No Arabic abstract
Background: The $K^pi=2^-$ excited band emerges systematically in $N=150$ isotones raging from Pu to No with even-$Z$ numbers, and a sharp drop in energies was observed in Cf. Purpose: I attempt to uncover the microscopic mechanism for the appearance of such a low-energy $2^-$ state in $^{248}$Cf. Furthermore, I investigate the possible occurrence of the low-energy $K^pi=2^+$ state to elucidate the mechanism that prefers the simultaneous breaking of the reflection and axial symmetry to the breaking of the axial symmetry alone in this mass region. Method: I employ a nuclear EDF method: the Skyrme-Kohn-Sham-Bogoliubov and the quasiparticle random-phase approximation are used to describe the ground state and the transition to excited states. Results: The Skyrme-type SkM* and SLy4 functionals reproduce the fall in energy, but not the absolute value, of the $K^pi=2^-$ state at $Z=98$, where the proton 2qp excitation $[633]7/2 otimes [521]3/2$ plays a decisive role for the peculiar isotonic dependence. I find interweaving roles by the pairing correlation of protons and the deformed shell closure at $Z=98$. The SkM* model predicts the $K^pi=2^-$ state appears lower in energy in $^{246}$Cf than in $^{248}$Cf as the Fermi level of neutrons is located in between the $[622]5/2$ and $[734]9/2$ orbitals. Except for $^{250}$Fm in the SkM* calculation, the $K^pi=2^+$ state is predicted to appear higher in energy than the $K^pi=2^-$ state because the quasi-proton $[521]1/2$ orbital is located above the $[633]7/2$ orbital. Conclusions: A systematic study of low-lying collective states in heavy actinide nuclei provides a rigorous testing ground for microscopic nuclear models. The present study shows a need for improvements in the EDFs to describe pairing correlations and shell structures in heavy nuclei, that are indispensable in predicting the heaviest nuclei.
The structure of low-energy collective states in proton-deficient N=28 isotones is analyzed using structure models based on the relativistic energy density functional DD-PC1. The relativistic Hartree-Bogoliubov model for triaxial nuclei is used to calculate binding energy maps in the $beta$-$gamma$ plane. The evolution of neutron and proton single-particle levels with quadrupole deformation, and the occurrence of gaps around the Fermi surface, provide a simple microscopic interpretation of the onset of deformation and shape coexistence. Starting from self-consistent constrained energy surfaces calculated with the functional DD-PC1, a collective Hamiltonian for quadrupole vibrations and rotations is employed in the analysis of excitation spectra and transition rates of $^{46}$Ar, $^{44}$S, and $^{42}$Si. The results are compared to available data, and previous studies based either on the mean-field approach or large-scale shell-model calculations. The present study is particularly focused on $^{44}$S, for which data have recently been reported that indicate pronounced shape coexistence.
The structure of low-lying excitation states of even-even $N=40$ isotones is studied using a five-dimensional collective Hamiltonian with the collective parameters determined from the relativistic mean-field plus BCS method with the PC-PK1 functional in the particle-hole channel and a separable paring force in the particle-particle channel. The theoretical calculations can reproduce not only the systematics of the low-lying states along the isotonic chain but also the detailed structure of the spectroscopy in a single nucleus. We find a picture of spherical-oblate-prolate shape transition along the isotonic chain of $N=40$ by analyzing the potential energy surfaces. The coexistence of low-lying excited $0^+$ states has also been shown to be a common feature in neutron-deficient $N=40$ isotones.
We present a new analysis of the pairing vibrations around 56Ni, with emphasis on odd-odd nuclei. This analysis of the experimental excitation energies is based on the subtraction of average properties that include the full symmetry energy together with volume, surface and Coulomb terms. The results clearly indicate a collective behavior of the isovector pairing vibrations and do not support any appreciable collectivity in the isoscalar channel.
In addition to shape oscillations, low-energy excitation spectra of deformed nuclei are also influenced by pairing vibrations. The simultaneous description of these collective modes and their coupling has been a long-standing problem in nuclear structure theory. Here we address the problem in terms of self-consistent mean-field calculations of collective deformation energy surfaces, and the framework of the interacting boson approximation. In addition to quadrupole shape vibrations and rotations, the explicit coupling to pairing vibrations is taken into account by a boson-number non-conserving Hamiltonian, specified by a choice of a universal density functional and pairing interaction. An illustrative calculation for $^{128}$Xe and $^{130}$Xe shows the importance of dynamical pairing degrees of freedom, especially for structures built on low-energy $0^+$ excited states, in $gamma$-soft and triaxial nuclei.
The binding energies of even-even and odd-odd N=Z nuclei are compared. After correcting for the symmetry energy we find that the lowest T=1 state in odd-odd N=Z nuclei is as bound as the ground state in the neighboring even-even nucleus, thus providing evidence for isovector np pairing. However, T=0 states in odd-odd N=Z nuclei are several MeV less bound than the even-even ground states. We associate this difference with a pair gap and conclude that there is no evidence for an isoscalar pairing condensate in N=Z nuclei.