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Register a new userObservation of Time-Reversal Symmetry Breaking in the Non-Centrosymmetric Superconductor Re6Zr
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We have investigated the superconducting state of the non-centrosymmetric compound Re6Zr using magnetization, heat capacity, and muon-spin relaxation/rotation (muSR) measurements. Re6Zr has a superconducting transition temperature, Tc = 6.75 K. Transverse-field muSR experiments, used to probe the superfluid density, suggest an s-wave character for the superconducting gap. However, zero and longitudinal-field muSR data reveal the presence of spontaneous static magnetic fields below Tc indicating that time-reversal symmetry is broken in the superconducting state and an unconventional pairing mechanism. An analysis of the pairing symmetries identifies the ground states compatible with time-reversal symmetry breaking.
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The single helical Fermi surface on the surface state of three-dimensional topological insulator Bi2Se3 is constrained by the time-reversal invariant bulk topology to possess a spin-singlet superconducting pairing symmetry. In fact, the Cu-doped, and pressure-tuned superconducting Bi2Se3 show no evidence of the time reversal symmetry breaking. We report on the detection of the time reversal symmetry (TRS) breaking in the topological superconductor Sr0.1Bi2Se3 , probed by zero-field (ZF) {mu}SR measurements. The TRS breaking provides strong evidence for the existence of spin-triplet pairing state. The temperature dependent super-fluid density deduced from transverse-field (TF) {mu}SR measurement yields nodeless superconductivity with low superconducting carrier density and penetration depth {lambda} = 1622(134) nm. From the microscopic theory of unconventional pairing, we find that such a fully gapped spin triplet pairing channel is promoted by the complex interplay between the structural hexagonal warping and higher order Dresselhaus spin-orbit coupling terms. Based on Ginzburg-Landau analysis, we delineate the mixing of singlet to triplet pairing symmetry as the chemical potential is tuned far above from the Dirac cone. Our observation of such spontaneous TRS breaking chiral superconductivity on a helical surface state, protected by the TRS invariant bulk topology, can open new avenues for interesting research and applications.
Fascinating phenomena have been known to arise from the Dirac theory of relativistic quantum mechanics, which describes high energy particles having linear dispersion relations. Electrons in solids usually have non-relativistic dispersion relations but their quantum excitations can mimic relativistic effects. In topological insulators, electrons have both a linear dispersion relation, the Dirac behavior, on the surface and a non-relativistic energy dispersion in the bulk. Topological phases of matter have attracted much interest, particularly broken-symmetry phases in topological insulator materials. Here, we report by Nb doping that the topological insulator Bi2Se3 can be turned into a bulk type-II superconductor while the Dirac surface dispersion in the normal state is preserved. A macroscopic magnetic ordering appears below the superconducting critical temperature of 3.2 K indicating a spontaneous spin rotation symmetry breaking of the Nb magnetic moments. Even though such a magnetic order may appear at the edge of the superconductor, it is mediated by superconductivity and presents a novel phase of matter which gives rise to a zero-field Hall effect.
In the recent search for unconventional- and topological superconductivity, noncentrosymmetric superconductors (NCSCs) rank among the most promising candidate materials. Surprisingly, some of them -- especially those containing rhenium -- seem to exhibit also time-reversal symmetry (TRS) breaking in their superconducting state, while TRS is preserved in many other isostructural NCSCs. To date, a satisfactory explanation for such discrepant behavior, albeit crucial for understanding the unconventional superconductivity of these materials, is still missing. Here we review the most recent developments regarding the Re-based class, where the muon-spin relaxation ($mu$SR) technique plays a key role due to its high sensitivity to the weak internal fields associated with the TRS breaking phenomenon. We discuss different cases of Re-containing superconductors, comprising both centrosymmetric- and noncentrosymmetric crystal structures and ranging from pure rhenium, to Re$T$ ($T$ = 3$d$-5$d$ early transition metals), to the dilute-Re case of ReBe$_{22}$. $mu$SR results suggest that the rhenium presence and its amount are two key factors for the appearance and the extent of TRS breaking in Re-based superconductors. Besides summarizing the existing findings, we also put forward future research ideas regarding the exciting field of materials showing TRS breaking.
We report point contact Andreev Reflection (PCAR) measurements on a high-quality single crystal of the non-centrosymmetric superconductor Re6Zr. We observe that the PCAR spectra can be fitted by taking two isotropic superconducting gaps with Delta_1 ~ 0.79 meV and Delta_2 ~ 0.22 meV respectively, suggesting that there are at least two bands which contribute to superconductivity. Combined with the observation of time reversal symmetry breaking at the superconducting transition from muon spin relaxation measurements (Phys. Rev. Lett. 112, 107002 (2014)), our results imply an unconventional superconducting order in this compound: A multiband singlet state that breaks time reversal symmetry or a triplet state dominated by interband pairing.
We report a comprehensive study of the noncentrosymmetric superconductor Mo$_3$P. Its bulk superconductivity, with $T_c = 5.5$ K, was characterized via electrical resistivity, magnetization, and heat-capacity measurements, while its microscopic electronic properties were investigated by means of muon-spin rotation/relaxation ($mu$SR) and nuclear magnetic resonance (NMR) techniques. In the normal state, NMR relaxation data indicate an almost ideal metallic behavior, confirmed by band-structure calculations, which suggest a relatively high electron density of states, dominated by the Mo $4d$-orbitals. The low-temperature superfluid density, determined via transverse-field $mu$SR and electronic specific heat, suggest a fully-gapped superconducting state in Mo$_3$P, with $Delta_0= 0.83$ meV, the same as the BCS gap value in the weak-coupling case, and a zero-temperature magnetic penetration depth $lambda_0 = 126$ nm. The absence of spontaneous magnetic fields below the onset of superconductivity, as determined from zero-field $mu$SR measurements, indicates a preserved time-reversal symmetry in the superconducting state of Mo$_3$P and, hence, spin-singlet pairing.
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