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Register a new userReal-time observation of charge-spin cooperative dynamics driven by a nonequilibrium phonon environment
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Quantum dots are recognized as a suitable platform for studying thermodynamic phenomena involving single electronic charges and spins in nano-scale devices. However, such a thermodynamic system is usually driven by electron reservoirs at different temperatures, not by a lattice temperature gradient. We report on experimental observations of charge-spin cooperative dynamics in transitions of two-electron spin states in a GaAs double quantum dot located in a non-equilibrium phonon environment. Enhancements in the spin-flip processes are observed, originating from phonon excitation combined with the spin-orbit interaction. In addition, due to the spatial gradient of phonon density between the dots, the spin-flip rate during an inter-dot electron tunnel from a hot to a cold dot is more enhanced than in the other direction, resulting in accumulation of parallel spin states in the double dot.
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The spreading of a bilayer gold film propagating outward from gold clusters, which are pinned to clean Si(111), is imaged in real time by low energy electron microscopy. By monitoring the evolution of the boundary of the gold film at fixed temperature, a linear dependence of the spreading radius on time is found. The measured spreading velocities in the temperature range of 800 < T < 930 K varied from below 100 pm/s to 50 nm/s. We show that the spreading rate is limited by the reaction to form Au silicide, and the spreading velocity is likely regulated by the reconstruction of the gold silicide that occurs at the interface.
Magnetic skyrmion is a promising building block for developing information storage and computing devices. It can be stabilized in a ferromagnetic thin film with the Dzyaloshinskii-Moriya interaction (DMI). The moving ferromagnetic skyrmion may show the skyrmion Hall effect, that is, the skyrmion shows a transverse shift when it is driven by a spin current. Here, we numerically and theoretically study the current-driven dynamics of a ferromagnetic nanoscale skyrmion in the presence of the anisotropic DMI, where the skyrmion has an elliptical shape. The skyrmion Hall effect of the elliptical skyrmion is investigated. It is found that the skyrmion Hall angle can be controlled by tuning the profile of elliptical skyrmion. Our results reveal the relation between the skyrmion shape and the skyrmion Hall effect, which could be useful for building skyrmion-based spintronic devices with preferred skyrmion Hall angle. Also, our results provide a method for the minimization of skyrmion Hall angle for applications based on in-line motion of skyrmions.
We propose an electrically driven spin injector into normal metals and semiconductors, which is based on a magnetic tunnel junction (MTJ) subjected to a microwave voltage. Efficient functioning of such an injector is provided by electrically induced magnetization precession in the free layer of MTJ, which generates the spin pumping into a metallic or semiconducting overlayer. We theoretically describe the spin and charge dynamics in the CoFeB/MgO/CoFeB/Au(GaAs) heterostructures. First, the magnedynamics in the free CoFeB layer is quantified with the account of a spin-transfer torque and a voltage-controlled magnetic anisotropy. By numerically solving the magnetodynamics equation, we determine dependences of the precession amplitude on the frequency $f$ and magnitude $V_mathrm{max}$ of the ac voltage applied to the MTJ. It is found that the frequency dependence changes drastically above the threshold amplitude $V_mathrm{max} approx 200$mV, exhibiting a break at the resonance frequency $f_mathrm{res}$ due to nonlinear effects. The results obtained for the magnetization dynamics are used to describe the spin injection and pumping into the Au and GaAs overlayers. Since the generated spin current creates additional charge current owing to the inverse spin Hall effect, we also calculate distribution of the electric potential in the thick Au overlayer. The calculations show that the arising transverse voltage becomes experimentally measurable at $f = f_mathrm{res}$. Finally, we evaluate the spin accumulation in a long n$^+$-GaAs bar coupled to the MTJ and determine its temporal variation and spatial distribution along the bar. It is found that the spin accumulation under resonant excitation is large enough for experimental detection even at micrometer distances from the MTJ. This result demonstrates high efficiency of the described nanoscale spin injector.
The generation and manipulation of carrier spin polarization in semiconductors solely by electric fields has garnered significant attention as both an interesting manifestation of spin-orbit physics as well as a valuable capability for potential spintronics devices. One realization of these spin-orbit phenomena, the spin Hall effect (SHE), has been studied as a means of all-electrical spin current generation and spin separation in both semiconductor and metallic systems. Previous measurements of the spin Hall effect have focused on steady-state generation and time-averaged detection, without directly addressing the accumulation dynamics on the timescale of the spin coherence time. Here, we demonstrate time-resolved measurement of the dynamics of spin accumulation generated by the extrinsic spin Hall effect in a doped GaAs semiconductor channel. Using electrically-pumped time-resolved Kerr rotation, we image the accumulation, precession, and decay dynamics near the channel boundary with spatial and temporal resolution and identify multiple evolution time constants. We model these processes using time-dependent diffusion analysis utilizing both exact and numerical solution techniques and find that the underlying physical spin coherence time differs from the dynamical rates of spin accumulation and decay observed near the sample edges.
Interfaces impede heat flow in micro/nanostructured systems. Conventional theories for interfacial thermal transport were derived based on bulk phonon properties of the materials making up the interface without explicitly considering the atomistic interfacial details, which are found critical to correctly describing thermal boundary conductance (TBC). Recent theoretical studies predicted the existence of localized phonon modes at the interface which can play an important role in understanding interfacial thermal transport. However, experimental validation is still lacking. Through a combination of Raman spectroscopy and high-energy resolution electron energy-loss spectroscopy (EELS) in a scanning transmission electron microscope, we report the first experimental observation of localized interfacial phonon modes at ~12 THz at a high-quality epitaxial Si-Ge interface. These modes are further confirmed using molecular dynamics simulations with a high-fidelity neural network interatomic potential, which also yield TBC agreeing well with that measured from time-domain thermoreflectance (TDTR) experiments. Simulations find that the interfacial phonon modes have obvious contribution to the total TBC. Our findings may significantly contribute to the understanding of interfacial thermal transport physics and have impact on engineering TBC at interfaces in applications such as electronics thermal management and thermoelectric energy conversion.
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