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Register a new userNonlinear Mid-infrared Metasurface based on a Phase-Change Material
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The mid-wave infrared (MWIR) spectral region (3-5 {mu}m) is important to a vast variety of applications in imaging, sensing, spectroscopy, surgery, and optical communications. Efficient third-harmonic generation (THG), converting light from the MWIR range into the near-infrared, a region with mature optical detection and manipulation technologies, offers the opportunity to mitigate a commonly recognized limitation of current MWIR systems. In this work, we present the possibility of boosting THG in the MWIR through a metasurface design. Specifically, we demonstrate a 30-fold enhancement in a highly nonlinear phase change material Ge2Sb2Se4Te1 (GSST), by patterning arrays of subwavelength cylinders supporting a magnetic dipolar resonance. The unprecedented broadband transparency, large refractive index, and remarkably high nonlinear response, together with unique phase-change properties, make GSST-based metasurfaces an appealing solution for reconfigurable and ultra-compact nonlinear devices operating in the MWIR.
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Metasurfaces offer the potential to control light propagation at the nanoscale for applications in both free-space and surface-confined geometries. Existing metasurfaces frequently utilize metallic polaritonic elements with high absorption losses, and/or fixed geometrical designs that serve a single function. Here we overcome these limitations by demonstrating a reconfigurable hyperbolic metasurface comprising of a heterostructure of isotopically enriched hexagonal boron nitride (hBN) in direct contact with the phase-change material (PCM) vanadium dioxide (VO2). Spatially localized metallic and dielectric domains in VO2 change the wavelength of the hyperbolic phonon polaritons (HPhPs) supported in hBN by a factor 1.6 at 1450cm-1. This induces in-plane launching, refraction and reflection of HPhPs in the hBN, proving reconfigurable control of in-plane HPhP propagation at the nanoscale15. These results exemplify a generalizable framework based on combining hyperbolic media and PCMs in order to design optical functionalities such as resonant cavities, beam steering, waveguiding and focusing with nanometric control.
We propose a nonvolatile, reconfigurable, and narrowband mid-infrared bandpass filter based on surface lattice resonance in phase-change material Ge2Sb2Te5 (GST). The proposed filter is composed of a two-dimensional gold nanorod array embedded in a thick GST film. Results show that when GST transits from the amorphous state to the crystalline state, the narrowband reflection spectrum of the proposed filter is tuned from 3.197 {mu}m to 4.795 {mu}m, covering the majority of the mid-infrared regime, the peak reflectance decreases from 72.6% to 25.8%, and the corresponding Q-factor decreases from 19.6 to 10.3. We show that the spectral tuning range can be adjusted by varying the incidence angle or the lattice period. By properly designing the gold nanorod sizes, we also show that the Q-factor can be greatly increased to 70 at the cost of relatively smaller peak reflection efficiencies, and that the peak reflection efficiency can be further increased to 80% at the cost of relatively smaller Q-factors. We expect this work will advance the engineering of GST-based nonvalatile tunable surface lattice resonances and will promote their applications especially in reconfigurable narrowband filters.
Spatial light modulators (SLMs) are devices for modulating amplitude, phase or polarization of a light beam on demand. Such devices have been playing an indispensable inuence in many areas from our daily entertainments to scientific researches. In the past decades, the SLMs have been mainly operated in electrical addressing (EASLM) manner, wherein the writing images are created and loaded via conventional electronic interfaces. However, adoption of pixelated electrodes puts limits on both resolution and efficiency of the EASLMs. Here, we present an optically addressed SLM based on a nonlinear metasurface (MS-OASLM), by which signal light is directly modulated by another writing beam requiring no electrode. The MS-OASLM shows unprecedented compactness and is 400 nm in total thickness benefitting from the outstanding nonlinearity of the metasurface. And their subwavelength feature size enables a high resolution up to 250 line pairs per millimeter, which is more than one order of magnitude better than any currently commercial SLMs. Such MS-OASLMs could provide opportunities to develop the next generation of high resolution displays and all-optical information processing technologies.
The ability to engineer nonlinear optical processes in all-dielectric nanostructures is both of fundamental interest and highly desirable for high-performance, robust, and miniaturized nonlinear optical devices. Herein, we propose a novel paradigm for the efficient tuning of second-harmonic generation (SHG) process in dielectric nanoantennas by integrating with chalcogenide phase change material. In a design with Ge$_{2}$Sb$_{2}$Te$_{5}$ (GST) film sandwiched between the AlGaAs nanoantennas and AlO$_{x}$ substrate, the nonlinear SHG signal from the AlGaAs nanoantennas can be boosted via the resonantly localized field induced by the optically-induced Mie-type resonances, and further modulated by exploiting the GST amorphous-to-crystalline phase change in a non-volatile, multi-level manner. The tuning strategy originates from the modulation of resonant conditions by changes in the refractive index of GST. With a thorough examination of tuning performances for different nanoantenna radii, a maximum modulation depth as high as 540$%$ is numerically demonstrated. This work not only reveals out the potential of GST in optical nonlinearity control, but also provides promising strategy in smart designing tunable and reconfigurable nonlinear optical devices, e.g., light emitters, modulators, and sensors.
Active metasurfaces promise reconfigurable optics with drastically improved compactness, ruggedness, manufacturability, and functionality compared to their traditional bulk counterparts. Optical phase change materials (O-PCMs) offer an appealing material solution for active metasurface devices with their large index contrast and nonvolatile switching characteristics. Here we report what we believe to be the first electrically reconfigurable nonvolatile metasurfaces based on O-PCMs. The O-PCM alloy used in the devices, Ge2Sb2Se4Te1 (GSST), uniquely combines giant non-volatile index modulation capability, broadband low optical loss, and a large reversible switching volume, enabling significantly enhanced light-matter interactions within the active O-PCM medium. Capitalizing on these favorable attributes, we demonstrated continuously tunable active metasurfaces with record half-octave spectral tuning range and large optical contrast of over 400%. We further prototyped a polarization-insensitive phase-gradient metasurface to realize dynamic optical beam steering.
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