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Register a new userShape staggering of mid-shell mercury isotopes from in-source laser spectroscopy compared with Density Functional Theory and Monte Carlo Shell Model calculations
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Neutron-deficient $^{177-185}$Hg isotopes were studied using in-source laser resonance-ionization spectroscopy at the CERN-ISOLDE radioactive ion-beam facility, in an experiment combining different detection methods tailored to the studied isotopes. These include either alpha-decay tagging or Multi-reflection Time-of-Flight gating to identify the isotopes of interest. The endpoint of the odd-even nuclear shape staggering in mercury was observed directly by measuring for the first time the isotope shifts and hyperfine structures of $^{177-180}$Hg. Changes in the mean-square charge radii for all mentioned isotopes, magnetic dipole and electric quadrupole moments of the odd-A isotopes and arguments in favor of $I = 7/2$ spin assignment for $^{177,179}$Hg were deduced. Experimental results are compared with Density Functional Theory (DFT) and Monte-Carlo Shell Model (MCSM) calculations. DFT calculations with several Skyrme parameterizations predict a large jump in the charge radius around the neutron $N = 104$ mid shell, with an odd-even staggering pattern related to the coexistence of nearly-degenerate oblate and prolate minima. This near-degeneracy is highly sensitive to many aspects of the effective interaction, a fact that renders perfect agreement with experiment out of reach for current functionals. Despite this inherent diffculty, the SLy5s1 and a modified UNEDF1^{SO} parameterization predict a qualitatively correct staggering that is off by two neutron numbers. MCSM calculations of states with the experimental spins and parities show good agreement for both electromagnetic moments and the observed charge radii. A clear mechanism for the origin of shape staggering within this context is identified: a substantial change in occupancy of the proton $pi h_{9/2}$ and neutron $ u i_{13/2}$ orbitals.
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The mean-square charge radii of $^{207,208}$Hg ($Z=80, N=127,128$) have been studied for the first time and those of $^{202,203,206}$Hg ($N=122,123,126$) remeasured by the application of in-source resonance-ionization laser spectroscopy at ISOLDE (CERN). The characteristic textit{kink} in the charge radii at the $N=126$ neutron shell closure has been revealed, providing the first information on its behavior below the $Z=82$ proton shell closure. A theoretical analysis has been performed within relativistic Hartree-Bogoliubov and non-relativistic Hartree-Fock-Bogoliubov approaches, considering both the new mercury results and existing lead data. Contrary to previous interpretations, it is demonstrated that both the kink at $N=126$ and the odd-even staggering (OES) in its vicinity can be described predominately at the mean-field level, and that pairing does not need to play a crucial role in their origin. A new OES mechanism is suggested, related to the staggering in the occupation of the different neutron orbitals in odd- and even-$A$ nuclei, facilitated by particle-vibration coupling for odd-$A$ nuclei.
item[Background] Ground-state spins and magnetic moments are sensitive to the nuclear wave function, thus they are powerful probes to study the nuclear structure of isotopes far from stability. item[Purpose] Extend our knowledge about the evolution of the $1/2^+$ and $3/2^+$ states for K isotopes beyond the $N = 28$ shell gap. item[Method] High-resolution collinear laser spectroscopy on bunched atomic beams. item[Results] From measured hyperfine structure spectra of K isotopes, nuclear spins and magnetic moments of the ground states were obtained for isotopes from $N = 19$ up to $N = 32$. In order to draw conclusions about the composition of the wave functions and the occupation of the levels, the experimental data were compared to shell-model calculations using SDPF-NR and SDPF-U effective interactions. In addition, a detailed discussion about the evolution of the gap between proton $1d_{3/2}$ and $2s_{1/2}$ in the shell model and {it{ab initio}} framework is also presented. item[Conclusions] The dominant component of the wave function for the odd-$A$ isotopes up to $^{45}$K is a $pi 1d_{3/2}^{-1}$ hole. For $^{47,49}$K, the main component originates from a $pi 2s_{1/2}^{-1}$ hole configuration and it inverts back to the $pi 1d_{3/2}^{-1}$ in $^{51}$K. For all even-$A$ isotopes, the dominant configuration arises from a $pi 1d_{3/2}^{-1}$ hole coupled to a neutron in the $ u 1f_{7/2}$ or $ u 2p_{3/2}$ orbitals. Only for $^{48}$K, a significant amount of mixing with $pi 2s_{1/2}^{-1} otimes u (pf)$ is observed leading to a $I^{pi}=1^{-}$ ground state. For $^{50}$K, the ground-state spin-parity is $0^-$ with leading configuration $pi 1d_{3/2}^{-1} otimes u 2p_{3/2}^{-1}$.
In the present work we have reported comprehensive analysis of recently available experimental data [H.M. David et al., Phys. Lett. B {bf 726}, 665 (2013)] for high-spin states up to $17^+$ with $T=0$ in the odd-odd $N=Z$ nucleus $^{62}$Ga using shell model calculations within the full $f_{5/2}pg_{9/2}$ model space and deformed shell model based on Hartee-Fock intrinsic states in the same space. The calculations have been performed using jj44b effective interaction developed recently by B.A. Brown and A.F. Lisetskiy for this model space. The results obtained with the two models are similar and they are in reasonable agreement with experimental data. In addition to the $T=0$ and $T=1$ energy bands, band crossings and electromagnetic transition probabilities, we have also calculated the pairing energy in shell model and all these compare well with the available theoretical results.
A set of global optical potential parameters, DA1p, for deuterons with the $1p$-shell nuclei is obtained by simultaneously fitting 67 sets of experimental data of deuteron elastic scattering from uc{6}{Li}, uc{9}{Be}, uc{10}{B}, uc{11}{B}, uc{12}{C}, uc{13}{C}, uc{14}{N}, uc{16}{O} and uc{18}{O} with incident energies between 5.25 and 170 MeV. DA1p improves the description of the deuteron elastic scattering from the $1p$-shell nuclei with respect to the existing systematic deuteron potentials and can give satisfactory reproduction to the experimental data with radiative nuclei such as uc{9}{Li}, uc{10}{Be}, uc{14}{C} and uc{14}{O}.
The shapes of neutron-rich exotic Ni isotopes are studied. Large-scale shell model calculations are performed by advanced Monte Carlo Shell Model (MCSM) for the $pf$-$g_{9/2}$-$d_{5/2}$ model space. Experimental energy levels are reproduced well by a single fixed Hamiltonian. Intrinsic shapes are analyzed for MCSM eigenstates. Intriguing interplays among spherical, oblate, prolate and gamma-unstable shapes are seen including shape fluctuations, $E$(5)-like situation, the magicity of doubly-magic $^{56,68,78}$Ni, and the coexistence of spherical and strongly deformed shapes. Regarding the last point, strong deformation and change of shell structure can take place simultaneously, being driven by the combination of the tensor force and changes of major configurations within the same nucleus.
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