No Arabic abstract
Linewidth-tunable lasers have great application requirements in the fields of high-resolution spectroscopy, optical communications and other industry and scientific research. Here, the switchable plasmonic scattering of the metal particles with plenty of nanogaps is proposed as an effective method to achieve linewidth-tunable random lasers. By using the nonlinear optical effect of the environment medium, the metal particles demonstrate the transition from local scattering of nanogaps with high spatial frequency to traditional Mie scattering free from detail information with increasing the pump power density. Based on these two scattering processes, random lasers can be continuously driven from a narrow-linewidth configuration exhibiting nanogap effect dominated resonances to a broad-linewidth regime of collectively coupling oscillating among nanowires (or nanoflowers), demonstrating the dynamic range of linewidth exceeds two orders of magnitude. This phenomenon may provide a platform for further studying of the conclusive mechanism of random lasing and supply a new approach to tune the linewidth of random lasers for further applications in high-illumination imaging and biology detection.
We report on lasing at visible wavelengths in arrays of ferromagnetic Ni nanodisks overlaid with an organic gain medium. We demonstrate that by placing an organic gain material within the mode volume of the plasmonic nanoparticles both the radiative and, in particular, the high ohmic losses of Ni nanodisk resonances can be compensated. Under increasing pump fluence, the systems exhibit a transition from lattice-modified spontaneous emission to lasing, the latter being characterized by highly directional and sub-nanometer linewidth emission. By breaking the symmetry of the array, we observe tunable multimode lasing at two wavelengths corresponding to the particle periodicity along the two principal directions of the lattice. Our results pave the way for loss-compensated magnetoplasmonic devices and topological photonics.
Propagation of light in a highly scattering medium is among the most fascinating optical effect that everyone experiences on an everyday basis and possesses a number of fundamental problems which have yet to be solved. Conventional wisdom suggests that non-linear effects do not play a significant role because the diffusive nature of scattering acts to spread the intensity, dramatically weakening these effects. We demonstrate the first experimental evidence of lasing on a Raman transition in a bulk three-dimensional random media. From a practical standpoint, Raman transitions allow for spectroscopic analysis of the chemical makeup of the sample. A random Raman laser could serve as a bright Raman source allowing for remote, chemically specific, identification of powders and aerosols. Fundamentally, the first demonstration of this new light source opens up an entire new field of study into non-linear light propagation in turbid media, with the most notable application related to non-invasive biomedical imaging.
Narrow linewidth lasers and optical frequency combs generated with mode-locked lasers revolutionized optical frequency metrology. The advent of soliton Kerr frequency combs in compact crystalline or integrated ring optical microresonators opens new horizons for applications. These combs, as was naturally assumed, however, require narrow-linewidth single-frequency pump lasers. We demonstrate that a regular multi-frequency Fabry-Perot laser diode self-injection locked to an optical whispering gallery mode (WGM) microresonator can be first efficiently transformed to a single-frequency ultra-narrow-linewidth source and then to coherent soliton comb oscillator with low power consumption and possibility of further integration.
Portable mid-infrared (mid-IR) spectroscopy and sensing applications require widely tunable, narrow linewidth, chip-scale, single-mode sources without sacrificing significant output power. However, no such lasers have been demonstrated beyond 3 $mu$m due to the challenge of building tunable, high quality-factor (Q) on-chip cavities. We demonstrate a tunable, single-mode mid-IR laser at 3.4 $mu$m using a high-Q silicon microring cavity with integrated heaters and a multi-mode Interband Cascade Laser (ICL). We show that the multiple longitudinal modes of an ICL collapse into a single frequency via self-injection locking with an output power of 0.4 mW and achieve an oxide-clad high confinement waveguide microresonator with a loaded Q of $2.8times 10^5$. Using integrated microheaters, our laser exhibits a wide tuning range of 54 nm at 3.4 $mu$m with 3 dB output power variation. We further measure an upper-bound effective linewidth of 9.1 MHz from the locked laser using a scanning Fabry-Perot interferometer. Our design of a single-mode laser based on a tunable high-Q microresonator can be expanded to quantum-cascade lasers at higher wavelengths and lead to the development of compact, portable, high-performance mid-IR sensors for spectroscopic and sensing applications.
We measured the ensemble-averaged spectral correlation functions and statistical distributions of spectral spacing and intensity for lasing modes in weakly scattering systems, and compared them to those of the amplified spontaneous emission spikes. Their dramatic differences illustrated the distinct physical mechanisms. Our numerical simulation revealed that even without reabsorption the number of potential lasing modes might be greatly reduced by local excitation of a weakly scattering system. The lasing modes could be drastically different from the quasimodes of the passive system due to selective amplification of the feedback from the scatterers within the local gain region.