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Near-optimal intense and powerful terahertz source by optical rectification in lithium niobate crystal

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 Added by Francois Blanchard
 Publication date 2021
  fields Physics
and research's language is English




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Using an affordable ytterbium laser with sub-mJ of energy combined with a novel pulse compression technique, we demonstrate an extremely competitive state-of-the-art terahertz (THz) source with 53 mW of average power and 310 kV/cm at focus from the tilted-pulse front pumping scheme in lithium niobate at room temperature. Key points of this demonstration include the use of a pump pulse duration of 280 fs in combination with an echelon mirror. Our results present unmatched combined characteristics and are highly competitive with the existing THz sources pumped at the mJ range. This demonstration is a step towards the democratization of access to intense and powerful THz pulses.



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Strong amplification in integrated photonics is one of the most desired optical functionalities for computing, communications, sensing, and quantum information processing. Semiconductor gain and cubic nonlinearities, such as four-wave mixing and stimulated Raman and Brillouin scattering, have been among the most studied amplification mechanisms on chip. Alternatively, material platforms with strong quadratic nonlinearities promise numerous advantages with respect to gain and bandwidth, among which nanophotonic lithium niobate is one of the most promising candidates. Here, we combine quasi-phase matching with dispersion engineering in nanophotonic lithium niobate waveguides and achieve intense optical parametric amplification. We measure a broadband phase-sensitive amplification larger than 45 dB/cm in a 2.5-mm-long waveguide. We further confirm high gain operation in the degenerate and non-degenerate regimes by amplifying vacuum fluctuations to macroscopic levels in a 6-mm-long waveguide, with gains exceeding 100 dB/cm over 600 nm of bandwidth around 2 $mu$m. Our results unlock new possibilities for on-chip few-cycle nonlinear optics, mid-infrared photonics, and quantum photonics.
The angular dependence of terahertz (THz) emission from birefringent crystals can differ significantly from that of cubic crystals. Here we consider optical rectification in uniaxial birefringent materials, such as chalcopyrite crystals. The analysis is verified in (110)-cut ZnGeP_2 and compared to (zincblende) GaP. Although the crystals share the same nonzero second-order tensor elements, the birefringence in chalcopyrite crystals cause the pump pulse polarization to evolve as it propagates through the crystal, resulting in a drastically different angular dependence in chalcopyrite crystals. The analysis is extended to {012}- and {114}-cut chalcopyrite crystals and predicts more efficient conversion for the {114} crystal cut over the {012}- and {110}-cuts.
Optical nonlinear functions are crucial for various applications in integrated photonics, such as all-optical information processing, photonic neural networks and on-chip ultrafast light sources. Due to the weak nonlinearities in most integrated photonic platforms, realizing optical nonlinear functions typically requires large driving energies in the picojoules level or beyond, thus imposing a barrier for most applications. Here, we tackle this challenge and demonstrate an integrated nonlinear splitter device in lithium niobate nano-waveguides by simultaneous engineering of the dispersion and quasi-phase matching. We achieve non-resonant all-optical switching with ultra-low energies down to tens of femtojoules, a near instantaneous switching time of 18 fs, and a large extinction ratio of more than 5 dB. Our nonlinear splitter simultaneously realizes switch-on and -off operations and features a state-of-the-art switching energy-time product as low as $1.4 times10^{-27}$ J$cdot$s. We also show a path toward attojoule level all-optical switching by further optimizing the device geometry. Our results can enable on-chip ultrafast and energy-efficient all-optical information processing, computing systems, and light sources.
166 - Bofeng Gao , Mengxin Ren , Wei Wu 2018
Lithium niobate is a multi-functional material, which has been regarded as one of the most promising platform for the multi-purpose optical components and photonic circuits. Targeting at the miniature optical components and systems, lithium niobate microstructures with feature sizes of several to hundreds of micrometers have been demonstrated, such as waveguides, photonic crystals, micro-cavities, and modulators, et al. In this paper, we presented subwavelength nanograting metasurfaces fabricated in a crystalline lithium niobate film, which hold the possibilities towards further shrinking the footprint of the photonic devices with new optical functionalities. Due to the collective lattice interactions between isolated ridge resonances, distinct transmission spectral resonances were observed, which could be tunable by varying the structural parameters. Furthermore, our metasurfaces are capable to show high efficiency transmission structural colors as a result of structural resonances and intrinsic high transparency of lithium niobate in visible spectral range. Our results would pave the way for the new types of ultracompact photonic devices based on lithium niobate.
Materials with strong $chi^{(2)}$ optical nonlinearity, especially lithium niobate, play a critical role in building optical parametric oscillators (OPOs). However, chip-scale integration of low-loss $chi^{(2)}$ materials remains challenging and limits the threshold power of on-chip $chi^{(2)}$ OPO. Here we report the first on-chip lithium niobate optical parametric oscillator at the telecom wavelengths using a quasi-phase matched, high-quality microring resonator, whose threshold power ($sim$30 $mu$W) is 400 times lower than that in previous $chi^{(2)}$ integrated photonics platforms. An on-chip power conversion efficiency of 11% is obtained at a pump power of 93 $mu$W. The OPO wavelength tuning is achieved by varying the pump frequency and chip temperature. With the lowest power threshold among all on-chip OPOs demonstrated so far, as well as advantages including high conversion efficiency, flexibility in quasi-phase matching and device scalability, the thin-film lithium niobate OPO opens new opportunities for chip-based tunable classical and quantum light sources and provides an potential platform for realizing photonic neural networks.
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