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Register a new userNanoscale electrometry based on a magnetic-field-resistant spin sensor
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The nitrogen-vacancy (NV) center is a potential atomic-scale spin sensor for electric field sensing. However, its natural susceptibility to the magnetic field hinders effective detection of the electric field. Here we propose a robust electrometric method utilizing continuous dynamic decoupling (CDD) technique. During the CDD period, the NV center evolves in a dressed-state space, where the sensor is resistant to magnetic fields but remains sensitive to electric fields. As an example, we use this method to isolate the electric noise from a complex electro-magnetical environment near diamond surface via measuring the dephasing rate between dressed states. By reducing the surface electric noise with different covered liquids, we observe an unambiguous relation between the dephasing rate and the dielectric permittivity of the liquid, which enables a quantitative investigation of electric noise model near diamond surface.
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We develop a systematic method of performing corrected gate operations on an array of exchange-coupled singlet-triplet qubits in the presence of both fluctuating nuclear Overhauser field gradients and charge noise. The single-qubit control sequences we present have a simple form, are relatively short, and form the building blocks of a corrected CNOT gate when also implemented on the inter-qubit exchange link. This is a key step towards enabling large-scale quantum computation in a semiconductor-based architecture by facilitating error reduction below the quantum error correction threshold for both single-qubit and multi-qubit gate operations.
As a nuclear spin model of scalable quantum register, the one-dimensional chain of the magnetic atoms with nuclear spins 1/2 substituting the basic atoms in the plate of nuclear spin free easy-axis 3D antiferromagnet is considered. It is formulated the generalized antiferromagnet Hamiltonian in spin-wave approximation (low temperatures) considering the inhomogeneous external magnetic field, which is directed along the easy axis normally to plane of the plate and has a constant gradient along the nuclear spin chain. Assuming a weak gradient, the asymptotic expression for coefficients of unitary transformations to the diagonal form of antiferromagnet Hamiltonian is found. With this result the expression for indirect interspin coupling, which is due to hyperfine nuclear electron coupling in atoms and the virtual spin wave propagation in antiferromagnet ground state, was evaluated. It is shown that the inhomogeneous magnetic field essentially modifies the characteristics of indirect interspin coupling. The indirect interaction essentially grows and even oscillates in relation to the interspin distance when the local field value in the middle point of two considered nuclear spin is close to the critical field for quantum phase transition of spin-flop type in bulk antiferromagnet or close to antiferromagnetic resonance. Thus, the external magnetic field, its gradient, microwave frequency and power can play the role of control parameters for qubit states. Finally, the one and two qubit states decoherence and longitudinal relaxation rate are caused by the interaction of nuclear spins with virtual spin waves in antiferromagnet ground state are calculated.
Recently we have demonstrated AC magnetic field sensing scheme using a simple continuous-wave optically detected magnetic resonance of nitrogen-vacancy centers in diamond [Appl. Phys. Lett. 113, 082405 (2018)]. This scheme is based on electronic spin double resonance excited by continuous microwaves and radio-frequency (RF) fields. Here we measured and analyzed the double resonance spectra and magnetic field sensitivity for various frequencies of microwaves and RF fields. As a result, we observed a clear anticrossing of RF-dressed electronic spin states in the spectra and estimated the bandwidth to be approximately 5 MHz at the center frequency of 9.9 MHz.
In nanoscale metrology applications, measurements are commonly limited by the performance of the sensor. Here we show that in nuclear magnetic resonance (NMR) spectroscopy measurements using single nitrogen-vacancy (NV) centers in diamond, the NV sensor electron spin limits spectral resolution down to a few hundred Hz, which constraints the characterization and coherent control of finite spin systems, and furthermore, is insufficient for high resolution NMR spectroscopy aiming at single molecule recognition and structure analysis of the latter. To overcome the limitation, we support an NV electron spin sensor with a nuclear spin qubit acting as quantum and classical memory allowing for intermediate nonvolatile storage of metrology information, while suppressing the deleterious back-action of the sensor onto the system under investigation. We demonstrate quantum and classical memory lifetimes of 8 ms and 4 minutes respectively under ambient conditions. Furthermore, we design and test measurement and decoupling protocols, which exploit such memory qubits efficiently. Using our hybrid quantum-classical sensor device, we achieve high resolution NMR spectra with linewidths of single spins down to 13 Hz. Our work is therefore a prerequisite for high resolution NMR spectroscopy on nanoscopic quantum systems down to the single level.
Quantum sensing exploits the strong sensitivity of quantum systems to measure small external signals. The nitrogen-vacancy (NV) center in diamond is one of the most promising platforms for real-world quantum sensing applications, predominantly used as a magnetometer. However, its magnetic field sensitivity vanishes when a bias magnetic field acts perpendicular to the NV axis. Here, we introduce a novel sensing strategy assisted by the nitrogen nuclear spin that uses the entanglement between the electron and nuclear spins to restore the magnetic field sensitivity. This, in turn, allows us to detect small changes in the magnetic field angle relative to the NV axis. Furthermore, based on the same underlying principle, we show that the NV coupling strength to magnetic noise, and hence its coherence time, exhibits a strong asymmetric angle dependence. This allows us to uncover the directional properties of the local magnetic environment and to realize maximal decoupling from anisotropic noise.
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