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Ultrafast holography enabled by quantum interference of ultrashort electrons

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 Added by Ivan Madan
 Publication date 2018
  fields Physics
and research's language is English




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Holography relies on the interference between a known reference and a signal of interest to reconstruct both the amplitude and phase of that signal. Commonly performed with photons and electrons, it finds numerous applications in imaging, cryptography and arts. With electrons, the extension of holography to the ultrafast time domain remains a challenge, although it would yield the highest possible combined spatio-temporal resolution. Here, we show that holograms of local electromagnetic fields can be obtained with combined attosecond/nanometer resolution in an ultrafast transmission electron microscope (UEM). Unlike conventional holography, where the signal and the reference are spatially separated and then recombined to interfere, in our method we use electromagnetic fields to split an electron wave function in a quantum coherent superposition of different energy states. In the image plane, spatial modulation of the electron-energy distribution reflects the phase relation between reference and signal fields, which we map via energy-filtered UEM. Beyond imaging applications, this approach allows implementing optically-controlled and spatially-resolved quantum measurements in parallel, providing an efficient and versatile tool for the exploration of electron quantum optics.

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We report experiments demonstrating Quantum Interference Control (QuIC) based on two nonlinear optical absorption processes in semiconductors. We use two optical beams of frequencies $omega$ and $3omega /2$ incident on AlGaAs and measure the injection current due to the interference between 2- and 3-photon absorption processes. We analyze the dependence of the injection current on the intensities and phases of the incident fields.
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Very much like the ubiquitous quantum interference of a single particle with itself, quantum interference of two independent, but indistinguishable, particles is also possible. This interference is a direct result of quantum exchange statistics, however, it is observed only in the joint probability to find the particles in two separated detectors. Here we report the first observation of such interference fringes between two independent and non-interacting electrons in an interferometer proposed by Yurke et al. and Samuelsson et al. Our experiment resembles the Hanbury Brown and Twiss (HBT) experiment, which was performed with classical waves. In the experiment, two independent and mutually incoherent electron beams were each partitioned into two trajectories. The combined four trajectories enclosed an Aharonov-Bohm (AB) flux (but not the two trajectories of a single electron). While individual currents were found to be independent of the AB flux, as expected, the cross-correlation between current fluctuations in two opposite points across the device exhibited strong AB oscillations. This is a direct signature of orbital entanglement between two electrons even though they never interact with each other.
Through a series of transverse magnetic focusing experiments, we show that hot electrons in a two-dimensional electron gas system undergo an ultrafast relaxation when generated by a quantum dot (QD) instead of a quantum point contact (QPC). We find here that QPC hot electrons were well described by the non-interacting Fermi gas model for excitations up to 1.5 meV above the Fermi level of 7.44 meV, whereas QD hot electrons exhibited an energy loss quadratic to the excitation. The energy relaxation was a sizeable fraction of the tested excitations, up to about 55%. With the proposal that the hot electrons are relaxed by the QD immediately after emission, we present a toy model in which a capacitive coupling between the QD and its leads results in a finite, ultrafast energy relaxation.
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We present a dispersive imaging method for trapped quantum gases based on digital off-axis holography. Both phase delay and intensity of the probe field are determined from the same image. Due to the heterodyne gain inherent to the holographic method it is possible to retrieve the phase delay induced by the atoms at probe beam doses two orders of magnitude lower than phase-contrast imaging methods. Using the full field of the probe beam we numerically correct for image defocusing.
Holography is a cornerstone characterisation and imaging technique that can be applied to the full electromagnetic spectrum, from X-rays to radio waves or even particles such as neutrons. The key property in all these holographic approaches is coherence that is required to extract the phase information through interference with a reference beam - without this, holography is not possible. Here we introduce a holographic imaging approach that operates on intrinsically incoherent and unpolarised beams, so that no phase information can be extracted from a classical interference measurement. Instead, the holographic information is encoded in the second order coherence of entangled states of light. Using spatial-polarisation hyper-entangled photons pairs, we remotely reconstruct phase images of complex objects. Information is encoded into the polarisation degree of the entangled state, allowing us to image through dynamic phase disorder and even in the presence of strong classical noise, with enhanced spatial resolution compared to classical coherent holographic systems. Beyond imaging, quantum holography quantifies hyper-entanglement distributed over 10^4 modes via a spatially-resolved Clauser-Horne-Shimony-Holt inequality measurement, with applications in quantum state characterisation.
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