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Register a new userA self referencing attosecond interferometer with zeptosecond precision
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In this work we demonstrate the generation of two intense, ultrafast laser pulses that allow a controlled interferometric measurement of higher harmonic generation pulses with 12.8 attoseconds in resolution (half the atomic unit of time) and a precision as low as 680 zeptoseconds ($10^{-21}$ seconds). We create two replicas of a driving femtosecond pulse which share the same optical path except at the focus where they converge to two foci. An attosecond pulse train emerges from each focus through the process of HHG. The two attosecond pulse trains from each focus interfere in the far field producing a clear interference pattern in the XUV region. By controlling the relative optical phase between the two driving laser pulses we are able to actively influence the delay between the pulses and are able to perform very stable and precise pump-probe experiments. Because of the phase operation occurs across the entire spatial profile we effectively create two indistinguishable intense laser pulses or a common path interferometer for attosecond pulses. Commonality across the two beams means that they are extremely stable to environmental and mechanical fluctuations up to a Rayleigh range from the focus. In our opinion this represents an ideal source for homodyne and heterodyne spectroscopic measurements with sub-attosecond precision.
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Photon exchange due to nuclear bremsstrahlung during nuclear collisions can cause Coulomb excitation in the projectile and the target nuclei. The corresponding process originated in nuclear timescales can also be observed in atomic phenomenon experimentally if it delayed by at least with an attosecond or longer timescales. We have found that this happens due to a mechanism involving the Eisenbud-Wigner-Smith time delay process. We have estimated photoionization time delays in atomic collisions utilizing the nonrelativistic version of random phase approximation with exchange and Hartree-Fock methods. We present three representative processes in which we can observe the phenomena in attosecond timescales even though they originate from excitations in the zeptosecond timescales. Thus the work represents an investigation of parallels between two neighboring areas of physics. Furthermore the present work suggests new possibilities for atomic physics research near the Coulomb barrier energy, where the laser is replaced by nuclear bremsstrahlung.
Photoionization is one of the fundamental light-matter interaction processes in which the absorption of a photon launches the escape of an electron. The time scale of the process poses many open questions. Experiments found time delays in the attosecond ($10^{-18}$ s) domain between electron ejection from different orbitals, electronic bands, or in different directions. Here, we demonstrate that across a molecular orbital the electron is not launched at the same time. The birth time rather depends on the travel time of the photon across the molecule, which is 247 zeptoseconds ($10^{-21}$ s) for the average bond length of H$_2$. Using an electron interferometric technique, we resolve this birth time delay between electron emission from the two centers of the hydrogen molecule.
We phase-coherently measure the frequency of continuous-wave (CW) laser light by use of optical-phase modulation and f-2f nonlinear interferometry. Periodic electro-optic modulation (EOM) transforms the CW laser into a continuous train of picosecond optical pulses. Subsequent nonlinear-fiber broadening of this EOM frequency comb produces a supercontinuum with 160 THz of bandwidth. A critical intermediate step is optical filtering of the EOM comb to reduce electronic-noise-induced decoherence of the supercontinuum. Applying f-2f self-referencing with the supercontinuum yields the carrier-envelope offset frequency of the EOM comb, which is precisely the difference of the CW laser frequency and an exact integer multiple of the EOM pulse repetition rate. Here we demonstrate absolute optical frequency metrology and synthesis applications of the self-referenced CW laser with <5E-14 fractional accuracy and stability.
We demonstrate an atom interferometer that uses a laser-cooled continuous beam of $^{87}$Rb atoms having velocities of 10--20 m/s. With spatially separated Raman beams to coherently manipulate the atomic wave packets, Mach--Zehnder interference fringes are observed at an interference distance of 2L = 19 mm. The apparatus operates within a small enclosed area of 0.07 mm$^2$ at a bandwidth of 190 Hz with a deduced sensitivity of $7.8times10^{-5}$ rad/s/$sqrt{{Hz}}$ for rotations. Using a low-velocity continuous atomic source in an atom interferometer enables high sampling rates and bandwidths without sacrificing sensitivity and compactness, which are important for applications in real dynamic environments.
The extreme miniaturization of a cold-atom interferometer accelerometer requires the development of novel technologies and architectures for the interferometer subsystems. We describe several component technologies and a laser system architecture to enable a path to such miniaturization. We developed a custom, compact titanium vacuum package containing a microfabricated grating chip for a tetrahedral grating magneto-optical trap (GMOT) using a single cooling beam. The vacuum package is integrated into the optomechanical design of a compact cold-atom sensor head with fixed optical components. In addition, a multichannel laser system driven by a single seed laser has been implemented with time-multiplexed frequency shifting using single sideband modulators, reducing the number of optical channels connected to the sensor head. This laser system architecture is compatible with a highly miniaturized photonic integrated circuit approach, and by demonstrating atom-interferometer operation with this laser system, we show feasibility for the integrated photonic approach. In the compact sensor head, sub-Doppler cooling in the GMOT produces 15 uK temperatures, which can operate at a 20 Hz data rate for the atom interferometer sequence. After validating atomic coherence with Ramsey interferometry, we demonstrate a light-pulse atom interferometer in a gravimeter configuration without vibration isolation for 10 Hz measurement cycle rate and T = 0 - 4.5 ms interrogation time, resulting in $Delta$g / g = 2.0e-6. All these efforts demonstrate progress towards deployable cold-atom inertial sensors under large amplitude motional dynamics.
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