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Register a new userA self-calibrating SI-traceable broadband Rydberg atom-based radio-frequency electric field probe and measurement instrument
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We present a self-calibrating, SI-traceable broadband Rydberg-atom-based radio-frequency (RF) electric field probe (the Rydberg Field Probe or RFP) and measurement instrument (Rydberg Field Measurement System or RFMS). The RFMS comprises an atomic RF field probe (RFP), connected by a ruggedized fiber-optic patch cord to a portable mainframe control unit with a software interface for RF measurement and analysis including real-time field readout and RF waveform visualization. The instrument employs electromagnetically induced transparency (EIT) readout of spectral signatures from RF-sensitive Rydberg states of an atomic vapor for continuous, pulsed, and modulated RF field measurement. The RFP exploits resonant and off-resonant Rydberg-field interactions to realize broadband RF measurements at frequencies ranging from ~10 MHz to sub-THz over a wide dynamic range. The RFMS incorporates an RF-field-free atomic reference and a laser-frequency tracker to ensure reliability and accuracy of the RF measurement. We characterize the RFP and measure polar field and polarization patterns of the RFP at 12.6 GHz RF in the far-field of a standard gain horn antenna. Measurements at 2.5 GHz are also performed. Measured patterns are in good agreement with simulations. A detailed calibration procedure and uncertainty analysis are presented that account for deviations from an isotropic response over a $4pi$ solid angle, arising from dielectric structures external to the atomic measurement volume. Contributions to the measurement uncertainty from the fundamental atomic measurement method and associated analysis as well as material, geometry, and hardware design choices are accounted for. A calibration (C) factor is used to establish absolute-standard SI-traceable calibration of the RFP. Pulsed and modulated RF field measurement, and time-domain RF-pulse waveform imaging are also demonstrated.
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In this work, we demonstrate the use of a Rydberg atom-based sensor for determining the angle-of-arrival of an incident radio-frequency (RF) wave or signal. The technique uses electromagnetically induced transparency in Rydberg atomic vapor in conjunction with a heterodyne Rydberg atom-based mixer. The Rydberg atom mixer measures the phase of the incident RF wave at two different locations inside an atomic vapor cell. The phase difference at these two locations is related to the direction of arrival of the incident RF wave. To demonstrate this approach, we measure phase differences of an incident 19.18 GHz wave at two locations inside a vapor cell filled with cesium atoms for various incident angles. Comparisons of these measurements to both full-wave simulation and to a plane-wave theoretical model show that these atom-based sub-wavelength phase measurements can be used to determine the angle-of-arrival of an RF field.
We demonstrate the use of multiple atomic-level Rydberg-atom schemes for continuous frequency detection of radio frequency (RF) fields. Resonant detection of RF fields by electromagnetically-induced transparency and Autler-Townes (AT) in Rydberg atoms is typically limited to frequencies within the narrow bandwidth of a Rydberg transition. By applying a second field resonant with an adjacent Rydberg transition, far-detuned fields can be detected through a two-photon resonance AT splitting. This two-photon AT splitting method is several orders of magnitude more sensitive than off-resonant detection using the Stark shift. We present the results of various experimental configurations and a theoretical analysis to illustrate the effectiveness of this multiple level scheme. These results show that this approach allows for the detection of frequencies in continuous band between resonances with adjacent Rydberg states.
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There is an increasing demand for precise molecular spectroscopy, in particular in the mid-infrared fingerprint window that hosts a considerable number of vibrational signatures, whether it be for modeling our atmosphere, interpreting astrophysical spectra or testing fundamental physics. We present a high-resolution mid-infrared spectrometer traceable to primary frequency standards. It combines a widely tunable ultra-narrow Quantum Cascade Laser (QCL), an optical frequency comb and a compact multipass cell. The QCL frequency is stabilized onto a comb controlled with a remote near-infrared ultra-stable laser, transferred through a fiber link. The resulting QCL frequency stability is below 10-15 from 0.1 to 10s and its frequency uncertainty of 4x10-14 is given by the remote frequency standards. Continuous tuning over ~400 MHz is reported. We use the apparatus to perform saturated absorption spectroscopy of methanol in the low-pressure multipass cell and demonstrate a statistical uncertainty at the kHz level on transition center frequencies, confirming its potential for driving the next generation technology required for precise spectroscopic measurements.
This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization technique demonstrates increased sensitivity for isotope separation and measurement of atomic parameters over non-resonant laser ionization methods. The setup was tested at the Collinear Resonance Ionization Spectroscopy experiment at ISOLDE-CERN to perform high-resolution measurements of transitions in the indium atom from the 5s$^2$5d~$^2$D$_{5/2}$ and 5s$^2$5d~$^2$D$_{3/2}$ states to 5s$^2$($n$)p~$^2$P and 5s$^2$($n$)f~$^2$F Rydberg states, up to a principal quantum number of $n$ = 72. The extracted Rydberg level energies were used to re-evaluate the ionization potential of the indium atom to be 46670.1055(21) cm$^{-1}$. The nuclear magnetic dipole and nuclear electric quadrupole hyperfine structure constants and level isotope shifts of the 5s$^2$5d~$^2$D$_{5/2}$ and 5s$^2$5d~$^2$D$_{3/2}$ states were determined for $^{113,115}$In. The results are compared to calculations using relativistic coupled-cluster theory. A good agreement is found with the ionization potential and isotope shifts, while disagreement of hyperfine structure constants indicates an increased importance of electron correlations in these excited atomic states. With the aim of further increasing the detection sensitivity for measurements on exotic isotopes, a systematic study of the field-ionization arrangement implemented in the work was performed and an improved design was simulated and is presented. The improved design offers increased background suppression independent of the distance from field ionization to ion detection.
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