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Brittle yielding of amorphous solids at finite shear rates

129   0   0.0 ( 0 )
 Added by Ludovic Berthier
 Publication date 2019
  fields Physics
and research's language is English




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Amorphous solids display a ductile to brittle transition as the kinetic stability of the quiescent glass is increased, which leads to a material failure controlled by the sudden emergence of a macroscopic shear band in quasi-static protocols. We numerically study how finite deformation rates influence ductile and brittle yielding behaviors using model glasses in two and three spatial dimensions. We find that a finite shear rate systematically enhances the stress overshoot of poorly-annealed systems, without necessarily producing shear bands. For well-annealed systems, the non-equilibrium discontinuous yielding transition is smeared out by finite shear rates and it is accompanied by the emergence of multiple shear bands that have been also reported in metallic glass experiments. We show that the typical size of the bands and the distance between them increases algebraically with the inverse shear rate. We provide a dynamic scaling argument for the corresponding lengthscale, based on the competition between the deformation rate and the propagation time of the shear bands.



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Amorphous solids increase their stress as a function of an applied strain until a mechanical yield point whereupon the stress cannot increase anymore, afterwards exhibiting a steady state with a constant mean stress. In stress controlled experiments the system simply breaks when pushed beyond this mean stress. The ubiquity of this phenomenon over a huge variety of amorphous solids calls for a generic theory that is free of microscopic details. Here we offer such a theory: the mechanical yield is a thermodynamic phase transition, where yield occurs as a spinodal phenomenon. At the spinodal point there exists a divergent correlation length which is associated with the system-spanning instabilities (known also as shear bands) which are typical to the mechanical yield. The theory, the order parameter used and the correlation functions which exhibit the divergent correlation length are universal in nature and can be applied to any amorphous solids that undergo mechanical yield.
Considering a recently proposed model for the yielding of amorphous solids under cyclic shear deformation, we show that it can be analyzed by mapping it, in the simplest case, to a random walk in a confining potential with an absorbing boundary. The dynamics is governed by the first passage time into the absorbing state, which captures the essential features of the original model, thereby providing insight into the observed robustness of earlier results. Including the possibility of activated escape from absorbing states leads to a unique determination of a threshold energy and yield strain, and further, suggests an appealing approach to understanding fatigue failure.
The holographic principle has proven successful in linking seemingly unrelated problems in physics; a famous example is the gauge-gravity duality. Recently, intriguing correspondences between the physics of soft matter and gravity are emerging, including strong similarities between the rheology of amorphous solids, effective field theories for elasticity and the physics of black holes. However, direct comparisons between theoretical predictions and experimental/simulation observations remain limited. Here, we study the effects of non-linear elasticity on the mechanical and thermodynamic properties of amorphous materials responding to shear, using effective field and gravitational theories. The predicted correlations among the non-linear elastic exponent, the yielding strain/stress and the entropy change due to shear are supported qualitatively by simulations of granular matter models. Our approach opens a path towards understanding complex mechanical responses of amorphous solids, such as mixed effects of shear softening and shear hardening, and offers the possibility to study the rheology of solid states and black holes in a unified framework.
130 - Srikanth Sastry 2020
Understanding the mechanical response and failure of solids is of obvious importance in their use as structural materials. The nature of plastic deformation leading to yielding of amorphous solids has been vigorously pursued in recent years. Investigations employing both unidirectional and cyclic deformation protocols reveal a strong dependence of yielding behaviour on the degree of annealing. Below a threshold degree of annealing, the nature of yielding changes qualitatively, to progressively more discontinuous yielding. Theoretical investigations of yielding in amorphous solids have almost exclusively focused on yielding under unidirectional deformation, but cyclic deformation reveals several interesting features that remain largely un-investigated. Focusing on athermal cyclic deformation, I investigate a family of models based on an energy landscape description. These models reproduce key interesting features observed in simulations, and provide an interpretation for the intriguing presence of a threshold energy.
It is known by now that amorphous solids at zero temperature do not possess a nonlinear elasticity theory: besides the shear modulus which exists, all the higher order coefficients do not exist in the thermodynamic limit. Here we show that the same phenomenon persists up to temperatures comparable to the glass transition. The zero temperature mechanism due to the prevalence of dangerous plastic modes of the Hessian matrix is replaced by anomalous stress fluctuations that lead to the divergence of the variances of the higher order elastic coefficients. The conclusion is that in amorphous solids elasticity can never be decoupled from plasticity: the nonlinear response is very substantially plastic.
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