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Energy-efficient generation of skyrmion phases in Co/Ni/Pt-based multilayers using Joule heating

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 Added by Jeffrey Brock
 Publication date 2020
  fields Physics
and research's language is English




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We have studied the effects of electrical current pulses on skyrmion formation in a series of Co/Ni/Pt-based multilayers. Transmission X-ray microscopy reveals that by applying electrical current pulses of duration and current density on the order of $tau$=50 $mu$s and j=1.7x10$^1$$^0$ A/m$^2$, respectively, in an applied magnetic field of $mu$$_0$Hz=50 mT, stripe-to-skyrmion transformations are attained. The skyrmions remain stable across a wide range of magnetic fields, including zero field. The skyrmions then remain stable across a wide range of magnetic fields, including zero field. We primarily attribute the transformation to current-induced Joule heating on the order of ~125 K. Reducing the magnetic moment and perpendicular anisotropy using thin rare-earth spacers dramatically reduces the pulse duration, current density, and magnetic field necessary to 25 $mu$s, 2.4x10$^9$ A/m$^2$, and 27 mT, respectively. These findings show that energetic inputs allow for the formation of skyrmion phases in a broad class of materials and that material properties can be tuned to yield more energy-efficient access to skyrmion phases.



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We experimentally investigate the current-induced magnetization reversal in Pt/[Co/Ni]$_3$/Al multilayers combining the anomalous Hall effect and magneto-optical Kerr effect techniques in crossbar geometry. The magnetization reversal occurs through nucleation and propagation of a domain of opposite polarity for a current density of the order of 0.3 TA/m$^2$. In these experiments we demonstrate a full control of each stage: i)the {O}rsted field controls the domain nucleation and ii) domain-wall propagation occurs by spin torque from the Pt spin Hall effect. This scenario requires an in-plane magnetic field to tune the domain wall center orientation along the current for efficient domain wall propagation. Indeed, as nucleated, domain walls are chiral and Neel like due to the interfacial Dzyaloshinskii-Moriya interaction.
We characterize the magnetic properties and domain structure of Pt/Ni/Co asymmetric superlattices in comparison to the more established Pt/Co/Ni structure. This reversal in stacking sequence leads to a marked drop in interfacial magnetic anisotropy and the magnitude of the interfacial Dzyaloshinskii-Moriya interaction (DMI) as inferred from the DW structure, which we speculate could be related to a degradation of the Pt/Co interface when Pt is deposited on top of the Co layer. Lorentz transmission electron microscopy reveals exclusively Neel type domain walls and, with a perpendicular field, Neel skyrmions in the Pt/Co/Ni films. Conversely, the Pt/Ni/Co samples show only achiral Bloch domain walls, which leads to the formation of achiral Bloch ($Q=1$) and type II bubbles ($Q=0$) at increased perpendicular field. Combined with the reduced anisotropy leading to greater bubble densities, the latter case makes for an excellent test bed to examine the benefits of topological charge on stability. Simultaneous observation of Bloch and type II bubbles shows a roughly 50 mT larger annihilation field for the former. An in-plane component to the magnetic field is shown to both impact the structure of the formed bubbles and separately suppress the topological benefit.
By means of systematic first-principles calculations based on density functional theory we search for suitable materials that can host antiferromagnetically coupled skyrmions. We concentrate on fcc-stacked (111)-oriented metallic $Z$/Co/Pt ($Z=4d$ series: Y$-$Pd, the noble metals: Cu, Ag, Au, post noble metals: Zn and Cd) magnetic multilayers of films of monatomic thickness. We present quantitative trends of magnetic properties: Magnetic moments, interlayer exchange coupling, spin-stiffness, Dzyaloshinskii-Moriya interaction, magnetic anisotropy, and the critical temperature. We show that some of the $Z$ elements (Zn, Y, Zr, Nb, Tc, Ru, Rh, and Cd) can induce antiferromagnetic interlayer coupling between the magnetic Co layers, and that they influence the easy magnetization axis. Employing a multiscale approach, we transfer the micromagnetic parameters determined from $ab$ $initio$ to a micromagnetic energy functional and search for one-dimensional spin-spiral solutions and two-dimensional skyrmions. We determine the skyrmion radius by numerically solving the equation of the skyrmion profile. We found an analytical expression for the skyrmion radius that covers our numerical results and is valid for a large regime of micromagnetic parameters. Based on this expression we have proposed a model that allows to extrapolate from the $ab$ $initio$ results of monatomic films to multilayers with Co films consisting of several atomic layers containing $10,$nm skyrmions. We found thickness regimes where tiny changes of the film thickness may alter the skyrmion radius by orders of magnitude. We estimated the skyrmion size as function of temperature and found that the size can easily double going from cryogenic to room temperature. We suggest promising material systems for ferromagnetically and antiferromagnetically coupled spin-spiral and skyrmion systems.
Using broadband ferromagnetic resonance, we measure the damping parameter of [Co(5 r{A})/Pt(3 r{A})]${times 6}$ multilayers whose growth was optimized to maximize the perpendicular anisotropy. Structural characterizations indicate abrupt interfaces essentially free of intermixing despite the miscible character of Co and Pt. Gilbert damping parameters as low as 0.021 can be obtained despite a magneto-crystalline anisotropy as large as $10^6~textrm{J/m}^3$. The inhomogeneous broadening accounts for part of the ferromagnetic resonance linewidth, indicating some structural disorder leading to a equivalent 20 mT of inhomogenity of the effective field. The unexpectedly relatively low damping factor indicates that the presence of the Pt heavy metal within the multilayer may not be detrimental to the damping provided that intermixing is avoided at the Co/Pt interfaces.
Materials hosting magnetic skyrmions at room temperature could enable new computing architectures as well as compact and energetically efficient magnetic storage such as racetrack memories. In a racetrack device, information is coded by the presence/absence of magnetic skyrmions forming a chain that is moved through the device. The skyrmion Hall effect that would eventually lead to an annihilation of the skyrmions at the edges of the racetrack can be suppressed for example by anti-ferromagnetically-coupled skyrmions. However, avoiding modifications of the inter-skyrmion distances in the racetrack remains challenging. As a solution to this issue, a chain of bits could also be encoded by two different solitons such as a skyrmion and a chiral bobber. The major limitation of this approach is that it has solely been realized in B20-type single crystalline material systems that support skyrmions only at low temperatures, thus hindering the efficacy for future applications. Here we demonstrate that a hybrid ferro/ferri/ferromagnetic multilayer system can host two distinct skyrmion phases at room temperature. By matching quantitative magnetic force microscopy data with micromagnetic simulations, we reveal that the two phases represent tubular skyrmions and partial skyrmions (similar to skyrmion bobbers). Furthermore, the tubular skyrmion can be converted into a partial skyrmion. Such multilayer systems may thus serve as a platform for designing skyrmion memory applications using distinct types of skyrmions and potentially for storing information using the vertical dimension in a thin film device.
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