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Register a new userInhomogeneous Kondo destruction by RKKY correlations
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The competition between the indirect exchange interaction (IEC) of magnetic impurities in metals and the Kondo effect gives rise to a rich quantum phase diagram, the Doniach Diagram. In disordered metals, both the Kondo temperature and the IEC are widely distributed due to the scattering of the conduction electrons from the impurity potential. Therefore, it is a question of fundamental importance, how this Doniach diagram is modified by the disorder, and if one can still identify separate phases. Recently, it has been investigated the effect of Ruderman-Kittel-Kasuya-Yosida (RKKY) correlations on the Kondo effect of two magnetic impurities, renormalizing the Kondo interaction based on the Bethe-Salpeter equation and performing the poor mens renormalization group (RG) analysis with the RKKY-renormalized Kondo coupling. In the present study, we extend this theoretical framework, allowing for different Kondo temperatures of two RKKY-coupled magnetic impurities due to different local exchange couplings and density of states. As a result, we find that the smaller one of the two Kondo temperatures is suppressed more strongly by the RKKY interaction, thereby enhancing their initial inequality. In order to find out if this relevance of inequalities between Kondo temperatures modifies the distribution of the Kondo temperature in a system of a finite density of randomly distributed magnetic impurities, we present an extension of the RKKY coupled Kondo RG equations. We discuss the implication of these results for the interplay between Kondo coupling and RKKY interaction in disordered electron systems and the Doniach diagram in disordered electron systems.
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In a Kondo lattice, the spin exchange coupling between a local spin and the conduction electrons acquires nonlocal contributions due to conduction electron scattering from surrounding local spins and the subsequent RKKY interaction. It leads to a hitherto unrecognized interference of Kondo screening and the RKKY interaction beyond the Doniach scenario. We develop a renormalization group theory for the RKKY-modified Kondo vertex. The Kondo temperature, $T_K(y)$, is suppressed in a universal way, controlled by the antiferromagnetic RKKY coupling parameter $y$. Complete spin screening ceases to exist beyond a critical RKKY strength $y_c$ even in the absence of magnetic ordering. At this breakdown point, $T_K(y)$ remains nonzero and is not defined for larger RKKY couplings, $y>y_c$. The results are in quantitative agreement with STM spectroscopy experiments on tunable two-impurity Kondo systems. The possible implications for quantum critical scenarios in heavy-fermion systems are discussed.
We apply our recently developed, selfconsistent renormalization group (RG) method to STM spectra of a two-impurity Kondo system consisting of two cobalt atoms connected by a one-dimensional Cu chain on a Cu surface. This RG method was developed to describe local spin screening in multi-impurity Kondo systems in presence of the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction. Using the RKKY interaction of a one-dimensional chain, we explain the experimentally observed suppression and oscillation of the Kondo temperature, $T_K(y)$, as a function of the length of the chain and the corresponding RKKY interaction parameter $y$, regardless of the RKKY coupling being ferromagnetic or antiferromagnetic.
We show that the paradigmatic Ruderman-Kittel-Kasuya-Yosida (RKKY) description of two local magnetic moments coupled to propagating electrons breaks down in helical Luttinger Liquids when the electron interaction is stronger than some critical value. In this novel regime, the Kondo effect overwhelms the RKKY interaction over all macroscopic inter-impurity distances. This phenomenon is a direct consequence of the helicity (realized, for instance, at edges of a time-reversal invariant topological insulator) and does not take place in usual (non-helical) Luttinger Liquids.
We study the impurity entanglement entropy $S_e$ in quantum impurity models that feature a Kondo-destruction quantum critical point (QCP) arising from a pseudogap in the conduction-band density of states or from coupling to a bosonic bath. On the local-moment (Kondo-destroyed) side of the QCP, the entanglement entropy contains a critical component that can be related to the order parameter characterizing the quantum phase transition. In Kondo models describing a spin-$Simp$, $S_e$ assumes its maximal value of $ln(2Simp+1)$ at the QCP and throughout the Kondo phase, independent of features such as particle-hole symmetry and under- or over-screening. In Anderson models, $S_e$ is nonuniversal at the QCP, and at particle-hole symmetry, rises monotonically on passage from the local-moment phase to the Kondo phase; breaking this symmetry can lead to a cusp peak in $S_e$ due to a divergent charge susceptibility at the QCP. Implications of these results for quantum critical systems and quantum dots are discussed.
The cooperative behavior of quantum impurities on 2D materials, such as graphene and bilayer graphene, is characterized by a non-trivial competition between screening (Kondo effect), and Ruderman-Kittel-Kasuya-Yosida (RKKY) magnetism. In addition, due to the small density of states at the Fermi level, impurities may not couple to the conduction electrons at all, behaving as free moments. Employing a recently developed {em{exact}} numerical method to study multi-impurity lattice systems, we obtain non-perturbative results that dramatically depart from expectations based on the conventional RKKY theory. At half-filling and for weak coupling, impurities remain in the local moment regime when they are on opposite sublattices, up to a critical value of the interactions when they start coupling anti-ferromagnetically with correlations that decay very slowly with inter-impurity distance. At finite doping, away from half-filling, ferromagnetism is completely absent and the physics is dominated by a competition between anti-ferromagnetism and Kondo effect. In bilayer graphene, impurities on opposite layers behave as free moments, unless the interaction is of the order of the hopping or larger.
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