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Light with orbital angular momentum interacting with trapped ions

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 Publication date 2011
  fields Physics
and research's language is English




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We study the interaction of a light beams carrying angular momentum with a single, trapped and well localized ion. We provide a detailed calculation of selection rules and excitation probabilities for quadrupole transitions. The results show the dependencies on the angular momentum and polarization of the laser beam as well as the direction of the quantization magnetic field. In order to observe optimally the specific effects, focusing the angular momentum beam close to the diffraction limit is required. We discuss a protocol for examining experimentally the effects on the S$_{1/2}$ to D$_{5/2}$ transition using a $^{40}$Ca$^+$ ion. Various applications and advantages are expected when using light carrying angular momentum: In quantum information processing, where qubit states of ion crystals are controlled, parasitic light shifts could be avoided as the ion is excited in the dark zone of the beam at zero electric field amplitude. Such interactions also open the door to high dimensional entanglement between light and matter. In spectroscopy one might access transitions which have escaped excitation so far due to vanishing transition dipole moments.



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Recent progresses on quantum control of cold atoms and trapped ions in both the scientific and technological aspects greatly advance the applications in precision measurement. Thanks to the exceptional controllability and versatility of these massive quantum systems, unprecedented sensitivity has been achieved in clocks, magnetometers and interferometers based on cold atoms and ions. Besides, these systems also feature many characteristics that can be employed to facilitate the applications in different scenarios. In this review, we briefly introduce the principles of optical clocks, cold atom magnetometers and atom interferometers used for precision measurement of time, magnetic field, and inertial forces. The main content is then devoted to summarize some recent experimental and theoretical progresses in these three applications, with special attention being paid to the new designs and possibilities towards better performance. The purpose of this review is by no means to give a complete overview of all important works in this fast developing field, but to draw a rough sketch about the frontiers and show the fascinating future lying ahead.
The interaction between the electric dipole moment of a trapped molecular ion and the configuration of the confined Coulomb crystal couples the orientation of the molecule to its motion. We consider the practical feasibility of harnessing this interaction to initialize, process, and read out quantum information encoded in molecular ion qubits without optically illuminating the molecules. We present two schemes wherein a molecular ion can be entangled with a co-trapped atomic ion qubit, providing, among other things, a means for molecular state preparation and measurement. We also show that virtual phonon exchange can significantly boost range of the intermolecular dipole-dipole interaction, allowing strong coupling between widely-separated molecular ion qubits.
We present an optomechanical device designed to allow optical transduction of orbital angular momentum of light. An optically induced twist imparted on the device by light is detected using an integrated cavity optomechanical system based on a nanobeam slot-mode photonic crystal cavity. This device could allow measurement of the orbital angular momentum of light when photons are absorbed by the mechanical element, or detection of the presence of photons when they are scattered into new orbital angular momentum states by a sub-wavelength grating patterned on the device. Such a system allows detection of a $l = 1$ orbital angular momentum field with an average power of $3.9times10^3$ photons modulated at the mechanical resonance frequency of the device and can be extended to higher order orbital angular momentum states.
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Conical intersections between electronic potential energy surfaces are paradigmatic for the study of non-adiabatic processes in the excited states of large molecules. However, since the corresponding dynamics occurs on a femtosecond timescale, their investigation remains challenging and requires ultrafast spectroscopy techniques. We demonstrate that trapped Rydberg ions are a platform to engineer conical intersections and to simulate their ensuing dynamics on larger length and time scales of the order of nanometers and microseconds, respectively; all this in a highly controllable system. Here, the shape of the potential energy surfaces and the position of the conical intersection can be tuned thanks to the interplay between the high polarizability and the strong dipolar exchange interactions of Rydberg ions. We study how the presence of a conical intersection affects both the nuclear and electronic dynamics demonstrating, in particular, how it results in the inhibition of the nuclear motion. These effects can be monitored in real-time via a direct spectroscopic measurement of the electronic populations in a state-of-the-art experimental setup.
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