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Register a new userWideband tunable infrared topological plasmon polaritons in dimerized chains of doped-silicon nanoparticles
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We investigate the topological plasmon polaritons (TPPs) in one-dimensional dimerized doped silicon nanoparticle chains, as an analogy of the topological edge states in the Su-Schrieffer-Heeger (SSH) model. The photonic band structures are analytically calculated by taking all near-field and far-field dipole-dipole interactions into account. For longitudinal modes, it is demonstrated that the band topology can be well characterized by the complex Zak phase irrespective of the lattice constant and doping concentration. By numerically solving the eigenmodes of a finite system, it is found that a dimerized chain with a nonzero complex Zak phase supports nontrivial topological eigenmodes localized over both edges. Moreover, by changing the doping concentration of Si, it is possible to tune the resonance frequency of the TPPs from far-infrared to near-infrared, and the localization length of the edge modes are also modulated accordingly. Since these TPPs are highly protected modes that can achieve a strong confinement of electromagnetic waves and are also immune to impurities and disorder, they can provide a potentially tunable tool for robust and enhanced light-matter interactions light-matter interaction in the infrared spectrum.
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We develop a quantum theory of plasmon polaritons in chains of metallic nanoparticles, describing both near- and far-field interparticle distances, by including plasmon-photon Umklapp processes. Taking into account the retardation effects of the long-range dipole-dipole interaction between the nanoparticles, which are induced by the coupling of the plasmonic degrees of freedom to the photonic continuum, we reveal the polaritonic nature of the normal modes of the system. We compute the dispersion relation and radiative linewidth, as well as the group velocities of the eigenmodes, and compare our numerical results to classical electrodynamic calculations within the point-dipole approximation. Interestingly, the group velocities of the polaritonic excitations present an almost periodic sign change and are found to be highly tunable by modifying the spacing between the nanoparticles. We show that, away from the intersection of the plasmonic eigenfrequencies with the free photon dispersion, an analytical perturbative treatment of the light-matter interaction is in excellent agreement with our fully retarded numerical calculations. We further study quantitatively the hybridization of light and matter excitations, through an analysis of Hopfields coefficients. Finally, we consider the limit of infinitely spaced nanoparticles and discuss some recent results on single nanoparticles that can be found in the literature.
We study the topological edge plasmon modes between two diatomic chains of identical plasmonic nanoparticles. Zak phase for longitudinal plasmon modes in each chain is calculated analytically by solutions of macroscopic Maxwells equations for particles in quasi-static dipole approximation. This approximation provides a direct analogy with the Su-Schrieffer-Heeger model such that the eigenvalue is mapped to the frequency dependent inverse-polarizability of the nanoparticles. The edge state frequency is found to be the same as the single-particle resonance frequency, which is insensitive to the separation distances within a unit cell. Finally, full electrodynamic simulations with realistic parameters suggest that the edge plasmon mode can be realized through near-field optical spectroscopy.
We theoretically investigate the application of topological plasmon polaritons (TPPs) to temperature sensing for the first time. Based on an analogy of the topological edge states in the Su-Schrieffer-Heeger model, TPPs are realized in a one-dimensional intrinsic indium antimonide (InSb) microsphere chain. The existence of TPPs is demonstrated by analyzing the topology of the photonic band structures and the eigenmode distribution. By exploiting the temperature dependence of the permittivity of InSb in the terahertz range, the resonance frequency of the TPPs can be largely tuned by the temperature. Moreover, it is shown that the temperature sensitivity of the TPP resonance frequency can be as high as $0.0264~mathrm{THz/K}$ at room temperature, leading to a figure of merit over 150. By calculating the LDOS near the chain, we further demonstrate that the temperature sensitivity of TPPs is experimentally detectable via near-field probing techniques. This sensitivity is robust since TPPs are highly protected modes immune to disorder and can achieve a strong confinement of radiation. We envisage these TPPs can be utilized as promising candidates for robust and enhanced temperature sensing.
We propose a new type of reflective polarizer based on polarization-dependent coupling to surface-plasmon polaritons (SPPs) from free space. This inexpensive polarizer is relatively narrowband but features an extinction ratio of up to 1000 with efficiency of up to 95% for the desired polarization (numbers from a calculation), and thus can be stacked to achieve extinction ratios of 106 or more. As a proof of concept, we experimentally realized a polarizer based on nanoporous aluminum oxide that operates around a wavelength of 10.6 um, corresponding to the output of a CO2 laser, using aluminum anodization, a low-cost electrochemical process.
We have observed laser-like emission of surface plasmon polaritons (SPPs) decoupled to the glass prism in an attenuated total reflection setup. SPPs were excited by optically pumped molecules in a polymeric film deposited on the top of the silver film. Stimulated emission was characterized by a distinct threshold in the input-output dependence and narrowing of the emission spectrum. The observed stimulated emission and corresponding to it compensation of the metallic absorption loss by gain enables many applications of metamaterials and nanoplasmonic devices.
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