No Arabic abstract
The Dirac semimetal PdTe$_2$ was recently reported to be a type-I superconductor with $T_c = 1.64$ K and a critical field $mu_0H_c = 13.6$ mT. Since type-I superconductivity is unexpected for binary compounds, we have conducted muon spin rotation experiments to probe the superconducting phase on the microscopic scale via its intermediate state. For crystals with a finite demagnetization factor, $N$, the intermediate state forms in applied fields $(1-N)H_c < H_a < H_c$. We have carried out transverse field muon spin rotation measurements on a thin disk-like crystal with the field perpendicular to ($N_{perp}=0.86$) and in the plane ($N_{parallel}=0.08$) of the disk. By analysing the $mu$SR signal we find that the volume fraction of the normal domains grows quasi-linearly with applied field at the expense of the Meissner domain fraction. This then provides solid evidence for the intermediate state and type-I superconductivity in the bulk of PdTe$_2$.
The type-II Dirac semimetal PdTe2 was recently reported to be a type-I superconductor with a superconducting transition temperature Tc = 1.65 K. However, the recent results from tunneling and point contact spectroscopy suggested the unusual state of a mixture of type-I and type-II superconductivity. These contradictory results mean that there is no clear picture of the superconducting phase diagram and warrants a detailed investigation of the superconducting phase. We report here the muon spin rotation and relaxation ($mu$SR) measurements on the superconducting state of the topological Dirac semimetal PdTe2. From $mu$SR measurements, we find that PdTe2 exhibits mixed type-I/type-II superconductivity. Using these results a phase diagram has been determined. In contrast to previous results where local type-II superconductivity persists up to Hc2 = 600 G, we observed that bulk superconductivity is destroyed above 225 G.
Type I superconductivity has recently been reported for the Dirac semimetal PdTe$_2$ (Tc approximately 1.6K) with, remarkably, multiple critical fields and a complex phase diagram. Here, measurements of the specific heat utilizing a thermal relaxation technique are presented. Conventional weak-coupling BCS superconductivity is confirmed by examining the temperature dependence of the specific heat in zero field. By probing the latent heat accompanying the superconducting transition, thermodynamic evidence for type I superconductivity is attained. The presence of the intermediate state is observed as a significant broadening of the superconducting transition onto lower temperatures at high fields as well as irreversibility in the specific heat in zero field cooled data at 8.5 mT.
The transition metal dichalcogenide PdTe$_2$ was recently shown to be a unique system where a type II Dirac semimetallic phase and a superconducting phase co-exist. This observation has led to wide speculation on the possibility of the emergence of an unconventional topological superconducting phase in PdTe$_2$. Here, through direct measurement of the superconducting energy gap by scanning tunneling spectroscopy (STS), and temperature and magnetic field evolution of the same, we show that the superconducting phase in PdTe$_2$ is conventional in nature. The superconducting energy gap is measured to be 326 $mu$eV at 0.38 K and it follows a temperature dependence that is well described within the framework of Bardeen-Cooper-Schriefers (BCS) theory of conventional superconductivity. This is surprising because our quantum oscillation measurements confirm that at least one of the bands participating in transport has topologically non-trivial character.
The comprehensive study of the temperature dependent x-ray absorption spectroscopy (XAS) reveals a dynamical spectral weight $alpha$ in YBa$_2$Cu$_3$O$_y$ (YBCO). Large spectral weight changes for both the Upper Hubbard band and the Zhang-Rice band due to dynamics of holes are experimentally found in the underdoped regime. A large value of $alpha geq 0.3$ is indispensable to describing XAS of YBCO with the conservation of states. The value of $alpha$ is linearly proportional to the pseudogap temperature in the underdoped regime, but becomes smaller as the doping level goes to the undoped limit. Our results clearly indicate that the pseudogap is related to the double occupancy and originates from bands in higher energies.
We report a polarization-resolved Raman spectroscopy study of the orbital dependence of the quasiparticles properties in the prototypical multi-band Fermi liquid Srtextsubscript{2}RuOtextsubscript{4}. We show that the quasiparticle scattering rate displays $omega^{2}$ dependence as expected for a Fermi liquid. Besides, we observe a clear polarization-dependence in the energy and temperature dependence of the quasiparticle scattering rate and mass, with the $d_{xz/yz}$ orbital derived quasiparticles showing significantly more robust Fermi liquid properties than the $d_{xy}$ orbital derived ones. The observed orbital dichotomy of the quasiparticles is consistent with the picture of Srtextsubscript{2}RuOtextsubscript{4} as a Hunds metal. Our study establishes Raman scattering as a powerful probe of Fermi liquid properties in correlated metals.