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Register a new userRotation symmetry breaking in the normal state of a kagome superconductor KV3Sb5
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Recently discovered kagome superconductors AV3Sb5 (A=K, Rb, Cs) provide a fresh opportunity to realize and study correlation-driven electronic phenomena on a kagome lattice. The observation of a 2a0 by 2a0 charge density wave (CDW) in the normal state of all members of AV3Sb5 kagome family has generated an enormous amount of interest, in an effort to uncover the nature of this CDW state, and identify any hidden broken symmetries. We use spectroscopic-imaging scanning tunneling microscopy to reveal a pronounced intensity anisotropy between different 2a0 CDW directions in KV3Sb5. In particular, by examining the strength of ordering wave vectors as a function of energy in Fourier transforms of differential conductance maps, we find that one of the CDW directions is distinctly different compared to the other two. This observation points towards an intrinsic rotation symmetry broken electronic ground state, where the symmetry is reduced from C6 to C2. Furthermore, in contrast to previous reports, we find that the CDW phase is insensitive to magnetic field direction, regardless of the presence or absence of atomic defects. Our experiments, combined with earlier observations of a stripe 4a0 charge ordering in CsV3Sb5, establish correlation-driven rotation symmetry breaking as a unifying feature of AV3Sb5 kagome superconductors.
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Intertwining quantum order and nontrivial topology is at the frontier of condensed matter physics. A charge density wave (CDW) like order with orbital currents has been proposed as a powerful resource for achieving the quantum anomalous Hall effect in topological materials and for the hidden phase in cuprate high-temperature superconductors. However, the experimental realization of such an order is challenging. Here we use high-resolution scanning tunnelling microscopy (STM) to discover an unconventional charge order in a kagome material KV3Sb5, with both a topological band structure and a superconducting ground state. Through both topography and spectroscopic imaging, we observe a robust 2x2 superlattice. Spectroscopically, an energy gap opens at the Fermi level, across which the 2x2 charge modulation exhibits an intensity reversal in real-space, signaling charge ordering. At impurity-pinning free region, the strength of intrinsic charge modulations further exhibits chiral anisotropy with unusual magnetic field response. Theoretical analysis of our experiments suggests a tantalizing unconventional chiral CDW in the frustrated kagome lattice, which can not only lead to large anomalous Hall effect with orbital magnetism, but also be a precursor of unconventional superconductivity.
We have investigated the superconducting state of the non-centrosymmetric compound Re6Zr using magnetization, heat capacity, and muon-spin relaxation/rotation (muSR) measurements. Re6Zr has a superconducting transition temperature, Tc = 6.75 K. Transverse-field muSR experiments, used to probe the superfluid density, suggest an s-wave character for the superconducting gap. However, zero and longitudinal-field muSR data reveal the presence of spontaneous static magnetic fields below Tc indicating that time-reversal symmetry is broken in the superconducting state and an unconventional pairing mechanism. An analysis of the pairing symmetries identifies the ground states compatible with time-reversal symmetry breaking.
The single helical Fermi surface on the surface state of three-dimensional topological insulator Bi2Se3 is constrained by the time-reversal invariant bulk topology to possess a spin-singlet superconducting pairing symmetry. In fact, the Cu-doped, and pressure-tuned superconducting Bi2Se3 show no evidence of the time reversal symmetry breaking. We report on the detection of the time reversal symmetry (TRS) breaking in the topological superconductor Sr0.1Bi2Se3 , probed by zero-field (ZF) {mu}SR measurements. The TRS breaking provides strong evidence for the existence of spin-triplet pairing state. The temperature dependent super-fluid density deduced from transverse-field (TF) {mu}SR measurement yields nodeless superconductivity with low superconducting carrier density and penetration depth {lambda} = 1622(134) nm. From the microscopic theory of unconventional pairing, we find that such a fully gapped spin triplet pairing channel is promoted by the complex interplay between the structural hexagonal warping and higher order Dresselhaus spin-orbit coupling terms. Based on Ginzburg-Landau analysis, we delineate the mixing of singlet to triplet pairing symmetry as the chemical potential is tuned far above from the Dirac cone. Our observation of such spontaneous TRS breaking chiral superconductivity on a helical surface state, protected by the TRS invariant bulk topology, can open new avenues for interesting research and applications.
We argue that the topological charge density wave phase in the quasi-2D Kagome superconductor AV$_3$Sb$_5$ is a chiral flux phase. Considering the symmetry of the Kagome lattice, we show that the chiral flux phase has the lowest energy among those states which exhibit $2times2$ charge orders observed experimentally. This state breaks the time-reversal symmetry and displays anomalous Hall effect. The explicit pattern of the density of this state in real space is calculated. These results are supported by recent experiments and suggest that these materials are a new platform to investigate the interplay between topology, superconductivity and electron-electron correlations.
Recently discovered Z2 topological kagome metals AV3Sb5 (A = K, Rb, and Cs) exhibit charge density wave (CDW) phases and novel superconducting paring states, providing a versatile platform for studying the interplay between electron correlation and quantum orders. Here we directly visualize CDW-induced bands renormalization and energy gaps in RbV3Sb5 using angle-resolved photoemission spectroscopy, pointing to the key role of tuning van Hove singularities to the Fermi energy in mechanisms of ordering phases. Near the CDW transition temperature, the bands around the Brillouin zone (BZ) boundary are shifted to high-binding energy, forming an M-shape band with singularities near the Fermi energy. The Fermi surfaces are partially gapped and the electronic states on the residual ones should be possibly dedicated to the superconductivity. Our findings are significant in understanding CDW formation and its associated superconductivity.
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