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Register a new userObservation of many-body dynamics of Rydberg atoms based on antiblockade using two-color excitation
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We investigate a long-range interaction between $64D_{5/2}$ Rydberg-atom pairs and antiblockade effect employing a two-color excitation scheme. The first color (pulse A) is set to resonantly excite the Rydberg transition and prepare a few seed atoms, which establish a blockade region due to strong long-range interaction between Rydberg-atom pairs. The second color (pulse B) is blue detuned relative to Rydberg transition and enables further Rydberg excitation of atoms by counteracting the blockade effect. It is found that a few seed atoms lead to a huge difference of the Rydberg excitation with pulse B. The dynamic evolution of antiblockade excitation by varying the pulse-B duration at 30-MHz blue detuning is also investigated. The evolution result reveals that a small amount of seed atoms can trigger an avalanche Rydberg excitation. A modified superatom model is used to simulate the antiblockade effect and relevant dynamic evolution. The simulations are consistent with the experimental measurements.
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We develop a theoretical approach for the dynamics of Rydberg excitations in ultracold gases, with a realistically large number of atoms. We rely on the reduction of the single-atom Bloch equations to rate equations, which is possible under various experimentally relevant conditions. Here, we explicitly refer to a two-step excitation-scheme. We discuss the conditions under which our approach is valid by comparing the results with the solution of the exact quantum master equation for two interacting atoms. Concerning the emergence of an excitation blockade in a Rydberg gas, our results are in qualitative agreement with experiment. Possible sources of quantitative discrepancy are carefully examined. Based on the two-step excitation scheme, we predict the occurrence of an antiblockade effect and propose possible ways to detect this excitation enhancement experimentally in an optical lattice as well as in the gas phase.
We investigate the excitation dynamics of Rydberg atoms in ultracold atomic samples by expanding the excitation probability and the correlation function between excited atoms in powers of the isolated atom Rabi frequency $Omega$. In the Heisenberg picture, we give recurrence relations to calculate any order of the expansions, which ere expected to be well-behaved for arbitrarily strong interactions. For homogeneous large samples, we give the explicit form of the expansions, up to $Omega^4$, averaged over all possible random spatial distributions of atoms, for the most important cases of excitation pulses and interactions.
The recent observation of high-lying Rydberg states of excitons in semiconductors with relatively high binding energy motivates exploring their applications in quantum nonlinear optics and quantum information processing. Here, we study Rydberg excitation dynamics of a mesoscopic array of excitons to demonstrate its application in simulation of quantum many-body dynamics. We show that the $mathbb{Z}_2$-ordered phase can be reached using physical parameters available for cuprous oxide (Cu$_2$O) by optimizing driving laser parameters such as duration, intensity, and frequency. In an example, we study the application of our proposed system to solving the Maximum Independent Set (MIS) problem based on the Rydberg blockade effect.
Interaction between Rydberg atoms can significantly modify Rydberg excitation dynamics. Under a resonant driving field the Rydberg-Rydberg interaction in high-lying states can induce shifts in the atomic resonance such that a secondary Rydberg excitation becomes unlikely leading to the Rydberg blockade effect. In a related effect, off-resonant coupling of light to Rydberg states of atoms contributes to the Rydberg anti-blockade effect where the Rydberg interaction creates a resonant condition that promotes a secondary excitation in a Rydberg atomic gas. Here, we study the light-matter interaction and dynamics of off-resonant two-photon excitations and include two- and three-atom Rydberg interactions and their effect on excited state dynamics in an ensemble of cold atoms. In an experimentally-motivated regime, we find the optimal physical parameters such as Rabi frequencies, two-photon detuning, and pump duration to achieve significant enhancement in the probability of generating doubly-excited collective atomic states. This results in large auto-correlation values due to the Rydberg anti-blockade effect and makes this system a potential candidate for a high-purity two-photon Fock state source.
In the last twenty years, Rydberg atoms have become a versatile and much studied system for implementing quantum many-body systems in the framework of quantum computation and quantum simulation. However, even in the absence of coherent evolution Rydberg systems exhibit interesting and non-trivial many-body phenomena such as kinetic constraints and non-equilibrium phase transitions that are relevant in a number of research fields. Here we review our recent work on such systems, where dissipation leads to incoherent dynamics and also to population decay. We show that those two effects, together with the strong interactions between Rydberg atoms, give rise to a number of intriguing phenomena that make cold Rydberg atoms an attractive test-bed for classical many-body processes and quantum generalizations thereof.
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