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Plutos atmospheric haze settles out rapidly compared with geological timescales. It needs to be accounted for as a surface material, distinct from Plutos icy bedrock and from the volatile ices that migrate via sublimation and condensation on seasonal timescales. This paper explores how a steady supply of atmospheric haze might affect three distinct provinces on Pluto. We pose the question of why they each look so different from one another if the same haze material is settling out onto all of them. Cthulhu is a more ancient region with comparatively little present-day geological activity, where the haze appears to simply accumulate over time. Sputnik Planitia is a very active region where glacial convection, as well as sublimation and condensation rapidly refresh the surface, hiding recently deposited haze from view. Lowell Regio is a region of intermediate age featuring very distinct coloration from the rest of Pluto. Using a simple model haze particle as a colorant, we are not able to match the colors in both Lowell Regio and Cthulhu. To account for their distinct colors, we propose that after arrival at Plutos surface, haze particles may be less inert than might be supposed from the low surface temperatures. They must either interact with local materials and environments to produce distinct products in different regions, or else the supply of haze must be non-uniform in time and/or location, such that different products are delivered to different places.
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Haze in Plutos atmosphere was detected in images by both the Long Range Reconnaissance Imager (LORRI) and the Multispectral Visible Imaging Camera (MVIC) on New Horizons. LORRI observed haze up to altitudes of at least 200 km above Plutos surface at solar phase angles from ~20{deg} to ~169{deg}. The haze is structured with about ~20 layers, and the extinction due to haze is greater in the northern hemisphere than at equatorial or southern latitudes. However, more haze layers are discerned at equatorial latitudes. A search for temporal variations found no evidence for motions of haze layers (temporal changes in layer altitudes) on time scales of 2 to 5 hours, but did find evidence of changes in haze scale height above 100 km altitude. An ultraviolet extinction attributable to the atmospheric haze was also detected by the ALICE ultraviolet spectrograph on New Horizons. The haze particles are strongly forward-scattering in the visible, and a microphysical model of haze is presented which reproduces the visible phase function just above the surface with 0.5 {mu}m spherical particles, but also invokes fractal aggregate particles to fit the visible phase function at 45 km altitude and account for UV extinction. A model of haze layer generation by orographic excitation of gravity waves is presented. This model accounts for the observed layer thickness and distribution with altitude. Haze particles settle out of the atmosphere and onto Plutos surface, at a rate sufficient to alter surface optical properties on seasonal time scales. Plutos regional scale albedo contrasts may be preserved in the face of the haze deposition by atmospheric collapse.
Pluto has a heterogeneous surface, despite a global haze deposition rate of ~1 micrometer per orbit (Cheng et al., 2017; Grundy et al., 2018). While there could be spatial variation in the deposition rate, this has not yet been rigorously quantified, and naively the haze should coat the surface more uniformly than was observed. One way (among many) to explain this contradiction is for atmospheric pressure at the surface to drop low enough to interrupt haze production and stop the deposition of particles onto part of the surface, driving heterogeneity. If the surface pressure drops to less than 10^-3 - 10^-4 microbar and the CH4 mixing ratio remains nearly constant at the observed 2015 value, the atmosphere becomes transparent to ultraviolet radiation (Young et al., 2018), which would shut off haze production at its source. If the surface pressure falls below 0.06 microbar, the atmosphere ceases to be global, and instead is localized over only the warmest part of the surface, restricting the location of deposition (Spencer et al., 1997). In Plutos current atmosphere, haze monomers collect together into aggregate particles at beginning at 0.5 microbar; if the surface pressure falls below this limit, the appearance of particles deposited at different times of year and in different locations could be different. We use VT3D, an energy balance model (Young, 2017), to model the surface pressure on Pluto in current and past orbital configurations for four possible static N2 ice distributions: the observed northern hemisphere distribution with (1) a bare southern hemisphere, (2) a south polar cap, (3) a southern zonal band, and finally (4) a distribution that is bare everywhere except inside the boundary of Sputnik Planitia. We also present a sensitivity study showing the effect of mobile N2 ice...(cont.)
The New Horizons flyby of Pluto confirmed the existence of hazes in its atmosphere. Observations of a large high- to low- phase brightness ratio, combined with the blue color of the haze, suggest that the haze particles are fractal aggregates, analogous to the photochemical hazes on Titan. Therefore, studying the Pluto hazes can shed light on the similarities and differences between the Pluto and Titan atmospheres. We model the haze distribution using the Community Aerosol and Radiation Model for Atmospheres assuming that the distribution is shaped by sedimentation and coagulation of particles originating from photochemistry. Hazes composed of both purely spherical and purely fractal aggregate particles are considered. Agreement between model results and occultation observations is obtained with aggregate particles when the downward flux of photochemical products is equal to the column-integrated methane destruction rate ~1.2 $times$ 10$^{-14}$ g cm$^{-2}$ s$^{-1}$, while for spherical particles the mass flux must be 2-3 times greater. This flux is nearly identical to the haze production flux of Titan previously obtained by comparing microphysical model results to Cassini observations. The aggregate particle radius is sensitive to particle charging, and a particle charge to radius ratio of 30 e-/{mu}m is necessary to produce ~0.1-0.2 {mu}m aggregates near Plutos surface, in accordance with forward scattering measurements. Such a particle charge to radius ratio is 2-4 times higher than those previously obtained for Titan. Hazes composed of spheres with the same particle charge to radius ratio have particles that are 4 times smaller. These results further suggest that the haze particles are fractal aggregates. We also consider the effect of condensation of HCN, and C$_{2}$-hydrocarbons on the haze particles, which may play an important role in shaping their distributions.
During the New Horizons spacecrafts encounter with Pluto, the Alice ultraviolet spectrograph conducted a series of observations that detected emissions from both the interplanetary medium (IPM) and Pluto. In the direction of Pluto, the IPM was found to be 133.4$pm$0.6R at Lyman $alpha$, 0.24$pm$0.02R at Lyman $beta$, and <0.10R at He I 584{AA}. We analyzed 3,900s of data obtained shortly before closest approach to Pluto and detect airglow emissions from H I, N I, N II, N$_2$, and CO above the disk of Pluto. We find Plutos brightness at Lyman $alpha$ to be $29.3pm1.9$R, in good agreement with pre-encounter estimates. The detection of the N II multiplet at 1085{AA} marks the first direct detection of ions in Plutos atmosphere. We do not detect any emissions from noble gasses and place a 3$sigma$ upper limit of 0.14 R on the brightness of the Ar I 1048{AA} line. We compare pre-encounter model predictions and predictions from our own airglow model, based on atmospheric profiles derived from the solar occultation observed by New Horizons, to the observed brightness of Plutos airglow. Although completely opaque at Lyman $alpha$, Plutos atmosphere is optically thin at wavelengths longer than 1425{AA}. Consequently, a significant amount of solar FUV light reaches the surface, where it can participate in space weathering processes. From the brightness of sunlight reflected from Pluto, we find the surface has a reflectance factor (I/F) of 17% between 1400-1850{AA}. We also report the first detection of an C$_3$ hydrocarbon molecule, methylacetylene, in absorption, at a column density of ~5$times10^{15}$ cm$^{-2}$, corresponding to a column-integrated mixing ratio of $1.6times10^{-6}$.
Early Earth may have hosted a biologically-mediated global organic haze during the Archean eon (3.8-2.5 billion years ago). This haze would have significantly impacted multiple aspects of our planet, including its potential for habitability and its spectral appearance. Here, we model worlds with Archean-like levels of carbon dioxide orbiting the ancient sun and an M4V dwarf (GJ 876) and show that organic haze formation requires methane fluxes consistent with estimated Earth-like biological production rates. On planets with high fluxes of biogenic organic sulfur gases (CS2, OCS, CH3SH, and CH3SCH3), photochemistry involving these gases can drive haze formation at lower CH4/CO2 ratios than methane photochemistry alone. For a planet orbiting the sun, at 30x the modern organic sulfur gas flux, haze forms at a CH4/CO2 ratio 20% lower than at 1x the modern organic sulfur flux. For a planet orbiting the M4V star, the impact of organic sulfur gases is more pronounced: at 1x the modern Earth organic sulfur flux, a substantial haze forms at CH4/CO2 ~ 0.2, but at 30x the organic sulfur flux, the CH4/CO2 ratio needed to form haze decreases by a full order of magnitude. Detection of haze at an anomalously low CH4/CO2 ratio could suggest the influence of these biogenic sulfur gases, and therefore imply biological activity on an exoplanet. When these organic sulfur gases are not readily detectable in the spectrum of an Earth-like exoplanet, the thick organic haze they can help produce creates a very strong absorption feature at UV-blue wavelengths detectable in reflected light at a spectral resolution as low as 10. In direct imaging, constraining CH4 and CO2 concentrations will require higher spectral resolution, and R > 170 is needed to accurately resolve the structure of the CO2 feature at 1.57 {mu}m, likely, the most accessible CO2 feature on an Archean-like exoplanet.
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