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Register a new userColossal quasiparticle radiation in the Lifshitz spin liquid phase of a two-dimensional quantum antiferromagnet
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Strong quantum fluctuations in magnetic systems can create disordered quantum spin liquid phases of matter which are not predicted by classical physics. The complexity of the exotic phenomena on display in spin liquids has led to a great deal of theoretical and experimental interest. However, understanding the fundamental nature of the excitations in these systems remains challenging. In this work, we consider the Lifshitz quantum critical point in a two-dimensional frustrated $XY$ antiferromagnet. At this point, quantum fluctuations destroy long range order, leading to the formation of an algebraic Lifshitz spin liquid. We demonstrate that the bosonic magnon excitations are long-lived and well-defined in the Lifshitz spin liquid phase, though paradoxically, the dynamic structure factor has a broad non-Lorentzian frequency distribution with no single-particle weight. We resolve this apparent contradiction by showing that the Lifshitz spin liquid suffers from an infrared catastrophe: An external physical probe always excites an infinite number of arbitrarily low energy quasiparticles, which leads to significant radiative broadening of the spectrum.
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Quantum spin liquid (QSL) is a novel state of matter which refuses the conventional spin freezing even at 0 K. Experimentally searching for the structurally perfect candidates is a big challenge in condensed matter physics. Here we report the successful synthesis of a new spin-1/2 triangular antiferromagnet YbMgGaO$_4$ with R$bar{3}$m symmetry. The compound with an ideal two-dimensional and spatial isotropic magnetic triangular-lattice has no site-mixing magnetic defects and no antisymmetric Dzyaloshinsky-Moriya (DM) interactions. No spin freezing down to 60 mK (despite $Theta$$_w$ $sim$ -4 K), the low-T power-law temperature dependence of heat capacity and nonzero susceptibility suggest that YbMgGaO$_4$ is a promising gapless ($leq$ $|$$Theta$$_w$$|$/100) QSL candidate. The residual spin entropy, which is accurately determined with a non-magnetic reference LuMgGaO$_4$, approaches zero ($<$ 0.6 %). This indicates that the possible QSL ground state (GS) of the frustrated spin system has been experimentally achieved at the lowest measurement temperatures.
Spin liquid ground states are predicted to arise within several distinct scenarios in condensed matter physics. The observation of these disordered magnetic states is particularly pervasive amongst a class of materials known as frustrated magnets, in which the competition between various magnetic exchange interactions prevents the system from adopting long-range magnetic order at low temperatures. Spin liquids continue to be of great interest due to their exotic nature and the possibility that they may support fractionalised excitations, such as Majorana fermions. Systems that allow for such phenomena are not only fascinating from a fundamental perspective but may also be practically significant in future technologies based on quantum computation. Here we show that the underlying antiferromagnetic sublattice in TbInO$_3$ undergoes a crystal field induced triangular-to-honeycomb dilution at low temperatures. The absence of a conventional magnetic ordering transition at the lowest measurable temperatures indicates that another critical mechanism must govern in the ground state selection of TbInO$_3$. We propose that anisotropic exchange interactions, mediated through strong spin-orbit coupling on the emergent honeycomb lattice of TbInO$_3$, give rise to a highly frustrated spin liquid.
We report magnetization and specific heat measurements in the 2D frustrated spin-1/2 Heisenberg antiferromagnet Cs2CuCl4 at temperatures down to 0.05 K and high magnetic fields up to 11.5 T applied along a, b and c-axes. The low-field susceptibility chi (T) M/B shows a broad maximum around 2.8 K characteristic of short-range antiferromagnetic correlations and the overall temperature dependence is well described by high temperature series expansion calculations for the partially frustrated triangular lattice with J=4.46 K and J/J=1/3. At much lower temperatures (< 0.4 K) and in in-plane field (along b and c-axes) several new intermediate-field ordered phases are observed in-between the low-field incommensurate spiral and the high-field saturated ferromagnetic state. The ground state energy extracted from the magnetization curve shows strong zero-point quantum fluctuations in the ground state at low and intermediate fields.
The study of randomness in low-dimensional quantum antiferromagnets is at the forefront of research in the field of strongly correlated electron systems, yet there have been relatively few experimental model systems. Complementary neutron scattering and numerical experiments demonstrate that the spin-diluted Heisenberg antiferromagnet La2Cu(1-z)(Zn,Mg)zO4 is an excellent model material for square-lattice site percolation in the extreme quantum limit of spin one-half. Measurements of the ordered moment and spin correlations provide important quantitative information for tests of theories for this complex quantum-impurity problem.
The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet fluctuating states exist. By combining complementary local-probe techniques with neutron scattering, we discover a crossover from a critical regime into a gapless spin-liquid phase with decreasing temperature. An additional unconventional instability of the latter phase leads to a second, distinct spin-liquid state that is stabilized at the lowest temperatures. We advance such complex behavior as a feature common to different frustrated quantum magnets.
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