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Quantum Interference Theory of Magnetoresistance in Dirac Materials

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 Added by Fu Bo
 Publication date 2019
  fields Physics
and research's language is English




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Magnetoresistance in many samples of Dirac semimetal and topological insulator displays non-monotonic behaviors over a wide range of magnetic field. Here a formula of magnetoconductivity is presented for massless and massive Dirac fermions in Dirac materials due to quantum interference in scalar impurity scattering potentials. It reveals a striking crossover from positive to negative magnetoresistivity, uncovering strong competition between weak localization and weak antilocalization in multiple Cooperon modes at different chemical potentials, effective masses and finite temperatures. The work sheds light on the important role of strong coupling of the conduction and valence bands in the quantum interference transport in topological nontrivial and trivial Dirac materials.



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Exotic electronic states are realized in novel quantum materials. This field is revolutionized by the topological classification of materials. Such compounds necessarily host unique states on their boundaries. Scanning tunneling microscopy studies of these surface states have provided a wealth of spectroscopic characterization, with the successful cooperation of ab initio calculations. The method of quasiparticle interference imaging proves to be particularly useful for probing the dispersion relation of the surface bands. Herein, how a variety of additional fundamental electronic properties can be probed via this method is reviewed. It is demonstrated how quasiparticle interference measurements entail mesoscopic size quantization and the electronic phase coherence in semiconducting nanowires; helical spin protection and energy-momentum fluctuations in a topological insulator; and the structure of the Bloch wave function and the relative insusceptibility of topological electronic states to surface potential in a topological Weyl semimetal.
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Massive Dirac fermions break the chiral symmetry explicitly and also make the Berry curvature of the band structure non-Abelian. By utilizing the Greens function technique, we develop a microscopic theory to establish a set of quantum diffusive equations for massive Dirac materials in the presence of electric and magnetic fields. It is found that the longitudinal magnetoresistance is always negative and quadratic in the magnetic field, and decays quickly with the mass. The theory is applicable to the systems with non-Abelian Berry curvature and resolves the puzzles of anomalous magnetotransport properties measured in topological materials.
Quantum anomalous Hall (QAH) effect appears in ferromagnetic topological insulators (FMTI) when a Dirac mass gap opens in the spectrum of the topological surface states (SS). Unaccountably, although the mean mass gap can exceed 28 meV (or ~320 K), the QAH effect is frequently only detectable at temperatures below 1 K. Using atomic-resolution Landau level spectroscopic imaging, we compare the electronic structure of the archetypal FMTI Cr_0.08(Bi_0.1Sb_0.9)_1.92Te_3 to that of its non-magnetic parent (Bi_0.1Sb_0.9)_2Te_3, to explore the cause. In (Bi_0.1Sb_0.9)_2Te_3, we find spatially random variations of the Dirac energy. Statistically equivalent Dirac energy variations are detected in Cr_0.08(Bi_0.1Sb_0.9)_1.92Te_3 with concurrent but uncorrelated Dirac mass gap disorder. These two classes of SS electronic disorder conspire to drastically suppress the minimum mass gap to below 100 {mu}eV for nanoscale regions separated by <1 {mu}m. This fundamentally limits the fully quantized anomalous Hall effect in Sb_2Te_3-based FMTI materials to very low temperatures.
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Electrons in low-temperature solids are governed by the non-relativistic Schr$ddot{o}$dinger equation, since the electron velocities are much slower than the speed of light. Remarkably, the low-energy quasi-particles given by electrons in various materials can behave as relativistic Dirac/Weyl fermions that obey the relativistic Dirac/Weyl equation. We refer to these materials as Dirac/Weyl materials, which provide a tunable platform to test relativistic quantum phenomena in table-top experiments. More interestingly, different types of physical fields in these Weyl/Dirac materials, such as magnetic fluctuations, lattice vibration, strain, and material inhomogeneity, can couple to the relativistic quasi-particles in a similar way as the $U(1)$ gauge coupling. As these fields do not have gauge-invariant dynamics in general, we refer to them as pseudo-gauge fields. In this chapter, we overview the concept and physical consequences of pseudo-gauge fields in Weyl/Dirac materials. In particular, we will demonstrate that pseudo-gauge fields can provide a unified understanding of a variety of physical phenomena, including chiral zero modes inside a magnetic vortex core of magnetic Weyl semimetals, a giant current response at magnetic resonance in magnetic topological insulators, and piezo-electromagnetic response in time-reversal invariant systems. These phenomena are deeply related to various concepts in high-energy physics, such as chiral anomaly and axion electrodynamics.
Exciton problem is solved in the two-dimensional Dirac model with allowance for strong electron-hole attraction. The exciton binding energy is assumed smaller than but comparable to the band gap. The exciton wavefunction is found in the momentum space as a superposition of all four two-particle states including electron and hole states with both positive and negative energies. The matrix element of exciton generation is shown to depend on the additional components of the exciton wavefunction. Both the Coulomb and the Rytova-Keldysh potentials are considered. The dependence of the binding energy on the coupling constant is analyzed for the ground and first excited exciton states. The binding energy and the oscillator strength are studied as functions of the environmental-dependent dielectric constant for real transition metal dichalcogenide monolayers. We demonstrate that the multicomponent nature of the exciton wavefunction is crucial for description of resonant optical properties of two-dimensional Dirac systems.
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