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Role of instability on the limits of laterally strained detonation waves

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 Added by Qiang Xiao
 Publication date 2020
  fields Physics
and research's language is English




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The present work examines the role of instability and diffusive phenomena in controlling the limits of detonations subject to lateral strain rates. Experiments were conducted in hydrocarbon-oxygen mixtures with varying levels of cellular instability. These detonations were propagated in channels with exponentially enlarging cross-sections, following the recent works of Radulescu & Borzou (2018) and Xiao & Radulescu (2020). Steady detonation waves were obtained at the macro-scale, with the near-limit reaction zone structures characterized by significant unreacted gas pockets. The turbulent flame burning velocity of these pockets was evaluated to be 30 m/s to 70 m/s, which is larger than the theoretical laminar value by a factor of 2 to 7. For all the mixtures tested, the characteristic $D-K$ relationships, relating the detonation mean propagation speed with lateral flow divergence, were obtained directly from experiments and as well from the generalized ZND model with lateral strain rates using detailed chemical kinetics. The results showed that the degree of departure between experiments and the theoretical predictions increases significantly with the detonation instability level. As compared to the laminar ZND wave, the more unstable detonations are much more detonable than the more stable detonations, with substantially larger limiting divergence rates and maximum velocity deficits. Such enhanced detonability with detonation instability can be manifested in the significantly enhanced global rates of energy release with the notably suppressed thermal character of ignition for the more unstable detonations. This globally enhanced burning mechanism is found to be realized by the intensified auto-ignition assisted by the turbulent diffusive burning of the unreacted gas pockets, substantially shortening the characteristic reaction zone lengths.



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84 - Prateek Gupta 2021
We begin with the theoretical study of spectral energy cascade due to the propagation of high amplitude sound in the absence of thermal sources. To this end, a first-principles-based system of governing equations, correct up to second order in perturbation variables is derived. The exact energy corollary of such second-order system of equations is then formulated and used to elucidate the spectral energy dynamics of nonlinear acoustic waves. We then extend this analysis to thermoacoustically unstable waves -- i.e. amplified as a result of thermoacoustic instability. We drive such instability up until the generation of shock waves. We further study the nonlinear wave propagation in geometrically complex case of waves induced by the spark plasma between the electrodes. This case adds the geometrical complexity of a curved, three-dimensional shock, yielding vorticity production due to baroclinic torque. Finally, detonation waves are simulated by using a low-order approach, in a periodic setup subjected to high pressure inlet and exhaust of combustible gaseous mixture. An order adaptive fully compressible and unstructured Navier Stokes solver is currently under development to enable higher fidelity studies of both the spark plasma and detonation wave problem in the future.
The present study addresses the reaction zone structure and burning mechanism of unstable detonations. Experiments investigated mainly two-dimensional methane-oxygen cellular detonations in a thin channel geometry. The sufficiently high temporal resolution permitted to determine the PDF of the shock distribution, a power-law with an exponent of -3, and the burning rate of unreacted pockets from their edges - through surface turbulent flames with a speed approximately 3-7 times larger than the laminar one at the local conditions. Numerical simulations were performed using a novel Large Eddy Simulation method where the reactions due to both auto-ignition and turbulent transport and treated exactly at the sub-grid scale in a reaction-diffusion formulation. The model is an extension of Kerstein & Menons Linear Eddy Model for Large Eddy Simulation to treat flows with shock waves and rapid gasdynamic transients. The two-dimensional simulations recovered well the amplification of the laminar flame speed owing to the turbulence generated mainly by the shear layers originating from the triple points and subsequent Richtmyer-Meshkov instability associated with the internal pressure waves. The simulations clarified how the level of turbulence generated controlled the burning rate of the pockets, the hydrodynamic thickness of the wave, the cellular structure and its distribution. Three-dimensional simulations were found in general good agreement with the two-dimensional ones, in that the sub-grid scale model captured the ensuing turbulent burning once the scales associated with the cellular dynamics, where turbulent kinetic energy is injected, are well resolved.
Instabilities in rotating detonation are concerned because of their potential influence on the stability of operation. Previous studies on instability of 2-D rotating detonation mainly cared about the one of the contact discontinuity originated from the conjunction of the detonation and oblique shock. Hishida et al. first found the rippled structure existed in the interface between fresh injections and burnt product from the previous cycle (Shock Waves 19, 2009), and a mechanism of Kelvin-Helmholtz instability was suggested as well. Similar structures were observed as well in simulations by current authors, where a fifth-order WENO-type scheme with improved resolution and 7-species-and-8-reaction chemical model were used. In order to achieve a deep understanding on the flow mechanism, more careful simulations are carried out by using three grids with increasing resolution. The results show that besides the previously-mentioned Kelvin-Helmholtz instability, there are two other mechanisms which take effect in the interface instability, i.e., the effect of baroclinic torque and Rayleigh-Taylor instability. Occurrence conditions for two instabilities are checked and testified. Especially, the spike- and bubble-like structures are observed at the interface, which show appearances different from canonical structures by Kelvin-Helmholtz instability.
We evaluate the effect of boundary layer losses on two-dimensional H2/O2/Ar cellular detonations obtained in narrow channels. The experiments provide the details of the cellular structure and the detonation speed deficits from the ideal CJ speed. We model the effect of the boundary layer losses by incorporating the flow divergence in the third dimension due to the negative boundary layer displacement thickness, modeled using Mirels theory. The cellular structures obtained numerically with the resulting quasi-2D formulation of the reactive Euler equations with two-step chain-branching chemistry are found in excellent agreement with experiment, both in terms of cell dynamics and velocity deficits, provided the boundary layer constant of Mirels is modified by a factor of 2. A significant increase in the cell size is found with increasing velocity deficit. This is found to be very well captured by the induction zone increase in slower detonations due to the lower temperatures in the induction zone.
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