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Register a new userDevelopment of Low Radioactive Molecular Sieves for Ultra-Low Background Particle Physics Experiment
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This study develops low radioactive molecular sieves (MS) for ultra-low background particle physics experiment. The manufactured MS is of type 4A. $^{226}$Ra and $^{232}$Th have concentrations of about 57 and 198 mBq/kg, respectively, measured by applying high-purity germanium (HPGe) measurement. The reduction of the radioactivity from the commercial one is about 99 and 97 percent for $^{226}$Ra and $^{232}$Th, respectively. Furthermore, the radon emanation rate from MS filter is about 2.1 mBq, which is measured by utilizing pin-photo type radon detector. This developed MS is expected to remove the impurity from the noble gas, in which low radioactivity is needed such as dark matter search experiment.
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Type 5A molecular sieves (MS) have been demonstrated to remove radon from SF$_6$ gas. This is important for ultra-sensitive SF$_6$ gas-based directional dark matter and related rare-event physics experiments, as radon can provide a source of unwanted background events. Unfortunately, commercially available sieves intrinsically emanate radon at levels not suitable for ultra-sensitive physics experiments. A method to produce a low radioactive MS has been developed in Nihon University (NU). In this work, we explore the feasibility of the NU-developed 5A type MS for use in such experiments. A comparison with a commercially available Sigma-Aldrich 5A type MS was made. The comparison was done by calculating a parameter indicating the amount of radon intrinsically emanated by the MS per unit radon captured from SF$_6$ gas. The measurements were made using a specially adapted DURRIDGE RAD7 radon detector. The NU-developed 5A MS emanated radon up to 61$pm$9$%$ less per radon captured (2.1$pm$0.1)$times 10^{-3}$, compared to the commercial Sigma-Aldrich MS (5.4$pm$0.4)$times 10^{-3}$, making it a better candidate for use in a radon filtration setup for future ultra-sensitive SF$_6$ gas based experiments.
We successfully developed a new photomultiplier tube (PMT) with a three-inch diameter, convex-shaped photocathode, R13111. Its prominent features include good performance and ultra-low radioactivity. The convex-shaped photocathode realized a large photon acceptance and good timing resolution. Low radioactivity was achieved by three factors: (1) the glass material was synthesized using low-radioactive-contamination material; (2) the photocathode was produced with $^{39}$K-enriched potassium; and (3) the purest grade of aluminum material was used for the vacuum seal. As a result each R13111 PMT contains only about 0.4 mBq of $^{226}$Ra, less than 2 mBq of $^{238}$U, 0.3 mBq of $^{228}$Ra, 2 mBq of $^{40}$K and 0.2 mBq of $^{60}$Co. We also examined and resolved the intrinsic leakage of Xe gas into PMTs that was observed in several older models. We thus succeeded in developing a PMT that has low background, large angular acceptance with high collection efficiency, good timing resolution, and long-term stable operation. These features are highly desirable for experiments searching for rare events beyond the standard model, such as dark matter particle interactions and neutrinoless double beta decay events.
For experiments searching for rare signals, background events from the detector itself are one of the major limiting factors for search sensitivity. Screening for ultra-low radioactive detector material is becoming ever more essential. We propose to develop a gaseous Time Projection Chamber (TPC) with Micromegas readout for radio-screening purposes. The TPC records three-dimensional trajectories of charged particles emitted from a flat sample placed inside the active volume. The detector is able to distinguish the origin of an event and identify the particle types with information from trajectories, which improves the screening sensitivity significantly. For $alpha$ particles from the sample surface, we find that our proposed detector can reach a sensitivity of better than 100~$mu$Bq$cdot$m$^{-2}$ within two days.
Rare event search experiments, such as those searching for dark matter and observations of neutrinoless double beta decay, require ultra low levels of radioactive background for unmistakable identification. In order to reduce the radioactive backgrounds of detectors used in these types of event searches, low background photosensors are required, as the physical size of these detectors become increasing larger, and hence the number of such photosensors used also increases rapidly. Considering that most dark matter and neutrinoless double beta decay experiments are turning towards using noble liquids as the target choice, liquid xenon and liquid argon for instance, photosensors that can work well at cryogenic temperatures are required, 165 K and 87 K for liquid xenon and liquid argon, respectively. The Silicon Geiger Hybrid Tube (SiGHT) is a novel photosensor designed specifically for use in ultra low background experiments operating at cryogenic temperatures. It is based on the proven photocathode plus silicon photomultiplier (SiPM) hybrid technology and consists of very few other, but also ultra radio-pure, materials like fused silica and silicon for the SiPM. The introduction of the SiGHT concept, as well as a feasibility study for its production, is reported in this paper.
Results are presented from radioactivity screening of two models of photomultiplier tubes designed for use in current and future liquid xenon experiments. The Hamamatsu 5.6 cm diameter R8778 PMT, used in the LUX dark matter experiment, has yielded a positive detection of four common radioactive isotopes: 238U, 232Th, 40K, and 60Co. Screening of LUX materials has rendered backgrounds from other detector materials subdominant to the R8778 contribution. A prototype Hamamatsu 7.6 cm diameter R11410 MOD PMT has also been screened, with benchmark isotope counts measured at <0.4 238U / <0.3 232Th / <8.3 40K / 2.0+-0.2 60Co mBq/PMT. This represents a large reduction, equal to a change of times 1/24 238U / times 1/9 232Th / times 1/8 40K per PMT, between R8778 and R11410 MOD, concurrent with a doubling of the photocathode surface area (4.5 cm to 6.4 cm diameter). 60Co measurements are comparable between the PMTs, but can be significantly reduced in future R11410 MOD units through further material selection. Assuming PMT activity equal to the measured 90% upper limits, Monte Carlo estimates indicate that replacement of R8778 PMTs with R11410 MOD PMTs will change LUX PMT electron recoil background contributions by a factor of times1/25 after further material selection for 60Co reduction, and nuclear recoil backgrounds by a factor of times 1/36. The strong reduction in backgrounds below the measured R8778 levels makes the R11410 MOD a very competitive technology for use in large-scale liquid xenon detectors.
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