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High transmission in twisted bilayer graphene with angle disorder

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 Publication date 2021
  fields Physics
and research's language is English




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Angle disorder is an intrinsic feature of twisted bilayer graphene and other moire materials. Here, we discuss electron transport in twisted bilayer graphene in the presence of angle disorder. We compute the local density of states and the Landauer-Buttiker transmission through an angle disorder barrier of width comparable to the moire period, using a decimation technique based on a real space description. We find that barriers which separate regions where the width of the bands differ by 50% or more lead to a minor suppression of the transmission, and that the transmission is close to one for normal incidence, which is reminiscent of Klein tunneling. These results suggest that transport in twisted bilayer graphene is weakly affected by twist angle disorder.

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Close to a magical angle, twisted bilayer graphene (TBLG) systems exhibit isolated flat electronic bands and, accordingly, strong electron localization. TBLGs have hence been ideal platforms to explore superconductivity, correlated insulating states, magnetism, and quantized anomalous Hall states in reduced dimension. Below a threshold twist angle ($sim$ $1.1^circ$), the TBLG superlattice undergoes lattice reconstruction, leading to a periodic moire structure which presents a marked atomic corrugation. Using a tight-binding framework, this research demonstrates that superlattice reconstruction affects significantly the electronic structure of small-angle TBLGs. The first magic angle at $sim$ $1.1^circ$ is found to be a critical case presenting globally maximized electron localization, thus separating reconstructed TBLGs into two classes with clearly distinct electronic properties. While low-energy Dirac fermions are still preserved at large twist angles $> 1.1 ^circ$, small-angle ($lesssim 1.1^circ$) TBLG systems present common features such as large spatial variation and strong electron localization observed in unfavorable AA stacking regions. However, for small twist angles below $1.1 ^circ$, the relative contribution of the local AA regions is progressively reduced, thus precluding the emergence of further magic angles, in very good agreement with existing experimental evidence.
We develop a theory for a qualitatively new type of disorder in condensed matter systems arising from local twist-angle fluctuations in two strongly coupled van der Waals monolayers twisted with respect to each other to create a flat band moire superlattice. The new paradigm of twist angle disorder arises from the currently ongoing intense research activity in the physics of twisted bilayer graphene. In experimental samples of pristine twisted bilayer graphene, which are nominally free of impurities and defects, the main source of disorder is believed to arise from the unavoidable and uncontrollable non-uniformity of the twist angle across the sample. To address this new physics of twist-angle disorder, we develop a real-space, microscopic model of twisted bilayer graphene where the angle enters as a free parameter. In particular, we focus on the size of single-particle energy gaps separating the miniband from the rest of the spectrum, the Van Hove peaks, the renormalized Dirac cone velocity near charge neutrality, and the minibandwidth. We find that the energy gaps and minibandwidth are strongly affected by disorder while the renormalized velocity remains virtually unchanged. We discuss the implications of our results for the ongoing experiments on twisted bilayer graphene. Our theory is readily generalized to future studies of twist angle disorder effects on all electronic properties of moire superlattices created by twisting two coupled van der Waals materials with respect to each other.
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