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Coherent population trapping with polarization modulation

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 Added by Enxue Yun
 Publication date 2016
  fields Physics
and research's language is English




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Coherent population trapping (CPT) is extensively studied for future vapor cell clocks of high frequency stability. In the constructive polarization modulation CPT scheme, a bichromatic laser field with polarization and phase synchronously modulated is applied on an atomic medium. A high contrast CPT signal is observed in this so-called double-modulation configuration, due to the fact that the atomic population does not leak to the extreme Zeeman states, and that the two CPT dark states, which are produced successively by the alternate polarizations, add constructively. Here we experimentally investigate CPT signal dynamics first in the usual configuration, a single circular polarization. The double-modulation scheme is then addressed in both cases: one pulse Rabi interaction and two pulses Ramsey interaction. The impact and the optimization of the experimental parameters involved in the time sequence are reviewed. We show that a simple sevenlevel model explains the experimental observations. The double-modulation scheme yields a high contrast similar to the one of other high contrast configurations like push-pull optical pumping or crossed linear polarization scheme, with a setup allowing a higher compactness. The constructive polarization modulation is attractive for atomic clock, atomic magnetometer and high precision spectroscopy applications.



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We demonstrate a vapor cell atomic clock prototype based on continuous-wave (CW) interrogation and double-modulation coherent population trapping (DM-CPT) technique. The DM-CPT technique uses a synchronous modulation of polarization and relative phase of a bi-chromatic laser beam in order to increase the number of atoms trapped in a dark state, i.e. a non-absorbing state. The narrow resonance, observed in transmission of a Cs vapor cell, is used as a narrow frequency discriminator in an atomic clock. A detailed characterization of the CPT resonance versus numerous parameters is reported. A short-term frequency stability of $3.2 times 10^{-13} tau^{-1/2}$ up to 100 s averaging time is measured. These performances are more than one order of magnitude better than industrial Rb clocks and comparable to those of best laboratory-prototype vapor cell clocks. The noise budget analysis shows that the short and mid-term frequency stability is mainly limited by the power fluctuations of the microwave used to generate the bi-chromatic laser. These preliminary results demonstrate that the DM-CPT technique is well-suited for the development of a high-performance atomic clock, with potential compact and robust setup due to its linear architecture. This clock could find future applications in industry, telecommunications, instrumentation or global navigation satellite systems.
144 - Peter Yun , Qinglin Li , Qiang Hao 2021
The coherent population trapping (CPT) atomic clock is very promising for use in next-generation spaceborne applications owing to its compactness and high performance. In this paper, we propose and implement a CPT atomic clock based on the direct modulation of a large-modulation-bandwidth and narrow-linewidth distributed Bragg reflector laser, which replaces the usually used external bulk modulator in the high-performance CPT clock. Our method retains the high performance while significantly reducing the size. Using this highly compact bichromatic light source and simplest CPT configuration, in which a circularly polarized bichromatic laser interrogates the ^{87}Rb atom system, a CPT signal of clock transition with a narrow linewidth and high contrast is observed. We then lock the local oscillator frequency to the CPT error signal and demonstrate a short-term frequency stability of 3.6 times 10^{-13} {tau}^{-1/2} (4 s le {tau} le 200 s). We attribute it to the ultralow laser frequency and intensity noise as well as to the high-quality-factor CPT signal. This study can pave the way for the development of compact high-performance CPT clocks based on our scheme.
In this letter we investigate the possibility to attain strongly confined atomic localization using interacting Rydberg atoms in a Coherent Population Trapping (CPT) ladder configuration, where a standing-wave (SW) is used as a coupling field in the second leg of the ladder. Depending on the degree of compensation of the Rydberg level energy shift induced by the van der Waals (vdW) interaction, by the coupling field detuning, we distinguish between two antiblockade regimes, i.e. a partial antiblockade (PA) and a full antiblockade (FA). While a periodic pattern of tightly localized regions can be achieved for both regimes, the PA allows much faster converge of spatial confinement yielding a high resolution Rydberg state-selective superlocalization regime for higher-lying Rydberg levels. In comparison, for lower-lying Rydberg levels the PA leads to an anomalous change of spectra linewidth, confirming the importance of using a stable uppermost state to achieve a superlocalization regime.
We report the realization and characterization using coherent population trapping (CPT) spectroscopy of an octadecyltrichlorosilane (OTS)-coated centimeter-scale Cs vapor cell. The dual-structure of the resonance lineshape, with presence of a narrow structure line at the top of a Doppler-broadened structure, is clearly observed. The linewidth of the narrow resonance is compared to the linewidth of an evacuated Cs cell and of a buffer gas Cs cell of similar size. The Cs-OTS adsorption energy is measured to be (0.42 $pm$ 0.03) eV, leading to a clock frequency shift rate of $2.7times10^{-9}/$K in fractional unit. A hyperfine population lifetime, $T_1$, and a microwave coherence lifetime, $T_2$, of 1.6 and 0.5 ms are reported, corresponding to about 37 and 12 useful bounces, respectively. Atomic-motion induced Ramsey narrowing of dark resonances is observed in Cs-OTS cells by reducing the optical beam diameter. Ramsey CPT fringes are detected using a pulsed CPT interrogation scheme. Potential applications of the Cs-OTS cell to the development of a vapor cell atomic clock are discussed.
The Dick effect can be a limitation of the achievable frequency stability of a passive atomic frequency standard when the ancillary frequency source is only periodically sampled. Here we analyze the Dick effect for a pulsed vapor cell clock using coherent population trapping (CPT). Due to its specific interrogation process without atomic preparation nor detection outside of the Ramsey pulses, it exhibits an original shape of the sensitivity function to phase noise of the oscillator. Numerical calculations using a three-level atom model are successfully compared with measurements; an approximate formula of the sensitivity function is given as an easy-to-use tool. A comparison of our CPT clock sensitivity to phase noise with a clock of the same duty cycle using a two-level system reveals a higher sensitivity in the CPT case. The influence of a free-evolution time variation and of a detection duration lengthening on this sensitivity is studied. Finally this study permitted to choose an adapted quartz oscillator and allowed an improvement of the clock fractional frequency stability at the level of 3.2x10-13 at 1s
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