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Register a new userDynamical response of a radiative thermal transistor based on suspended insulator-metal transition membranes
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We investigate the dynamical control of the heat flux exchanged in near-field regime between a membrane made with a phase-change material and a substrate when the temperature of the membrane is tuned around its critical value. We show that in interaction with an external source of thermal radiation, this system is multistable and behaves as a thermal transistor, being able to dynamically modulate and even amplify super-Planckian heat fluxes. This behavior could be used to dynamically control heat fluxes exchanged at the nanoscale in systems out of thermal equilibrium and to process thermal information employing suspended membranes.
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Studying thermal transport at the nanoscale poses formidable experimental challenges due both to the physics of the measurement process and to the issues of accuracy and reproducibility. The laser-induced transient thermal grating (TTG) technique permits non-contact measurements on nanostructured samples without a need for metal heaters or any other extraneous structures, offering the advantage of inherently high absolute accuracy. We present a review of recent studies of thermal transport in nanoscale silicon membranes using the TTG technique. An overview of the methodology, including an analysis of measurements errors, is followed by a discussion of new findings obtained from measurements on both solid and nanopatterned membranes. The most important results have been a direct observation of non-diffusive phonon-mediated transport at room temperature and measurements of thickness-dependent thermal conductivity of suspended membranes across a wide thickness range, showing good agreement with first-principles-based theory assuming diffuse scattering at the boundaries. Measurements on a membrane with a periodic pattern of nanosized holes indicated fully diffusive transport and yielded thermal diffusivity values in agreement with Monte Carlo simulations. Based on the results obtained to-date, we conclude that room-temperature thermal transport in membranebased silicon nanostructures is now reasonably well understood.
A suspended system for measuring the thermal properties of membranes is presented. The sensitive thermal measurement is based on the 3$omega$ dynamic method coupled to a V$ddot{o}$lklein geometry. The device obtained using micro-machining processes allows the measurement of the in-plane thermal conductivity of a membrane with a sensitivity of less than 10nW/K (+/-$5x10^{-3}$Wm$^{-1}K^{-1}$ at room temperature) and a very high resolution ($Delta K/K =10^{-3}$). A transducer (heater/thermometer) centered on the membrane is used to create an oscillation of the heat flux and to measure the temperature oscillation at the third harmonic using a Wheatstone bridge set-up. Power as low as 0.1nanoWatt has been measured at room temperature. The method has been applied to measure thermal properties of low stress silicon nitride and polycrystalline diamond membranes with thickness ranging from 100 nm to 400 nm. The thermal conductivity measured on the polycrystalline diamond membrane support a significant grain size effect on the thermal transport.
The celebrated Wiedemann-Franz (WF) law is believed to be robust in metals as long as interactions between electrons preserve their fermion-quasiparticle character. We study thermal transport and the fate of the WF law close to a continuous metal-insulator transition (MIT) in the Falicov-Kimball model (FKM) using cluster-dynamical mean-field theory (CDMFT). Surprisingly, as for electrical transport, we find robust and novel quantum critical scaling in thermal transport across the MIT. We unearth the deeper reasons for these novel findings in terms of (i) the specific structure of energy-current correlations for the FKM and (ii) the microscopic electronic processes which facil- itate energy transport while simultaneously blocking charge transport close to the MIT. However, within (C)DMFT, we also find that the WF law survives at T=0 in the incoherent metal right up to the MIT, even in absence of Landau quasiparticles.
A wide range of disordered materials, including disordered correlated systems, show Universal Dielectric Response (UDR), followed by a superlinear power-law increase in their optical responses over exceptionally broad frequency regimes. While extensively used in various contexts over the years, the microscopics underpinning UDR remains controversial. Here, we investigate the optical response of the simplest model of correlated fermions, Falicov-Kimball model (FKM), across the continuous metal-insulator transition (MIT) and analyze the associated quantum criticality in detail using cluster extension of dynamical mean field theory (CDMFT). Surprisingly, we find that UDR naturally emerges in the quantum critical region associated with the continuous MIT. We tie the emergence of these novel features to a many-body orthogonality catastrophe accompanying the onset of strongly correlated electronic glassy dynamics close to the MIT, providing a microscopic realization of Jonschers time-honored proposal as well as a rationale for similarities in optical responses between correlated electronic matter and canonical glass formers.
In a family of experiments carried on all-metallic supercurrent nano-transistors a surprising gating effect has been recently shown. These include the full suppression of the critical supercurrent, the increase of quasiparticle population, the manipulation of the superconducting phase, and the broadening of the switching current distributions. Aside from the high potential for future applications, these findings raised fundamental questions on the origin of these phenomena. To date, two complementary hypotheses are under debate: an electrostatically-triggered orbital polarization at the superconductor surface, or the injection of highly-energetic quasiparticles extracted from the gate. Here, we tackle this crucial issue via a fully suspended gate-controlled Ti nano-transistor. Our geometry allows to eliminate any direct injection of quasiparticles through the substrate thereby making cold electron field emission through the vacuum the only possible charge transport mechanism. With the aid of a fully numerical 3D model in combination with the observed phenomenology and thermal considerations we can rule out, with any realistic likelihood, the occurrence of cold electron field emission. Excluding these two trivial phenomena is pivotal in light of understanding the microscopic nature of gating effect in superconducting nanostructures, which represents an unsolved puzzle in contemporary superconductivity. Yet, from the technological point of view, our suspended fabrication technique provides the enabling technology to implement a variety of applications and fundamental studies combining, for instance, superconductivity with nano-mechanics.
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