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Entanglement measures quantify nonclassical correlations present in a quantum system, but can be extremely difficult to calculate, even more so, when information on its state is limited. Here, we consider broad families of entanglement criteria that are based on variances of arbitrary operators and analytically derive the lower bounds these criteria provide for two relevant entanglement measures: the best separable approximation (BSA) and the generalized robustness (GR). This yields a practical method for quantifying entanglement in realistic experimental situations, in particular, when only few measurements of simple observables are available. As a concrete application of this method, we quantify bipartite and multipartite entanglement in spin-squeezed Bose-Einstein condensates of $sim 500$ atoms, by lower bounding the BSA and the GR only from measurements of first and second moments of the collective spin operator.
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We create a multi-partite entangled state by storing a single photon in a crystal that contains many large atomic ensembles with distinct resonance frequencies. The photon is re-emitted at a well-defined time due to an interference effect analogous to multi-slit diffraction. We derive a lower bound for the number of entangled ensembles based on the contrast of the interference and the single-photon character of the input, and we experimentally demonstrate entanglement between over two hundred ensembles, each containing a billion atoms. In addition, we illustrate the fact that each individual ensemble contains further entanglement. Our results are the first demonstration of entanglement between many macroscopic systems in a solid and open the door to creating even more complex entangled states.
We investigate the collective scattering of coherent light from a thermal alkali-metal vapor with temperatures ranging from 350 to 450 K, corresponding to average atomic spacings between $0.7 lambda$ and $0.1 lambda$. We develop a theoretical model treating the atomic ensemble as coherent, interacting, radiating dipoles. We show that the two-time second-order correlation function of a thermal ensemble can be described by an average of randomly positioned atomic pairs. Our model illustrates good agreement with the experimental results. Furthermore, we show how fine-tuning of the experimental parameters may make it possible to explore several photon statistics regimes.
We consider an ensemble of atoms with $Lambda$-type level structure trapped in a single-mode cavity, and propose a geometric scheme of coherent manipulation of quantum states on the subspace of zero-energy states within the quantum Zeno subspace of the system. We find that the particular subspace inherits the decoherence-free nature of the quantum Zeno subspace and features a symmetry-protected degeneracy, fulfilling all the conditions for a universal scheme of arbitrary unitary operations on it.
State-of-the-art atomic clocks are based on the precise detection of the energy difference between two atomic levels, measured as a quantum phase accumulated in a given time interval. Optical-lattice clocks (OLCs) now operate at or near the standard quantum limit (SQL) that arises from the quantum noise associated with discrete measurement outcomes. While performance beyond the SQL has been achieved in microwave clocks and other atomic sensors by engineering quantum correlations (entanglement) between the atoms, the generation of entanglement on an optical-clock transition and operation of such a clock beyond the SQL represent major goals in quantum metrology that have never been demonstrated. Here we report creation of a many-atom entangled state on an optical transition, and demonstrate an OLC with an Allan deviation below the SQL. We report a metrological gain of $4.4^{+0.6}_{-0.4}$ dB over the SQL using an ensemble consisting of a few hundred 171Yb atoms, allowing us to reach a given stability $2.8{pm}0.3$ times faster than the same clock operated at the SQL. Our results should be readily applicable to other systems, thus enabling further advances in timekeeping precision and accuracy. Entanglement-enhanced OLCs will have many scientific and technological applications, including precision tests of the fundamental laws of physics, geodesy, or gravitational wave detection.
We study numerically the slow (subradiant) decay of the fluorescence of motionless atoms after a weak pulsed excitation. We show that, in the linear-optics regime and for an excitation detuned by several natural linewidths, the slow decay rate can be dominated by close pairs of atoms (dimers) forming superradiant and subradiant states. However, for a large-enough resonant optical depth and at later time, the dynamics is dominated by collective many-body effects. In this regime, we study the polarization and the spectrum of the emitted light, as well as the spatial distribution of excitation inside the sample, as a function of time during the decay dynamics. The behavior of these observables is consistent with what would be expected for radiation trapping of nearly resonant light. This finding sheds light on subradiance in dilute samples by providing an interpretation based on the light behavior of the system (multiple scattering) which is complementary to the more commonly used picture of the collective atomic Dicke state.
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