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Coherent X-rays with Tunable Time-Dependent Polarization

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 Added by Nicholas Sudar
 Publication date 2020
  fields Physics
and research's language is English




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We describe a method for producing high power, coherent x-ray pulses from a free electron laser with femtosecond scale periodic temporal modulation of the polarization vector. This approach relies on the generation of a temporal intensity modulation after self seeding either by modulating the seed intensity or the beam current. After generating a coherent temporally modulated $s$-polarization pulse, the electron beam is delayed by half a modulation period and sent into a short orthogonally oriented undulator, serving as a $p$-polarization afterburner. We provide simulations of three configurations for realizing this polarization switching, namely, enhanced self seeding with an intensity modulation generated by 2 color self seeding, enhanced self seeding of a current modulated bunch, and regular self seeding of a current modulated bunch. Start to end simulations for the Linac Coherent Light Source-II are provided for the latter.



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Tunable polarization over a wide spectral range is a required feature of light sources employed to investigate the properties of local symmetry in both condensed and low-density matter. Among new-generation sources, free-electron lasers possess a unique combination of very attractive features, as they allow to generate powerful and coherent ultra-short optical pulses in the VUV and X-ray spectral range. However, the question remains open about the possibility to freely vary the light polarization of a free-electron laser, when the latter is operated in the so-called nonlinear harmonic-generation regime. In such configuration, one collects the harmonics of the free-electron laser fundamental emission, gaining access to the shortest possible wavelengths the device can generate. In this letter we provide the first experimental characterization of the polarization of the harmonic light produced by a free-electron laser and we demonstrate a method to obtain tunable polarization in the VUV and X-ray spectral range. Experimental results are successfully compared to those obtained using a theoretical model based on the paraxial solution of Maxwells equations. Our findings can be expected to have a deep impact on the design and realization of experiments requiring full control of light polarization to explore the symmetry properties of matter samples.
Coherent population trapping (CPT) is extensively studied for future vapor cell clocks of high frequency stability. In the constructive polarization modulation CPT scheme, a bichromatic laser field with polarization and phase synchronously modulated is applied on an atomic medium. A high contrast CPT signal is observed in this so-called double-modulation configuration, due to the fact that the atomic population does not leak to the extreme Zeeman states, and that the two CPT dark states, which are produced successively by the alternate polarizations, add constructively. Here we experimentally investigate CPT signal dynamics first in the usual configuration, a single circular polarization. The double-modulation scheme is then addressed in both cases: one pulse Rabi interaction and two pulses Ramsey interaction. The impact and the optimization of the experimental parameters involved in the time sequence are reviewed. We show that a simple sevenlevel model explains the experimental observations. The double-modulation scheme yields a high contrast similar to the one of other high contrast configurations like push-pull optical pumping or crossed linear polarization scheme, with a setup allowing a higher compactness. The constructive polarization modulation is attractive for atomic clock, atomic magnetometer and high precision spectroscopy applications.
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