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Register a new userCoexistence of type-I and type-II superconductivity in topological superconductor PdTe$_2$
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The type-II Dirac semimetal PdTe2 was recently reported to be a type-I superconductor with a superconducting transition temperature Tc = 1.65 K. However, the recent results from tunneling and point contact spectroscopy suggested the unusual state of a mixture of type-I and type-II superconductivity. These contradictory results mean that there is no clear picture of the superconducting phase diagram and warrants a detailed investigation of the superconducting phase. We report here the muon spin rotation and relaxation ($mu$SR) measurements on the superconducting state of the topological Dirac semimetal PdTe2. From $mu$SR measurements, we find that PdTe2 exhibits mixed type-I/type-II superconductivity. Using these results a phase diagram has been determined. In contrast to previous results where local type-II superconductivity persists up to Hc2 = 600 G, we observed that bulk superconductivity is destroyed above 225 G.
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The transition metal dichalcogenide PdTe$_2$ was recently shown to be a unique system where a type II Dirac semimetallic phase and a superconducting phase co-exist. This observation has led to wide speculation on the possibility of the emergence of an unconventional topological superconducting phase in PdTe$_2$. Here, through direct measurement of the superconducting energy gap by scanning tunneling spectroscopy (STS), and temperature and magnetic field evolution of the same, we show that the superconducting phase in PdTe$_2$ is conventional in nature. The superconducting energy gap is measured to be 326 $mu$eV at 0.38 K and it follows a temperature dependence that is well described within the framework of Bardeen-Cooper-Schriefers (BCS) theory of conventional superconductivity. This is surprising because our quantum oscillation measurements confirm that at least one of the bands participating in transport has topologically non-trivial character.
Type I superconductivity has recently been reported for the Dirac semimetal PdTe$_2$ (Tc approximately 1.6K) with, remarkably, multiple critical fields and a complex phase diagram. Here, measurements of the specific heat utilizing a thermal relaxation technique are presented. Conventional weak-coupling BCS superconductivity is confirmed by examining the temperature dependence of the specific heat in zero field. By probing the latent heat accompanying the superconducting transition, thermodynamic evidence for type I superconductivity is attained. The presence of the intermediate state is observed as a significant broadening of the superconducting transition onto lower temperatures at high fields as well as irreversibility in the specific heat in zero field cooled data at 8.5 mT.
We report on the structure and physical properties of bulk Palladium Tellurium superconductor, which is synthesized via quartz vacuum encapsulation technique at 750 C. The as synthesized compound is crystallized in hexagonal crystal structure. Magnetization and Magneto-transport measurements provided the values of lower and upper critical field to be 250 and 1200 Gauss respectively at 2 Kelvin. The Coherence length and GL parameter are estimated from the experimentally determined upper and lower critical fields, which are 45 nm and 1.48 respectively. The jump in Cp(T) at Tc is found to be 1.33 and the Debye temperature and electronic specific heat constant are 203 Kelvin and 6.01mJ/mole-K2 respectively.
Superconductors usually display either type-I or type-II superconductivity and the coexistence of these two types in the same material, for example at different temperatures is rare in nature. We the employed muon spin rotation (muSR) technique to unveil the superconducting phase diagram of the dodecaboride ZrB12 and obtained clear evidence of both type-I and type-II characteristics. Most importantly, we found a region showing unusual behavior where the usually mutually exclusive muSR signatures of type-I and type-II superconductivity coexist. We reproduced that behavior in theoretical modeling that required taking into account multiple bands and multiple coherence lengths, which suggests that material has one coherence length larger and another smaller than the magnetic field penetration length (the type-1.5 regime). At stronger fields, a footprint of the type-II mixed state showing square flux-line lattice was also obtained using neutron diffraction.
The Dirac semimetal PdTe$_2$ was recently reported to be a type-I superconductor with $T_c = 1.64$ K and a critical field $mu_0H_c = 13.6$ mT. Since type-I superconductivity is unexpected for binary compounds, we have conducted muon spin rotation experiments to probe the superconducting phase on the microscopic scale via its intermediate state. For crystals with a finite demagnetization factor, $N$, the intermediate state forms in applied fields $(1-N)H_c < H_a < H_c$. We have carried out transverse field muon spin rotation measurements on a thin disk-like crystal with the field perpendicular to ($N_{perp}=0.86$) and in the plane ($N_{parallel}=0.08$) of the disk. By analysing the $mu$SR signal we find that the volume fraction of the normal domains grows quasi-linearly with applied field at the expense of the Meissner domain fraction. This then provides solid evidence for the intermediate state and type-I superconductivity in the bulk of PdTe$_2$.
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