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Register a new userPair-density-wave superconductivity of faces, edges and vertices in systems with imbalanced fermions
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We describe boundary effects in superconducting systems with Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconducting instability, using Bogoliubov-de-Gennes and Ginzburg-Landau (GL) formalisms. First, we show that in dimensions larger than one the standard GL functional formalism for FFLO superconductors is unbounded from below. This is demonstrated by finding solutions with zero Laplacian terms near boundaries. We generalize the GL formalism for these systems by retaining higher order terms. Next, we demonstrate that a cuboid sample of a superconductor with imbalanced fermions at a mean-field level has a sequence of the phase transitions. At low temperatures it forms Larkin-Ovchinnikov state in the bulk but has a different modulation pattern close to the boundaries. When temperature is increased the first phase transition occurs when the bulk of the material becomes normal while the faces remain superconducting. The second transition occurs at higher temperature where the system retains superconductivity on the edges. The third transition is associated with the loss of edge superconductivity while retaining superconducting gap in the vertices. We obtain the same sequence of phase transition by numerically solving the Bogoliubov-de Gennes model.
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We investigate in underdoped cuprates possible coexistence of the superconducting (SC) order at zero momentum and pair density wave (PDW) at momentum ${bf Q}=(pi, pi)$ in the presence of a Neel order. By symmetry, the $d$-wave uniform singlet pairing $dS_0$ can coexist with the $d$-wave triplet PDW $dT_{bf Q}$, and the $p$-wave singlet PDW $pS_{bf Q}$ can coexist with the $p$-wave uniform triplet $pT_0$. At half filling, we find the novel $pS_{bf Q}+pT_0$ state is energetically more favorable than the $dS_0+dT_{bf Q}$ state. At finite doping, however, the $dS_0+dT_{bf Q}$ state is more favorable. In both types of states, the variational triplet parameters, $dT_{bf Q}$ and $pT_0$, are of secondary significance. Our results point to a fully symmetric $mathrm{Z_2}$ quantum spin liquid with spinon Fermi surface in proximity to the Neel order at zero doping, and to intertwined $d$-wave triplet PDW fluctuations and spin moment fluctuations along with the dominant $d$-wave singlet SC at finite doping. The results are obtained by variational quantum Monte Carlo simulations.
The defining characteristic of hole-doped cuprates is $d$-wave high temperature superconductivity. However, intense theoretical interest is now focused on whether a pair density wave state (PDW) could coexist with cuprate superconductivity (D. F. Agterberg et al., Annual Review of Condensed Matter Physics 11, 231 (2020)). Here, we use a strong-coupling mean-field theory of cuprates, to model the atomic-scale electronic structure of an eight-unit-cell periodic, $d$-symmetry form factor, pair density wave (PDW) state coexisting with $d$-wave superconductivity (DSC). From this PDW+DSC model, the atomically-resolved density of Bogoliubov quasiparticle states N(r,E) is predicted at the terminal BiO surface of Bi$_2$Sr$_2$CaCu$_2$O$_8$ and compared with high-precision electronic visualization experiments using spectroscopic imaging STM. The PDW+DSC model predictions include the intra-unit-cell structure and periodic modulations of N(r,E), the modulations of the coherence peak energy $Delta_p$ (r), and the characteristics of Bogoliubov quasiparticle interference in scattering-wavevector space (q-space). Consistency between all these predictions and the corresponding experiments indicates that lightly hole-doped Bi$_2$Sr$_2$CaCu$_2$O$_8$ does contain a PDW+DSC state. Moreover, in the model the PDW+DSC state becomes unstable to a pure DSC state at a critical hole density p*, with empirically equivalent phenomena occurring in the experiments. All these results are consistent with a picture in which the cuprate translational symmetry breaking state is a PDW, the observed charge modulations are its consequence, the antinodal pseudogap is that of the PDW state, and the cuprate critical point at p* ~ 19% occurs due to disappearance of this PDW.
The recently discovered family of vanadium-based kagome metals with topological band structures offer a new opportunity to study frustrated, correlated and topological quantum states. These layered compounds are nonmagnetic and undergo charge density wave (CDW) transitions before developing superconductivity at low temperatures. Here we report the observation of unconventional superconductivity and pair density wave (PDW) in the vanadium-based kagome lattice CsV3Sb5 using scanning tunneling microscope/spectroscopy (STM/STS) and Josephson STS. The differential conductance exhibits a V-shaped pairing gap about 0.5 meV below a transition temperature Tc about 2.3 K. Superconducting phase coherence is observed by Josephson effect and Cooper-pair tunneling to a superconducting tip. We find that CsV3Sb5 is a strong-coupling superconductor (2delta/kBTc about 5) and coexists with 4a0 unidirectional and 2x2 charge order. Remarkably, we discover a 4a0/3 bidirectional PDW accompanied by spatial modulations of the coherence peak and gap-depth in the tunneling conductance. We term the latter as a roton-PDW that can produce a commensurate vortex-antivortex lattice to account for the observed conductance modulations. Above Tc, we observe long-range ordered 4a0 unidirectional and 2a0 bidirectional CDW and a large V-shaped pseudogap in the density of state. Electron-phonon calculations attribute the 2x2 CDW to phonon softening induced structural reconstruction, but the phonon mediated pairing cannot describe the observed strong-coupling superconductor. Our findings show that electron correlations in the charge sector can drive the 4a0 unidirectional CDW, unconventional superconductivity, and roton-PDW with striking analogies to the phenomenology of cuprate high-Tc superconductors, and provide the groundwork for understanding their microscopic origins in the vanadium-based kagome superconductors.
Interest in modulated paired states, long sought since the first proposals by Fulde and Ferrell and by Larkin and Ovchinnikov, has grown recently in the context of strongly coupled superconductors under the name of pair density wave. However, there is little theoretical understanding of how such a state might arise out of strong coupling physics in simple models. Although density matrix renormalization group has been a powerful tool for exploring strong coupling modulation phenomena of spin and charge stripe in the Hubbard model and the t-J model, there has been no numerical evidence of PDW within these models using DMRG. Here we note that a system with inversion breaking, C3v point group symmetry may host a PDW-like state. Motivated by the fact that spin-valley locked band structure of hole-doped group VI transition metal dichalcogenides materializes such a setting, we use DMRG to study the superconducting tendencies in spin-valley locked systems with strong short-ranged repulsion. Remarkably we find robust evidence for a PDW and the first of such evidence within DMRG studies of a simple fermionic model.
Pair density wave superconductivity constitutes a novel electronic condensate proposed to be realized in certain unconventional superconductors. Establishing its potential existence is important for our fundamental understanding of superconductivity in correlated materials. Here we compute the dynamical magnetic susceptibility in the presence of a pair density wave ordered state, and study its fingerprints on the spin-wave spectrum including the neutron resonance. In contrast to the standard case of d-wave superconductivity, we show that the pair density wave phase exhibits neither a spin-gap nor a magnetic resonance peak, in agreement with a recent neutron scattering experiment on underdoped La$_{1.905}$Ba$_{0.095}$CuO$_4$ [Z. Xu et al., Phys. Rev. Lett. 113, 177002 (2014)].
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