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The microscopic mechanism behind the fission-barrier asymmetry (II): The rare-earth region $50 < Z < 82$ and $82 < N < 126$

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 Added by Takatoshi Ichikawa
 Publication date 2018
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and research's language is English




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It is well known that most actinides fission into fragments of unequal size. The first attempt to understand this difference suggested that division leading to one of the fragments being near doubly magic $^{132}$Sn is favored by gain in binding energy. After the Strutinsky shell-correction method was developed an alternative idea that gained popularity was that the fission saddle might be lower for mass-asymmetric shapes and that this asymmetry was preserved until scission. Recently it was observed [Phys. Rev. Lett. {bf 105} (2010) 252502] that $^{180}$Hg preferentially fissions asymmetrically in contradiction to the fragment-magic-shell expectation which suggested symmetric division peaked around $^{90}$Zr, with its magic neutron number $N=50$, so it was presented as a new type of asymmetric fission. However, in a paper [Phys. Lett. 34B (1971) 349] a simple microscopic mechanism behind the asymmetry of the actinide fission saddle points was proposed to be related the coupling between levels of type [40$LambdaOmega$] and [51$LambdaOmega$]. The paper then generalizes this idea and made the remarkable prediction that analogous features could exist in other regions. In particular it was proposed that in the rare-earth region couplings between levels of type [30$LambdaOmega$] and [41$LambdaOmega$] would favor mass-asymmetric outer saddle shapes. In this picture the asymmetry of $^{180}$Hg is not a new type of asymmetric fission but of analogous origin as the asymmetry of actinide fission. This prediction has never been cited in the discussion of the recently observed fission asymmetries in the new region of asymmetry, in nuclear physics also referred to as the rare-earth region. We show by detailed analysis that the mechanism of the saddle asymmetry in the sub-Pb region is indeed the one predicted half a century ago.



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We revisit the studies of the isotopic shift in the charge radii of {it even-even} isotopes of Sn and Pb nuclei at $N$ = 82, and 126, respectively, within the relativistic mean-field and Relativistic-Hartree-Bogoliubov approach. The shell model is also used to estimate isotopic shift in these nuclei, for the first time, to the best of our knowledge. The ground state single-particle energies ($spe$) are calculated for non-linear NL3 & NL3$^*$ and density-dependent DD-ME2 parameter sets compared with the experimental data, wherever available. We establish a correlation between the filling of single-particle levels and the isotopic shift in occupation probabilities. The obtained $spe$ from the relativistic mean-field and Relativistic-Hartree-Bogoliubov approaches are in line with those used in the shell model and experimental data for both the Sn and Pb isotopic chains. The shell model calculated isotopic shift agrees with relativistic mean-field and Relativistic-Hartree-Bogoliubov approaches that explain the experimental data quite well.
In this work, we identify a unique and novel feature of central density depletion in both proton and neutron named as doubly bubble nuclei in 50$leq$Z(N)$leq$82 region. The major role of 2d-3s single-particle (s.p.) states in the existence of halo and bubble nuclei is probed. The occupancy in s.p. state 3s$_{1/2}$ leads to the extended neutron density distribution or halo while the unoccupancy results in the central density depletion. By employing the Relativistic Mean-Field (RMF) approach along with NL3* parameter, the separation energies, single-particle energies, pairing energies, proton, and neutron density profiles along with deformations of even-even nuclei are investigated. Our results are in concise with few other theories and available experimental data. Emergence on new shell closure and the magicity of conventional shell closures are explored systematically in this yet unknown region.
We probe the $N=82$ nuclear shell closure by mass measurements of neutron-rich cadmium isotopes with the ISOLTRAP spectrometer at ISOLDE-CERN. The new mass of $^{132}$Cd offers the first value of the $N=82$, two-neutron shell gap below $Z=50$ and confirms the phenomenon of mutually enhanced magicity at $^{132}$Sn. Using the recently implemented phase-imaging ion-cyclotron-resonance method, the ordering of the low-lying isomers in $^{129}$Cd and their energies are determined. The new experimental findings are used to test large-scale shell-model, mean-field and beyond-mean-field calculations, as well as the ab initio valence-space in-medium similarity renormalization group.
Presence of closed proton and/or neutron shells causes deviation from macroscopic properties of nuclei which are understood in terms of the liquid drop model. It is important to investigate experimentally the stabilizing effects of shell closure, if any, against fission. This work aims to investigate probable effects of proton shell ($Z = 82$) closure in the compound nucleus, in enhancing survival probability of the evaporation residues formed in heavy ion-induced fusion-fission reactions. Evaporation residue cross sections have been measured for the reactions $^{19}$F+$^{180}$Hf, $^{19}$F+$^{181}$Ta and $^{19}$F+$^{182}$W from $simeq9%$ below to $simeq42%$ above the Coulomb barrier, leading to formation of compound nuclei with same number of neutrons ($N = 118$) but different number of protons across $Z = 82$. Measured excitation functions have been compared with statistical model calculation, in which reduced dissipation coefficient is the only adjustable parameter. Evaporation residue cross section, normalized by capture cross section, is found to decrease gradually with increasing fissility of the compound nucleus. Measured evaporation residue cross sections require inclusion of nuclear viscosity in the model calculations. Reduced dissipation coefficient in the range of 1textendash3 $times$ $10^{21}$ s$^{-1}$ reproduces the data quite well. No abrupt enhancement of evaporation residue cross sections has been observed in the reaction forming compound nucleus with $Z = 82$. Thus, this work does not find enhanced stabilizing effects of $Z = 82$ shell closure against fission in the compound nucleus. One may attempt to measure cross sections of individual exit channels for further confirmation of our observation.
81 - C.-B. Moon , P. Lee , C. S. Lee 2015
We study for the first time the internal structure of 140Te through the beta-delayed gamma-ray spectroscopy of 140Sb. The very neutron-rich 140Sb, Z = 51 and N = 89, ions were produced by the in-flight fission of 238U beam on a 9Be target at 345 MeV per nucleon at the Radioactive Ion Beam Factory, RIKEN. The half-life and spin-parity of 140Sb are reported as 124(30) ms and (4-), respectively. In addition to the excited states of 140Te produced by the beta-decay branch, the beta-delayed one-neutron and two-neutron emission branches were also established. By identifying the first 2+ and 4+ excited states of 140Te, we found that Te isotopes persist their vibrator character with E(4+)/E(2+) = 2. We discuss the distinctive features manifest in this region, such as valence neutron symmetry and asymmetry, revealed in pairs of isotopes with the same neutron holes and particles with respect to N = 82.
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