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Dipole-phonon quantum logic with trapped polar molecular ions

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 Added by Eric Hudson
 Publication date 2019
  fields Physics
and research's language is English




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The interaction between the electric dipole moment of a trapped molecular ion and the configuration of the confined Coulomb crystal couples the orientation of the molecule to its motion. We consider the practical feasibility of harnessing this interaction to initialize, process, and read out quantum information encoded in molecular ion qubits without optically illuminating the molecules. We present two schemes wherein a molecular ion can be entangled with a co-trapped atomic ion qubit, providing, among other things, a means for molecular state preparation and measurement. We also show that virtual phonon exchange can significantly boost range of the intermolecular dipole-dipole interaction, allowing strong coupling between widely-separated molecular ion qubits.



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We present a quantum logic scheme to detect atomic and molecular ions in different states of angular momentum based on their magnetic $g$-factors. The state-dependent magnetic $g$-factors mean that electronic, rotational or hyperfine states may be distinguished by their Zeeman splittings in a given magnetic field. Driving motional sidebands of a chosen Zeeman splitting enables reading out the corresponding state of angular momentum with an auxillary logic ion. As a proof-of-principle demonstration, we show that we can detect the ground electronic state of a ${^{174}}$Yb$^+$ ion using ${^{171}}$Yb$^+$ as the logic ion. Further, we can distinguish between the ${^{174}}$Yb$^+$ ion being in its ground electronic state versus the metastable ${^{2}}D_{3/2}$ state. We discuss the suitability of this scheme for the detection of rotational states in molecular ions.
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Control over physical systems at the quantum level is a goal shared by scientists in fields as diverse as metrology, information processing, simulation and chemistry. For trapped atomic ions, the quantized motional and internal degrees of freedom can be coherently manipulated with laser light. Similar control is difficult to achieve with radio frequency or microwave radiation because the essential coupling between internal degrees of freedom and motion requires significant field changes over the extent of the atoms motion. The field gradients are negligible at these frequencies for freely propagating fields; however, stronger gradients can be generated in the near-field of microwave currents in structures smaller than the free-space wavelength. In the experiments reported here, we coherently manipulate the internal quantum states of the ions on time scales of 20 ns. We also generate entanglement between the internal degrees of freedom of two atoms with a gate operation suitable for general quantum computation. We implement both operations through the magnetic fields from microwave currents in electrodes that are integrated into the micro-fabricated trap structure and create an entangled state with fidelity 76(3) %. This approach, where the quantum control mechanism is integrated into the trapping device in a scalable manner, can potentially benefit quantum information processing, simulation and spectroscopy.
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