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Rejuvenation and Shear-Banding in model amorphous solids

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 Added by Sylvain Patinet Dr.
 Publication date 2019
  fields Physics
and research's language is English




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We measure the local yield stress, at the scale of small atomic regions, in a deeply quenched two-dimensional glass model undergoing shear banding in response to athermal quasistatic (AQS) deformation. We find that the occurrence of essentially a single plastic event suffices to bring the local yield stress distribution to a well-defined value for all strain orientations, thus essentially erasing the memory of the initial structure. It follows that in a well-relaxed sample, plastic events cause the abrupt (nucleation-like) emergence of a local softness contrast and thus precipitate the formation of a band, which, in its early stages, is measurably softer than the steady-state flow. Moreover, this postevent yield stress ensemble presents a mean value comparable to that of the inherent states of a supercooled liquid around the mode-coupling temperature $T_{rm MCT}$. This, we argue, explains that the transition between brittle and ductile yielding in amorphous materials occurs around a comparable parent temperature. Our data also permit to capture quantitatively the contributions of pressure and density changes and demonstrate unambiguously that they are negligible compared with the changes of softness caused by structural rejuvenation.

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Dynamic recrystallization (DRX) is often observed in conjunction with adiabatic shear banding (ASB) in polycrystalline materials. The recrystallized nanograins in the shear band have few dislocations compared to the material outside of the shear band. In this paper, we reformulate the recently-developed Langer-Bouchbinder-Lookman (LBL) continuum theory of polycrystalline plasticity and include the creation of grain boundaries. While the shear-banding instability emerges because thermal heating is faster than heat dissipation, recrystallization is interpreted as an entropic effect arising from the competition between dislocation creation and grain boundary formation. We show that our theory closely matches recent results in sheared ultrafine-grained titanium. The theory thus provides a thermodynamically consistent way to systematically describe the formation of shear bands and recrystallized grains therein.
We study the structural origin of the Bauschinger effect by accessing numerically the local plastic thresholds in the steady state flow of a two-dimensional model glass under athermal quasistatic deformation. More specifically, we compute the local residual strength, $Deltatau^{c}$, for arbitrary loading orientations and find that plastic deformation generically induces material polarization, i.e., a forward-backward asymmetry in the $Deltatau^{c}$ distribution. In steady plastic flow, local packings are on average closer to forward (rather than backward) instabilities, due to the stress-induced bias of barriers. However, presumably due to mechanical noise, a significant fraction of zones lie close to reverse (backward) yielding, as the distribution of $Deltatau^{c}$ for reverse shearing extends quasilinearly down to zero local residual strength. By constructing an elementary model of the early plastic response, we then show that unloading causes reverse plasticity of a growing amplitude, i.e., reverse softening, while it shifts away forward-yielding barriers. This result in an inversion of polarization in the low-$Deltatau^{c}$ region and, consequently, in the Bauschinger effect. This scenario is quite generic, which explains the pervasiveness of the effect.
Amorphous solids display a ductile to brittle transition as the kinetic stability of the quiescent glass is increased, which leads to a material failure controlled by the sudden emergence of a macroscopic shear band in quasi-static protocols. We numerically study how finite deformation rates influence ductile and brittle yielding behaviors using model glasses in two and three spatial dimensions. We find that a finite shear rate systematically enhances the stress overshoot of poorly-annealed systems, without necessarily producing shear bands. For well-annealed systems, the non-equilibrium discontinuous yielding transition is smeared out by finite shear rates and it is accompanied by the emergence of multiple shear bands that have been also reported in metallic glass experiments. We show that the typical size of the bands and the distance between them increases algebraically with the inverse shear rate. We provide a dynamic scaling argument for the corresponding lengthscale, based on the competition between the deformation rate and the propagation time of the shear bands.
We present an analytical study of a toy model for shear banding, without normal stresses, which uses a piecewise linear approximation to the flow curve (shear stress as a function of shear rate). This model exhibits multiple stationary states, one of which is linearly stable against general two-dimensional perturbations. This is in contrast to analogous results for the Johnson-Segalman model, which includes normal stresses, and which has been reported to be linearly unstable for general two-dimensional perturbations. This strongly suggests that the linear instabilities found in the Johnson-Segalman can be attributed to normal stress effects.
Amorphous solids increase their stress as a function of an applied strain until a mechanical yield point whereupon the stress cannot increase anymore, afterwards exhibiting a steady state with a constant mean stress. In stress controlled experiments the system simply breaks when pushed beyond this mean stress. The ubiquity of this phenomenon over a huge variety of amorphous solids calls for a generic theory that is free of microscopic details. Here we offer such a theory: the mechanical yield is a thermodynamic phase transition, where yield occurs as a spinodal phenomenon. At the spinodal point there exists a divergent correlation length which is associated with the system-spanning instabilities (known also as shear bands) which are typical to the mechanical yield. The theory, the order parameter used and the correlation functions which exhibit the divergent correlation length are universal in nature and can be applied to any amorphous solids that undergo mechanical yield.
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