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Register a new userDecoherence of dipolar spin ensembles in diamond
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We present a combined theoretical and experimental study of solid-state spin decoherence in an electronic spin bath, focusing specifically on ensembles of nitrogen vacancy (NV) color centers in diamond and the associated substitutional nitrogen spin bath. We perform measurements of NV spin free induction decay times $T_2^*$ and spin-echo coherence times $T_2$ in 25 diamond samples with nitrogen concentrations [N] ranging from 0.01 to 300,ppm. We introduce a microscopic model and perform numerical simulations to quantitatively explain the degradation of both $T_2^*$ and $T_2$ over four orders of magnitude in [N]. Our results resolve a long-standing discrepancy observed in NV $T_2$ experiments, enabling us to describe NV ensemble spin coherence decay shapes as emerging consistently from the contribution of many individual NV.
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We consider an ensemble of atoms with $Lambda$-type level structure trapped in a single-mode cavity, and propose a geometric scheme of coherent manipulation of quantum states on the subspace of zero-energy states within the quantum Zeno subspace of the system. We find that the particular subspace inherits the decoherence-free nature of the quantum Zeno subspace and features a symmetry-protected degeneracy, fulfilling all the conditions for a universal scheme of arbitrary unitary operations on it.
We demonstrate that CPMG and XYXY decoupling sequences with non-ideal $pi$ pulses can reduce dipolar interactions between spins of the same species in solids. Our simulations of pulsed electron spin resonance (ESR) experiments show that $pi$ rotations with small ($<$~10%) imperfections refocus instantaneous diffusion. Here, the intractable N-body problem of interacting dipoles is approximated by the average evolution of a single spin in a changing mean field. These calculations agree well with experiments and do not require powerful hardware. Our results add to past attempts to explain similar phenomena in solid state nuclear magnetic resonance (NMR). Although the fundamental physics of NMR are similar to ESR, the larger linewidths in ESR and stronger dipolar interactions between electron spins compared to nuclear spins preclude drawing conclusions from NMR studies alone. For bulk spins, we also find that using XYXY results in less inflation of the deduced echo decay times as compared to decays obtained with CPMG.
We present an experimental and theoretical study of electronic spin decoherence in ensembles of nitrogen-vacancy (NV) color centers in bulk high-purity diamond at room temperature. Under appropriate conditions, we find ensemble NV spin coherence times (T_2) comparable to that of single NVs, with T_2 > 600 microseconds for a sample with natural abundance of 13C and paramagnetic impurity density ~10^15 cm^(-3). We also observe a sharp decrease of the coherence time with misalignment of the static magnetic field relative to the NV electronic spin axis, consistent with theoretical modeling of NV coupling to a 13C nuclear spin bath. The long coherence times and increased signal-to-noise provided by room-temperature NV ensembles will aid many applications of NV centers in precision magnetometry and quantum information.
We experimentally study the spin dynamics of mesoscopic ensembles of ultracold magnetic spin-3 atoms located in two separated wells of an optical dipole trap. We use a radio-frequency sweep to selectively flip the spin of the atoms in one of the wells, which produces two separated spin domains of opposite polarization. We observe that these engineered spin domains are metastable with respect to the long-range magnetic dipolar interactions between the two ensembles. The absence of inter-cloud dipolar spin-exchange processes reveals a classical behavior, in contrast to previous results with atoms loaded in an optical lattice. When we merge the two subsystems, we observe spin-exchange dynamics due to contact interactions which enable the first determination of the s-wave scattering length of 52Cr atoms in the S=0 molecular channel a_0=13.5^{+11}_{-10.5}a_B (where a_B is the Bohr radius).
Entanglement measures quantify nonclassical correlations present in a quantum system, but can be extremely difficult to calculate, even more so, when information on its state is limited. Here, we consider broad families of entanglement criteria that are based on variances of arbitrary operators and analytically derive the lower bounds these criteria provide for two relevant entanglement measures: the best separable approximation (BSA) and the generalized robustness (GR). This yields a practical method for quantifying entanglement in realistic experimental situations, in particular, when only few measurements of simple observables are available. As a concrete application of this method, we quantify bipartite and multipartite entanglement in spin-squeezed Bose-Einstein condensates of $sim 500$ atoms, by lower bounding the BSA and the GR only from measurements of first and second moments of the collective spin operator.
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