We have investigated the structural, magnetic and superconducting properties of [Nb(1.5nm)/Fe(x)]$_{10}$ superlattices deposited on a thick Nb(50nm) layer. Our investigation showed that the Nb(50nm) layer grows epitaxially at 800$^circ$C on Al$_2$O$_3$(1$bar{1}$02) substrate. Samples grown at this condition posses a high residual resistivity ratio of 15-20. By using neutron reflectometry we show that Fe/Nb superlattices with $x<$ 4 nm form a depth-modulated FeNb alloy with concentration of iron varying between 60% and 90%. This alloy has properties of a weak ferromagnet. Proximity of this weak ferromagnetic layer to a thick superconductor leads to an intermediate phase that is characterized by co-existing superconducting and normal-state domains. By increasing the thickness of the Fe layer to $x$ = 4 nm the intermediate phase disappears. We attribute the intermediate state to proximity induced non-homogeneous superconductivity in the periodic Fe/Nb structure.
We report an investigation of the structural and electronic properties of hybrid superconductor/ferromagnet (S/F) bilayers of composition Nb/Cu$_{60}$Ni$_{40}$ prepared by magnetron sputtering. X-ray and neutron reflectometry show that both the overall interfacial roughness and vertical correlations of the roughness of different interfaces are lower for heterostructures deposited on Al$_2$O$_3$(1$bar{1}$02) substrates than for those deposited on Si(111). Mutual inductance experiments were then used to study the influence of the interfacial roughness on the superconducting transition temperature, $T_C$. These measurements revealed a $sim$ 4% higher $T_C$ in heterostructures deposited on Al$_2$O$_3$, compared to those on Si. We attribute this effect to a higher mean-free path of electrons in the S layer, caused by a suppression of diffusive scattering at the interfaces. However, the dependence of the $T_C$ on the thickness of the ferromagnetic layer is not significantly different in the two systems, indicating a weak influence of the interfacial roughness on the transparency for Cooper pairs.
The physics of the $pi$ phase shift in ferromagnetic Josephson junctions may enable a range of applications for spin-electronic devices and quantum computing. We investigate transitions from ``0 to ``$pi$ states in Nb/Fe/Nb Josephson junctions by varying the Fe barrier thickness from 0.5 nm to 5.5 nm. From magnetic measurements we estimate for Fe a magnetic dead layer of about 1.1 nm. By fitting the characteristic voltage oscillations with existing theoretical models we extrapolate an exchange energy of 256 meV, a Fermi velocity of $1.98 times 10^5$ m/s and an electron mean free path of 6.2 nm, in agreement with other reported values. From the temperature dependence of the $I_CR_N$ product we show that its decay rate exhibits a nonmonotonic oscillatory behavior with the Fe barrier thickness.
We have used spin-polarized neutron reflectometry to investigate the magnetization profile of superlattices composed of ferromagnetic Gd and superconducting Nb layers. We have observed a partial suppression of ferromagnetic (F) order of Gd layers in [Gd($d_F$)/Nb(25nm)]$_{12}$ superlattices below the superconducting (S) transition of the Nb layers. The amplitude of the suppression decreases with increasing $d_F$. By analyzing the neutron spin asymmetry we conclude that the observed effect has an electromagnetic origin - the proximity-coupled S layers screen out the external magnetic field and thus suppress the F response of the Gd layers inside the structure. Our investigation demonstrates the considerable influence of electromagnetic effects on the magnetic properties of S/F systems.
Measurements of the polar Kerr effect using a zero-area-loop Sagnac magnetometer on Pb/Ni and Al/(Co-Pd) proximity-effect bilayers show unambiguous evidence for the inverse proximity effect, in which the ferromagnet (F) induces a finite magnetization in the superconducting (S) layer. To avoid probing the magnetic effects in the ferromagnet, the superconducting layer was prepared much thicker than the lights optical penetration depth. The sign and size of the effect, as well as its temperature dependence agree with recent predictions by Bergeret et al..
$mathrm{YBa_2Cu_3O_7/La_{2/3}Ca_{1/3}MnO_3}$ superconducting/ferromagnetic (SC/FM) multilayers have been studied by neutron reflectometry. Evidence for a characteristic difference between the structural and magnetic depth profiles is obtained from the occurrence of a structurally forbidden Bragg peak in the FM state. The comparison with simulated reflectivity curves allows us to identify two possible magnetization profiles: a sizable magnetic moment within the SC layer antiparallel to the one in the FM layer (inverse proximity effect), or a ``dead region in the FM layer with zero net magnetic moment. The former scenario is supported by an anomalous SC-induced enhancement of the off-specular reflection, which testifies to a strong mutual interaction of SC and FM order parameters.