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Register a new userSuperior ultra-transparent broadband terahertz polarizers by nanoimprint lithography
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Added by
Tatiana G. Rappoport
Publication date
2021
fields
Physics
and research's language is
English
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We report the largest broadband terahertz (THz) polarizer based on a flexible ultra-transparent cyclic olefin copolymer (COC). The COC polarizers were fabricated by nanoimprint soft lithography with the lowest reported pitch of 2 or 3 micrometers and depth of 3 micrometers and sub-wavelength Au bilayer wire grid. Fourier Transform Infrared spectroscopy in a large range of 0.9 -20 THz shows transmittance of bulk materials such as doped and undoped Si and polymers. COC polarizers present more than doubled transmission intensity and larger transmitting band when compared to Si. COC polarizers present superior performance when compared to Si polarizers, with extinctions ratios of at least 4.4 dB higher and registered performance supported by numerical simulations. Fabricated Si and COC polarizers show larger operation gap when compared to a commercial polarizer. Fabrication of these polarizers can be easily up-scaled which certainly meets functional requirements for many THz devices and applications, such as high transparency, lower cost fabrication and flexible material.
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Two types of optical metamaterials operating at near-IR and mid-IR frequencies, respectively, have been designed, fabricated by nanoimprint lithography (NIL), and characterized by laser spectroscopic ellipsometry. The structure for the near-IR range was a metal/dielectric/metal stack fishnet structure that demonstrated negative permittivity and permeability in the same frequency region and hence exhibited a negative refractive index at a wavelength near 1.7 um. In the mid-IR range, the metamaterial was an ordered array of four-fold symmetric L-shaped resonators (LSRs) that showed both a dipole plasmon resonance resulting in negative permittivity and a magnetic resonance with negative permeability near wavelengths of 3.7 um and 5.25 um, respectively. The optical properties of both metamaterials are in agreement with theoretical predictions. This work demonstrates the feasibility of designing various optical negative-index metamaterials and fabricating them using the nanoimprint lithography as a low-cost, high-throughput fabrication approach.
The Brewsters law predicts zero reflection of p-polarization on a dielectric surface at a particular angle. However, when loss is introduced into the permittivity of the dielectric, the Brewster condition breaks down and reflection unavoidably appears. In this work, we found an exception to this long-standing dilemma by creating a class of nonmagnetic anisotropic metamaterials, where an anomalous Brewster effects with independently tunable absorption and refraction emerges. This loss-independent Brewster effect is bestowed by the extra degrees of freedoms introduced by anisotropy and strictly protected by the reciprocity principle. The bandwidth can cover an extremely wide spectrum from dc to optical frequencies. Two examples of reflectionless Brewster absorbers with different Brewster angles are both demonstrated to achieve large absorbance in a wide spectrum via microwave experiments. Our work extends the scope of Brewster effect to the horizon of nonmagnetic absorptive materials, which promises an unprecedented wide bandwidth for reflectionless absorption with high efficiency.
A microwave ultra-broadband polarization-independent metamaterial absorber is demonstrated. It is composed of a periodic array of metal-dielectric multilayered quadrangular frustum pyramids. These pyramids possess resonant absorption modes at multi-frequencies, of which the overlapping leads to the total absorption of the incident wave over an ultra-wide spectral band. The experimental absorption at normal incidence is above 90% in the frequency range of 7.8-14.7GHz, and the absorption is kept large when the incident angle is smaller than 60 degrees. The experimental results agree well with the numerical simulation.
We present an ultra broadband thin-film infrared absorber made of saw-toothed anisotropic metamaterial. Absorbtivity of higher than 95% at normal incidence is supported in a wide range of frequencies, where the full absorption width at half maximum is about 86%. Such property is retained well at a very wide range of incident angles too. Light of shorter wavelengths are harvested at upper parts of the sawteeth of smaller widths, while light of longer wavelengths are trapped at lower parts of larger tooth widths. This phenomenon is explained by the slowlight modes in anisotropic metamaterial waveguide. Our study can be applied in the field of designing photovoltaic devices and thermal emitters.
Magnetoplasmonics is highly promising to devise active optical elements: modulating the plasmon resonance condition with magnetic field can boost the performance of refractometric sensors and nanophotonic optical devices. Nevertheless, real life applications are hampered by the magnetoplasmonic trilemma: 1) a good plasmonic metal has sharp optical resonances but low magneto-optical response; 2) a magnetic metal has strong magneto-optical response but a very broad plasmonic resonance; 3) mixing the two components degrades the quality of both features. To overcome the trilemma, we use a different class of materials, transparent conductive oxide nanocrystals (NCs) with plasmonic response in the near infrared. Although non-magnetic, they combine a large cyclotron frequency (due to small electron effective mass) with sharp plasmonic resonances. We benchmark the concept with F- and In- doped CdO (FICO) and Sn-doped In2O3 (ITO) NCs to boost the magneto-optical Faraday rotation and ellipticity, reaching the highest magneto-optical response for a non-magnetic plasmonic material, and exceeding the performance of state-of-the-art ferromagnetic nanostructures. The magnetoplasmonic response of these NCs was rationalized with analytical model based on the excitation of circular magnetoplasmonic modes. Finally, proof of concept experiments demonstrated the superior performance of FICO NCs with respect to current state of the art in magnetoplasmonic refractometric sensing, approaching the sensitivity of leading localized plasmon refractometric methods with the advantage of not requiring complex curve fitting.
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