude and shape of the proton light yield relation was also explored. This work enables accurate simulation of the performance of advanced neutron detectors and supports the development of next-generation neutron imaging systems.
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Plastic organic scintillators have been tailored in composition to achieve ultra-fast temporal response, thereby enabling the design and development of fast neutron detection systems with high timing resolution. Eljen Technologys plastic organic scintillators -- EJ-230, EJ-232, and EJ-232Q -- are prospective candidates for use in emerging neutron imaging systems, where fast timing is paramount. To support the neutron response characterization of these materials, the relative proton light yields of EJ-230, EJ-232, and EJ-232Q were measured at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a broad-spectrum neutron source and a double time-of-flight technique, the proton light yield relations were obtained over a proton recoil energy range of approximately 300 keV to 4 MeV. The EJ-230, EJ-232, and EJ-232Q scintillators exhibited similar proton light yield relations to each other as well as to other plastic scintillators with the same polymer base material. A comparison of the relative proton light yield of different sized cylindrical EJ-232 and EJ-232Q scintillators also revealed consistent results. This work provides key input data for the realistic computational modeling of neutron detection technologies employing these materials, thereby supporting new capabilities in near-field radionuclide detection for national security applications.
A comparative study of the neutron-$gamma$ Pulse Shape Discrimination (PSD) with seven organic scintillators is performed using an identical setup and digital electronics. The scintillators include plastics (EJ-299-33 and a plastic prototype), single crystals (stilbene and the recent doped $p$-terphenyl) and liquids (BC501A, NE213 and the deuterated liquid BC537). First, the overall PSD performance of the different scintillators is compared and threshold neutron energies for a given discrimination quality are determined. Then, using statistical arguments, two intrinsic contributions to the PSD capability of the scintillating materials are disentangled: the light yield and the specific pulse shapes induced by neutrons and $gamma$-rays. This separation provides additional insight into the behaviour of organic scintillators and allows a detailed comparison of the discrimination performance of the various materials. On the basis of this analysis, limitations of current organic scintillators and of recently proposed alternative scintillators are discussed.
A new double time-of-flight (dTOF) neutron spectroscopy technique has been developed for pulsed broad spectrum sources with a duty cycle that results in frame overlap, where fast neutrons from a given pulse overtake slower neutrons from previous pulses. Using a tunable beam at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory, neutrons were produced via thick-target breakup of 16 MeV deuterons on a beryllium target in the cyclotron vault. The breakup spectral shape was deduced from a dTOF measurement using an array of EJ-309 organic liquid scintillators. Simulation of the neutron detection efficiency of the scintillator array was performed using both GEANT4 and MCNP6. The efficiency-corrected spectral shape was normalized using a foil activation technique to obtain the energy-dependent flux of the neutron beam at zero degrees with respect to the incoming deuteron beam. The dTOF neutron spectrum was compared to spectra obtained using HEPROW and GRAVEL pulse height spectrum unfolding techniques. While the unfolding and dTOF results exhibit some discrepancies in shape, the integrated flux values agree within two standard deviations. This method obviates neutron time-of-flight spectroscopy challenges posed by pulsed beams with frame overlap and opens new opportunities for pulsed white neutron source facilities.
Compact neutron imagers using double-scatter kinematic reconstruction are being designed for localization and characterization of special nuclear material. These neutron imaging systems rely on scintillators with a rapid prompt temporal response as the detection medium. As n-p elastic scattering is the primary mechanism for light generation by fast neutron interactions in organic scintillators, proton light yield data are needed for accurate assessment of scintillator performance. The proton light yield of a series of commercial fast plastic organic scintillators---EJ-200, EJ-204, and EJ-208---was measured via a double time-of-flight technique at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a tunable deuteron breakup neutron source, target scintillators housed in a dual photomultiplier tube configuration, and an array of pulse-shape-discriminating observation scintillators, the fast plastic scintillator light yield was measured over a broad and continuous energy range down to proton recoil energies of approximately 50 keV. This work provides key input to event reconstruction algorithms required for utilization of these materials in emerging neutron imaging modalities.
A simple model for the estimation of the light yield of a scintillation detector is developed under general assumptions and relying exclusively on the knowledge of its optical properties. The model allows to easily incorporate effects related to Rayleigh scattering and absorption of the photons.The predictions of the model are benchmarked with the outcomes of Monte Carlo simulations of specific scintillation detectors. An accuracy at the level of few percent is achieved. The case of a real liquid argon based detector is explicitly treated and the predicted light yield is compared with the measured value.
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