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The largest moon of Neptune, Triton, possess a cold and hazy atmosphere. Since the discovery of near-surface haze layer during the Voyager fly in 1989, the haze formation mechanism has not been investigated in detail. Here, we provide the first haze microphysical model on Triton. Our model solves the evolution of both size and porosity distributions of haze particles in a self-consistent manner. We simulated the formation of sphere and aggregate hazes with and without condensation of the C$_2$H$_4$ ice. The haze particles can grow into fractal aggregates with mass-equivalent sphere sizes of $sim0.1$--$1~{rm {mu}m}$ and fractal dimension of $D_{rm f} = 1.8$--$2.2$. The ice-free hazes cannot simultaneously explain both UV and visible observations of Voyager 2, while including the condensation of C$_2$H$_4$ ices provides two better solutions. For ice aggregates, the required total haze mass flux is $sim2times{10}^{-15}~{rm g~{cm}^{-2}~s^{-1}}$. For the icy sphere scenario, the column integrated C$_2$H$_4$ production rate is $sim8times{10}^{-15}~{rm g~{cm}^{-2}~s^{-1}}$, and the ice-free mass flux of $sim6times{10}^{-17}~{rm g~{cm}^{-2}~s^{-1}}$. The UV occultation observations at short wavelength $<0.15~{rm {mu}m}$ may slightly favor the icy aggregates. Observations of the haze optical depth and the degree of forward scattering in UV and visible should be able to distinguish whether Tritons hazes are icy spheres or ice aggregates in future Triton missions.
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New observing capabilities coming online over the next few years will provide opportunities for characterization of exoplanet atmospheres. However, clouds/hazes could be present in the atmospheres of many exoplanets, muting the amplitude of spectral features. We use laboratory simulations to explore photochemical haze formation in H2-rich exoplanet atmospheres at 800 K with metallicity either 100 and 1000 times solar. We find that haze particles are produced in both simulated atmospheres with small particle size (20 to 140 nm) and relative low production rate (2.4 x 10-5 to 9.7 x 10-5 mg cm-3 h-1), but the particle size and production rate is dependent on the initial gas mixtures and the energy sources used in the simulation experiments. The gas phase mass spectra show that complex chemical processes happen in these atmospheres and generate new gas products that can further react to form larger molecules and solid haze particles. Two H2-rich atmospheres with similar C/O ratios (~0.5) yield different haze particles size, haze production rate, and gas products, suggesting both the elemental abundances and their bonding environments in an atmosphere can significantly affect the photochemistry. There is no methane (CH4) in our initial gas mixtures, although CH4 is often believed to be required to generate organic hazes. However, haze production rates from our experiments with different initial gas mixtures indicate that CH4 is neither required to generate organic hazes nor necessary to promote the organic haze formation. The variety and relative yield of the gas products indicate that CO and N2 enrich chemical reactions in H2-rich atmospheres.
Sulfur gases significantly affect the photochemistry of planetary atmospheres in our Solar System, and are expected to be important components in exoplanet atmospheres. However, sulfur photochemistry in the context of exoplanets is poorly understood due to a lack of chemical-kinetics information for sulfur species under relevant conditions. Here, we study the photochemical role of hydrogen sulfide (H2S) in warm CO2-rich exoplanet atmospheres (800 K) by carrying out laboratory simulations. We find that H2S plays a significant role in photochemistry, even when present in the atmosphere at relatively low concentrations (1.6%). It participates in both gas and solid phase chemistry, leading to the formation of other sulfur gas products (CH3SH/SO, C2H4S/OCS, SO2/S2, and CS2) and to an increase in solid haze particle production and compositional complexity. Our study shows that we may expect thicker haze with small particle sizes (20 to 140 nm) for warm CO2-rich exoplanet atmospheres that possess H2S.
UV radiation can induce photochemical processes in exoplanet atmospheres and produce haze particles. Recent observations suggest that haze and/or cloud layers could be present in the upper atmospheres of exoplanets. Haze particles play an important role in planetary atmospheres and may provide a source of organic material to the surface which may impact the origin or evolution of life. However, very little information is known about photochemical processes in cool, high-metallicity exoplanetary atmospheres. Previously, we investigated haze formation and particle size distribution in laboratory atmosphere simulation experiments using AC plasma as the energy source. Here, we use UV photons to initiate the chemistry rather than the AC plasma, since photochemistry driven by UV radiation is important for understanding exoplanet atmospheres. We present photochemical haze formation in current UV experiments, we investigated a range of atmospheric metallicities (100x, 1000x, and 10000x solar metallicity) at three temperatures (300 K, 400 K, and 600 K). We find that photochemical hazes are generated in all simulated atmospheres with temperature-dependent production rates: the particles produced in each metallicity group decrease as the temperature increases. The images taken with atomic force microscopy show the particle size (15-190 nm) varies with temperature and metallicity. Our laboratory experimental results provide new insight into the formation and properties of photochemical haze, which could guide exoplanet atmosphere modeling and help to analyze and interpret current and future observations of exoplanets.
A diurnal varying haze layer at the bright spots of Occator on dwarf planet Ceres has been reported from images of the Dawn Framing Camera. This finding is supported by ground-based observations revealing diurnal albedo changes at Occators longitude. In the present work, we further investigate the previously reported haze phenomenon in more detail using additional Framing Camera images. We demonstrate that the light scattering behavior at the central floor of Occator is different compared to a typical cerean surface and is likely inconsistent with a pure solid surface scatterer. The identified deviation is best explained by an additional component to the scattered light of the surface, i.e., a haze layer. Our results support the water vapor detection by Herschel observations though the existence of a tenuous cerean exosphere is not yet confirmed.
Haze in Plutos atmosphere was detected in images by both the Long Range Reconnaissance Imager (LORRI) and the Multispectral Visible Imaging Camera (MVIC) on New Horizons. LORRI observed haze up to altitudes of at least 200 km above Plutos surface at solar phase angles from ~20{deg} to ~169{deg}. The haze is structured with about ~20 layers, and the extinction due to haze is greater in the northern hemisphere than at equatorial or southern latitudes. However, more haze layers are discerned at equatorial latitudes. A search for temporal variations found no evidence for motions of haze layers (temporal changes in layer altitudes) on time scales of 2 to 5 hours, but did find evidence of changes in haze scale height above 100 km altitude. An ultraviolet extinction attributable to the atmospheric haze was also detected by the ALICE ultraviolet spectrograph on New Horizons. The haze particles are strongly forward-scattering in the visible, and a microphysical model of haze is presented which reproduces the visible phase function just above the surface with 0.5 {mu}m spherical particles, but also invokes fractal aggregate particles to fit the visible phase function at 45 km altitude and account for UV extinction. A model of haze layer generation by orographic excitation of gravity waves is presented. This model accounts for the observed layer thickness and distribution with altitude. Haze particles settle out of the atmosphere and onto Plutos surface, at a rate sufficient to alter surface optical properties on seasonal time scales. Plutos regional scale albedo contrasts may be preserved in the face of the haze deposition by atmospheric collapse.
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